Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

The role of absorption saturation and amplified spontaneous emission in cryogenic optical refrigeration

Mansoor Sheik‐Bahae, Jackson L. Kock

Published Mar 4, 2022• 2 citations
Publisher

Abstract

The effects of amplified spontaneous emission (ASE) as well as absorption saturation in cryogenic optical refrigeration in rare-earth doped materials are analyzed theoretically. It is seen that ASE may pose a limitation on power scaling under strong feedback conditions (i.e. in high finesse pump circulator cavities). Absorption saturation may have similar effect depending on the value of the background absorption.

DOI
10.1117/12.2615924

Related papers

Bidirectional description of amplified spontaneous emission induced by three-photon absorption

Alexander S. Baev, Viktor Kimberg, Sergey P. Polyutov +2 more

A semiclassical dynamic theory of the nonlinear propagation of a few interacting intense light pulses is applied to study the nonlinear counterpropagation of amplified spontaneous emission (ASE) induced by three-photon absorption of short intense laser pulses in a chromophore solution. Several important results from the modeling are reached for the ASE process developing in the regime of strong saturation. Accounting for ASE in both forward and backward directions with respect to the pump pulse results in a smaller efficiency of nonlinear conversion for the forward ASE compared with the case in which forward emission is considered alone, something that results from the partial repump of the absorbed energy to the backward ASE component; the overall efficiency is nevertheless higher than for the forward emission considered alone. The efficiency of nonlinear conversion of the pump energy to the counterpropagating ASE pulses is strongly dependent on the concentration of active molecules so that a particular combination of concentration versus cell length optimizes the conversion coefficient. Under certain specified conditions, the ASE effect is found to be oscillatory; the origin of oscillations is dynamical competition between stimulated emission and off-resonant absorption. This result can be considered one of the possible explanations of the temporal fluctuations of the forward ASE pulse [Nature 415, 767 (2002)].

Journal of the Optical Society of America B•Feb 1, 2005•8 citations

Theory of optical-gain measurements

Peter S. Cross, William G. Oldham

The widely used technique for determining optical gain and absorption from single-pass, amplified spontaneous emission (ASE) is analyzed with particular attention given to active-volume saturation and three-dimensional effects. The results for homogeneously broadened media show that the population inversion and hence the gain in the active region is diminished by high levels of spontaneous and ASE. The externally measured gain is further reduced for large output collection apertures that admit incompletely amplified off-axis rays. Criteria are given for the excitation and detection geometries required to ensure accurate (∼10-percent) gain measurement. The simultaneous measurement of the equilibrium absorption coefficient can be made under less restrictive conditions.

IEEE Journal of Quantum Electronics•May 1, 1975•66 citations

Energy extraction from pulsed amplified stimulated emission lasers operating under conditions of strong saturation

S. M. Hooker, David James Spence

The output of pulsed, homogeneously broadened amplified spontaneous emission (ASE) lasers operating under conditions of strong saturation is considered. An expression for the maximum power (energy) per unit volume that may be extracted from steady-state (pulsed) systems is derived and shown to be independent of the saturation intensity. Numerical calculations of the temporal evolution of the populations in the laser levels and the growth in the ASE fluence, peak intensity, and spectral width are presented for three types of laser system: quasi steady state, short pump pulses, and self-termination. In all cases the growth in the fluence of the ASE pulse is found to agree with an analytic solution derived for conditions of strong saturation. The calculated growth in intensity of the ASE pulse is compared with expressions derived by Pert [J. Opt. Soc. Am. B11, 1425 (1994)] for the steady-state case. As expected, good agreement is found for the quasi-steady-state system, but in the limit of strong saturation significant differences occur for the short pump pulse and self-terminating laser systems considered. For all cases considered, the variation of the spectral width of the ASE pulse is found to be in reasonable agreement with that predicted by Pert for steady-state conditions.

Journal of the Optical Society of America B•Jun 1, 2006•2 citations

Second-order coherence properties of amplified spontaneous emission

Iliya V. Doronin, E. S. Andrianov, A. A. Zyablovsky +4 more

Properties of light sources based on amplified spontaneous emission (ASE) are similar to the properties of lasers in many regards. However, even though ASE has been widely studied, its photon statistics have not been settled. There are no reliable theoretical estimates or unambiguous experimental data for the second-order coherence function of photons that characterizes the coherence properties of a light source. Our computer simulation clearly establishes that, independently of pump power, the light produced by ASE is similar to that of a thermal source. This result lays bare the fundamental difference between ASE radiation and laser radiation.

Optics Express•Apr 4, 2019•28 citations

Purcell-enhanced optical refrigeration

Peng Ju, Kunhong Shen, Stefan Püschel +3 more

Optical refrigeration of solids with anti-Stokes fluorescence has been widely explored as a vibration-free cryogenic cooling technology. A minimum temperature of 87 K has been demonstrated with rare-earth-ion-doped crystals using optical refrigeration. However, the depletion of the upper-lying energy levels in the ground-state manifold hinders further cooling to below the liquid nitrogen ( LN 2 ) temperatures, restricting its applications. In this work, we introduce a Purcell-enhanced optical refrigeration method to circumvent this limitation. This approach enhances the emission of high-energy photons by coupling the emitters to an optical cavity, blueshifting the mean emission wavelength. Such Purcell-enhanced emission facilitates cooling starting from a lower-energy level in the ground-state manifold, which exhibits a higher occupation below the LN 2 temperatures. Using experimentally measured optical coefficients, our theoretical analysis predicts a minimum achievable internal temperature of about 38 K for a Yb 3 + : YLiF 4 nanocrystal near a cavity under realistic conditions. The proposed method is applicable to other rare-earth-ion-doped materials and semiconductors and will have applications in creating superconducting and other quantum devices through solid-state cooling.

arXiv:2404.19142•Physical Review Research•Mar 21, 2026•2 citations

Laser cooling in solids: advances and prospects

Denis V. Seletskiy, Richard I. Epstein, Mansoor Sheik‐Bahae

This review discusses the progress and ongoing efforts in optical refrigeration. Optical refrigeration is a process in which phonons are removed from a solid by anti-Stokes fluorescence. The review first summarizes the history of optical refrigeration, noting the success in cooling rare-earth-doped solids to cryogenic temperatures. It then examines in detail a four-level model of rare-earth-based optical refrigeration. This model elucidates the essential roles that the various material parameters, such as the spacing of the energy levels and the radiative quantum efficiency, play in the process of optical refrigeration. The review then describes the experimental techniques for cryogenic optical refrigeration of rare-earth-doped solids employing non-resonant and resonant optical cavities. It then examines the work on laser cooling of semiconductors, emphasizing the differences between optical refrigeration of semiconductors and rare-earth-doped solids and the new challenges and advantages of semiconductors. It then describes the significant experimental results including the observed optical refrigeration of CdS nanostructures. The review concludes by discussing the engineering challenges to the development of practical optical refrigerators, and the potential advantages and uses of these refrigerators.

Reports on Progress in Physics•Aug 3, 2016•126 citations
The effects of amplified spontaneous emission (ASE) as well as absorption saturation in cryogenic optical refrigeration in rare-earth doped materials are analyzed theoretically. It is seen that ASE may pose a limitation on power scaling under strong feedback conditions (i.e. in high finesse pump circulator cavities). Absorption saturation may have similar effect depending on the value of the background absorption.
A semiclassical dynamic theory of the nonlinear propagation of a few interacting intense light pulses is applied to study the nonlinear counterpropagation of amplified spontaneous emission (ASE) induced by three-photon absorption of short intense laser pulses in a chromophore solution. Several important results from the modeling are reached for the ASE process developing in the regime of strong saturation. Accounting for ASE in both forward and backward directions with respect to the pump pulse results in a smaller efficiency of nonlinear conversion for the forward ASE compared with the case in which forward emission is considered alone, something that results from the partial repump of the absorbed energy to the backward ASE component; the overall efficiency is nevertheless higher than for the forward emission considered alone. The efficiency of nonlinear conversion of the pump energy to the counterpropagating ASE pulses is strongly dependent on the concentration of active molecules so that a particular combination of concentration versus cell length optimizes the conversion coefficient. Under certain specified conditions, the ASE effect is found to be oscillatory; the origin of oscillations is dynamical competition between stimulated emission and off-resonant absorption. This result can be considered one of the possible explanations of the temporal fluctuations of the forward ASE pulse [Nature 415, 767 (2002)].
The widely used technique for determining optical gain and absorption from single-pass, amplified spontaneous emission (ASE) is analyzed with particular attention given to active-volume saturation and three-dimensional effects. The results for homogeneously broadened media show that the population inversion and hence the gain in the active region is diminished by high levels of spontaneous and ASE. The externally measured gain is further reduced for large output collection apertures that admit incompletely amplified off-axis rays. Criteria are given for the excitation and detection geometries required to ensure accurate (∼10-percent) gain measurement. The simultaneous measurement of the equilibrium absorption coefficient can be made under less restrictive conditions.
The output of pulsed, homogeneously broadened amplified spontaneous emission (ASE) lasers operating under conditions of strong saturation is considered. An expression for the maximum power (energy) per unit volume that may be extracted from steady-state (pulsed) systems is derived and shown to be independent of the saturation intensity. Numerical calculations of the temporal evolution of the populations in the laser levels and the growth in the ASE fluence, peak intensity, and spectral width are presented for three types of laser system: quasi steady state, short pump pulses, and self-termination. In all cases the growth in the fluence of the ASE pulse is found to agree with an analytic solution derived for conditions of strong saturation. The calculated growth in intensity of the ASE pulse is compared with expressions derived by Pert [J. Opt. Soc. Am. B11, 1425 (1994)] for the steady-state case. As expected, good agreement is found for the quasi-steady-state system, but in the limit of strong saturation significant differences occur for the short pump pulse and self-terminating laser systems considered. For all cases considered, the variation of the spectral width of the ASE pulse is found to be in reasonable agreement with that predicted by Pert for steady-state conditions.
Properties of light sources based on amplified spontaneous emission (ASE) are similar to the properties of lasers in many regards. However, even though ASE has been widely studied, its photon statistics have not been settled. There are no reliable theoretical estimates or unambiguous experimental data for the second-order coherence function of photons that characterizes the coherence properties of a light source. Our computer simulation clearly establishes that, independently of pump power, the light produced by ASE is similar to that of a thermal source. This result lays bare the fundamental difference between ASE radiation and laser radiation.
Optical refrigeration of solids with anti-Stokes fluorescence has been widely explored as a vibration-free cryogenic cooling technology. A minimum temperature of 87 K has been demonstrated with rare-earth-ion-doped crystals using optical refrigeration. However, the depletion of the upper-lying energy levels in the ground-state manifold hinders further cooling to below the liquid nitrogen ( LN 2 ) temperatures, restricting its applications. In this work, we introduce a Purcell-enhanced optical refrigeration method to circumvent this limitation. This approach enhances the emission of high-energy photons by coupling the emitters to an optical cavity, blueshifting the mean emission wavelength. Such Purcell-enhanced emission facilitates cooling starting from a lower-energy level in the ground-state manifold, which exhibits a higher occupation below the LN 2 temperatures. Using experimentally measured optical coefficients, our theoretical analysis predicts a minimum achievable internal temperature of about 38 K for a Yb 3 + : YLiF 4 nanocrystal near a cavity under realistic conditions. The proposed method is applicable to other rare-earth-ion-doped materials and semiconductors and will have applications in creating superconducting and other quantum devices through solid-state cooling.
This review discusses the progress and ongoing efforts in optical refrigeration. Optical refrigeration is a process in which phonons are removed from a solid by anti-Stokes fluorescence. The review first summarizes the history of optical refrigeration, noting the success in cooling rare-earth-doped solids to cryogenic temperatures. It then examines in detail a four-level model of rare-earth-based optical refrigeration. This model elucidates the essential roles that the various material parameters, such as the spacing of the energy levels and the radiative quantum efficiency, play in the process of optical refrigeration. The review then describes the experimental techniques for cryogenic optical refrigeration of rare-earth-doped solids employing non-resonant and resonant optical cavities. It then examines the work on laser cooling of semiconductors, emphasizing the differences between optical refrigeration of semiconductors and rare-earth-doped solids and the new challenges and advantages of semiconductors. It then describes the significant experimental results including the observed optical refrigeration of CdS nanostructures. The review concludes by discussing the engineering challenges to the development of practical optical refrigerators, and the potential advantages and uses of these refrigerators.