A principal goal of distributed quantum processing is the ability to generate, manipulate, and transfer quantum states between distant nodes of a quantum network. These protocols generally require connecting photonic and material carriers of quantum information. Here we present two experimental realizations of light-matter interfaces that allow for engineered atom-photon interactions in free-space settings. First, we utilize reconfigurable arrays of trapped single atoms to study light scattering in low-dimensional systems. We observe noncollinear phase-matching geometries that have suppressed sensitivity to particle localization. We show that the scattered radiation can be controllably enhanced or diminished as a result of Bragg interference. Such scattering can be used for mapping collective states within an array of neutral atoms onto propagating light fields and for establishing quantum links between separated arrays. Second, we create a quasi-two-level system in a regime of Rydberg excitation blockade for a mesoscopic ensemble of several hundred atoms confined in a magic-wavelength optical lattice. We demonstrate coherent driving and Ramsey interference measurements of light shifts, with timescales on the order of ∼ 10 μs. Whereas the coupling producing the Rabi oscillations is enhanced by a factor of √N, there is no corresponding enhancement for the light shifts. These results may prove useful in applying collective qubits with Rydberg interactions to scalable quantum networking architectures.
A principal goal of distributed quantum processing is the ability to generate, manipulate, and transfer quantum states between distant nodes of a quantum network. These protocols generally require connecting photonic and material carriers of quantum information. Here we present two experimental realizations of light-matter interfaces that allow for engineered atom-photon interactions in free-space settings. First, we utilize reconfigurable arrays of trapped single atoms to study light scattering in low-dimensional systems. We observe noncollinear phase-matching geometries that have suppressed sensitivity to particle localization. We show that the scattered radiation can be controllably enhanced or diminished as a result of Bragg interference. Such scattering can be used for mapping collective states within an array of neutral atoms onto propagating light fields and for establishing quantum links between separated arrays. Second, we create a quasi-two-level system in a regime of Rydberg excitation blockade for a mesoscopic ensemble of several hundred atoms confined in a magic-wavelength optical lattice. We demonstrate coherent driving and Ramsey interference measurements of light shifts, with timescales on the order of ∼ 10 μs. Whereas the coupling producing the Rabi oscillations is enhanced by a factor of √N, there is no corresponding enhancement for the light shifts. These results may prove useful in applying collective qubits with Rydberg interactions to scalable quantum networking architectures.
A principal goal of distributed quantum processing is the ability to generate, manipulate, and transfer quantum states between distant nodes of a quantum network. These protocols generally require connecting photonic and material carriers of quantum information. In this thesis, I present investigations of two experimental realizations of light-matter interfaces that allow for engineered atom-photon interactions in free-space settings. First, we utilize reconfigurable arrays of trapped single atoms to study light scattering in lowdimensional systems. We observe noncollinear phase-matching geometries that have suppressed sensitivity to particle localization. We show that the scattered radiation can be controllably enhanced or diminished as a result of Bragg interference. Such scattering can be used for mapping collective states within an array of neutral atoms onto propagating light fields and for establishing quantum links between separated arrays. Second, we utilize ensembles of trapped Rydberg atoms to study collective many-body phenomena that arise due to strong dipole-dipole interactions. To do so, we employ a magic-wavelength optical lattice that allows for the simultaneous trapping of both ground and Rydberg levels. Using the enhanced coherence times enabled by this trapping scheme, we measure the so-called magic lattice detunings and use them to extract the 6P3/2 − nS1/2 reduced electric dipole matrix elements. Furthermore, we perform precision measurements of differential nuclear-spin dependent light shifts in the Paschen-Back regime in order to determine the hyperfine splitting of Rydberg levels. We create a quasi-two-level system in a regime of Rydberg excitation blockade for a mesoscopic ensemble of several hundred atoms. Using this system, we study Hanbury Brown-Twiss interference between the field radiated by the atoms and an input probe field with a controllable relative phase. Finally, we demonstrate coherent driving and Ramsey interference measurements of light shifts, with timescales on the order of ≃ 10 µs. Whereas the coupling producing the Rabi oscillations is enhanced, there is no corresponding enhancement for the lightshifts. These results may prove useful in applying collective qubits with Rydberg interactions to scalable quantum networking architectures.
Scalable quantum computers and quantum networks require the combination of quantum processing nodes with efficient light-matter interfaces to distribute quantum information in local or long-distance quantum networks. Neutral-atom arrays have both been coupled to Rydberg states to enable high-fidelity quantum gates in universal processing architectures, and to optical cavities to realize interfaces to photons. However, combining these two capabilities and coupling atom arrays to highly excited Rydberg states in the mode of an optical cavity has been an outstanding challenge. Here we present a novel cavity-coupled Rydberg array that achieves this long-standing goal. We prepare, detect, and control individual atoms in a scalable optical tweezer array, couple them strongly to the optical mode of a high-finesse optical cavity and excite them in a controlled way to Rydberg states. We show that high-cooperativity coupling to an optical cavity -- demonstrated via the dispersive shift of the resonance of the cavity in presence of the atoms -- and strong Rydberg interactions -- demonstrated via the collective enhancement of Rydberg coupling in the atomic array -- can be achieved in our setup at the same spatial location. Our presented experimental platform opens the path to several new directions, including the realization of quantum network nodes, quantum simulation of long-range interacting, open quantum systems and photonic-state engineering leveraging high-fidelity Rydberg control.
Recent experimental advances in preparing regular defect-free 2D arrays of atoms with optical traps have offered new opportunities to engineer strong collective couplings between light and atoms as quantum optical dipoles. Applications of such collective light-matter interactions include the realization of atom-thick mirrors, retrieval of quantum memories with high efficiency, or the implementation of topological quantum optics. I will present novel applications in the context of quantum networking. First, I will discuss the design of a chiral photonic quantum link, where distant single atoms interact by exchanging photons propagating in a unique direction in free space. This is achieved by coupling both single atoms, representing qubits implemented using a pair of Rydberg states, to bi-layer atomic arrays which act as quantum phased-array antennas. Exploiting the combination of a “Rydberg-dressing” laser and a control laser driving the atomic arrays, an effective Rydberg dipole-dipole interaction can be engineered between atoms and atomic arrays as quantum emitters, allowing to match the spatial modes of spontaneously emitted and absorbed photons to a Gaussian mode of interest. In this way, we realize a chiral quantum interface, i.e., where atoms couple to photonic modes with a unique direction of propagation. This setup provides a basic building block of a novel platform for quantum networks in free space, i.e., without requiring coupling atoms to modes of cavities or nanostructures, which I will illustrate with the deterministic coherent transfer of quantum states between single atoms with high fidelity. Second, I will discuss the collective radiation properties of two distant single-layer atomic arrays acting as quantum memories. This system can support a long-lived non-local superposition state of atomic excitations exhibiting strong subradiance. This “dark” mode consists of an atomic excitation which is delocalized between the two distant atomic arrays, in such a way that the overall radiation is strongly suppressed by quantum interference. I will describe the preparation of these states and their application as resource of non-local entanglement. In particular, by weakly driving the arrays, the state of the quantum memories, localized in each array, can be transferred to this “non-local” subradiant state, allowing again for a deterministic coherent quantum state transfer with high fidelity between the memories. Finally, I will discuss experimental realizations using cold atoms in optical trap arrays, and the effect of experimental imperfections in the arrays, such as finite defect probability, temperature, and depth of the optical traps.
Integrating Rydberg-state control of atom-atom interactions with cavity control of atom-light interactions enables the combination of local entangling operations with photon-mediated long-range coupling, measurement, and communication. Such integration is challenging because electric fields generated by charges on cavity optics and by cavity-stabilizing actuators may disturb Rydberg-state coherence. Here, we couple a Rydberg tweezer array to a high-cooperativity optical cavity, suppressing the electric fields produced by cavity length actuation so that the residual field variation of about 3mV/cm rms does not limit Rydberg coherence. We demonstrate two capabilities that neither system provides alone. First, we use Purcell-enhanced fluorescence to read out atoms directly in the ground-Rydberg basis within 7.5μs, well within the Rydberg-state lifetime, with ground- and Rydberg-state detection infidelities of 3% and 5%, respectively, and with low atom loss. Second, we use Rydberg-Rydberg interactions to control collective light-atom scattering into the cavity mode. Specifically, we drive blockaded Rabi oscillations between a state with two ground-state atoms, which scatter collectively with a superradiant or subradiant rate controlled by the atomic positions, and an entangled state with a single Rydberg excitation, which scatters like a single atom. These capabilities open routes toward networked Rydberg processors, mid-circuit measurements in analog quantum simulators, and many-body quantum optics with entangled emitters coupled collectively to light.
Rydberg interactions of trapped alkali-metal atoms are used widely to facilitate quantum gate operations in quantum processors and repeaters. In most laboratory realizations using this protocol, the Rydberg states are repelled by the trapping laser fields, requiring that the fields be turned off during gate operations. Here we create a quasi-two-level system in a regime of Rydberg excitation blockade for a mesoscopic Rb ensemble of several hundred atoms confined in a magic-wavelength optical lattice. We observe many-body Rabi oscillations between the ground and collective Rydberg state. In addition we use Ramsey interference techniques to obtain the light shifts of both the lower and upper states of the collective qubit. Whereas the coupling producing the Rabi oscillations is enhanced by a factor of sqrt[N], there is no corresponding enhancement for the light shifts. We derive an effective two-level model which is in good agreement with our observations. Trapped Rydberg qubits and an effective two-level description are expected to have broad applicability for studies of quantum simulation and networking using collective encoding in ensembles of neutral atoms.
We present a complete protocol for cavity-free quantum networking based on collective enhancement in Rydberg atom ensembles. The scheme combines Rydberg blockade, collectively enhanced light--matter coupling, and phase-matched directional emission to remove the need for optical cavities while retaining efficiencies comparable to cavity-assisted interfaces. The protocol proceeds in three steps: (i)~local control--ensemble entanglement generated by Rydberg blockade with gate fidelity Fgate≈99.93%; (ii)~atom--photon conversion through Raman emission from an oblate spheroidal ensemble, yielding directional emission efficiency ηdir≈73% and single-node efficiency ηnode≈40%; and (iii)~remote atom--atom entanglement via Hong--Ou--Mandel interference, producing Bell states with fidelity F>97.5%. Incorporating quantum memories allows up to M≈100 retry attempts within a coherence time T2>100μs, enabling entanglement generation rates of approximately 4kHz over a 20~km separation. Collectively enhanced Rydberg ensembles thus provide a practical, cavity-free interface for scalable distributed quantum computing and secure quantum communication.