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Optically controlled nano-etching through nearly-forbidden transitions enhanced by the surface structure

Tojo, S., Mashimo, T., Masashi Abe, Takashi Yatsui, Masaki Yamaguchi, Tsuboi, T., Katsuyuki Nobusada, Fabrice Stehlin, Olivier Soppera, Daniel Bloch

Published Mar 24, 2019• 0 citations
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We investigate the mediation of symmetry-forbidden atomic transitions using plasmonic nanostructures. We show that the excitation of the electric dipole-forbidden, quadrupole-allowed $6{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}\ensuremath{-}5{\phantom{\rule{0.16em}{0ex}}}^{2}{D}_{5/2}$ transition in cesium may be enhanced by more than 6 orders of magnitude in the intense, inhomogeneous near field of a plasmonic nanoantenna. Using optical reciprocity, the enhancement can be understood to apply to spontaneous emission as well, allowing the fast and efficient optical detection of excited atoms.