Recent developments in opto-optical modulation technique calls for improved temporal control of light modulation processes of coherent XUV light. This thesis project evaluates an experimental method aimed at achieving redirection and amplitude modulation of XUV-light, by using precise determination of decay times in states of noble gases that are deemed suitable for opto-optical control. It is possible to obtain a higher signal-to-noise ratio than previously possible when performing decay time measurements using a recently developed technique to obtain spatial phase control of the states that are being measured.
We extend the recently developed technique of opto-optical modulation (OOM) to probe state-resolved ac-Stark-induced phase variations of a coherently excited ensemble of helium atoms. In a joint experimental and theoretical study, we find that the spatial redirection of the resonant emission from the OOM process is different for the low-lying
1s2p state as compared with the higher-lying Rydberg states, and that this redirection can be controlled through the spatial characteristics of the infrared (IR) probe beam. In particular, we observe that the intensity dependence of the IR-induced Stark phase on the
1s2p emission is nonlinear, and that the phase accumulation changes sign for moderate intensities. Our results suggest that OOM, combined with precise experimental shaping of the probe beam, could allow future measurements of Stark-induced phase shifts of excited states.
In this work, we present an Opto-Electro-Mechanical Modulator (OEMM) for RF-to-optical transduction realized via an ultra-coherent nanomembrane resonator capacitively coupled to an rf injection circuit made of a microfabricated read-out able to improve the electro-optomechanical interaction. This device configuration can be embedded in a Fabry–Perot cavity for electromagnetic cooling of the LC circuit in a dilution refrigerator exploiting the opto-electro-mechanical interaction. To this aim, an optically measured steady-state frequency shift of 380 Hz was seen with a polarization voltage of 30 V and a Q-factor of the assembled device above 106 at room temperature. The rf-sputtered titanium nitride layer can be made superconductive to develop efficient quantum transducers.