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Acta Physica Sinica

Experimental study of retrieval efficiency of Duan-Lukin-Cirac-Zoller quantum memory by optical cavity-enhanced

Teng-Fei Ma, Minjie Wang, Shengzhi Wang, Haole Jiao, Yan Xie, Shujing Li, Zhongxiao Xu, Hai Wang

Published Jan 1, 2022• 1 citation
Publisher

Abstract

Long-distance entanglement distribution is an important task for quantum communication, but difficult to achieve due to the loss of photons in optical fiber transmission. Quantum repeater is a scheme to solve this problem. In this scheme, the long distance of entanglement distribution is divided into several small parts, the entanglement is established first at both ends of each part, then, the entanglement distance is extended through the entanglement exchange of adjacent interval parts, in order to achieve the long distance entanglement distribution. Of them, the Duan-Lukin-Cirac-Zoller (DLCZ) protocol based on the cold atom ensemble and the linear optics which can generate and store entanglement, is regarded as one of the most potential schemes. In the process of DLCZ, retrieval efficiency is an important index of the quantum repeater, because it will influence each entanglement exchange operation between adjacent quantum repeater nodes. Generally, the retrieval efficiency is improved by optimizing the reading pulse, increasing the optical depth (OD) of the atomic ensemble and the cavity enhancement. The ring cavity constrains the light field to increase the intensity of the interaction between light and atoms, and effectively improve the retrieval efficiency of the quantum memory. In this work, atomic ensembles are placed in a ring cavity. The cavity length is 3.3 m and the fineness is 13.5. The optical loss of all ring cavity is 21%, mainly including 15% loss of other optical elements and 6% loss of the cell. In order to increase the retrieval efficiency, we need to ensure the mode resonance of read-out photon, write-out photon and locking. The cavity needs two input beams of light: one comes from the path of read-out photon and the other from the path of write-out photon in the reverse direction. The two beams are locked at the same frequency as the write-out photon and the read-out photon respectively. The cavity length is adjusted by moving the cavity mirrors’ positions through translating the frame, to make two light modes resonate. The acousto-optic modulator (AOM) is inserted into the path of the locking to control the frequency of the locking. By adjusting the AOM to change the frequency of the locking, the locking can be coincident with the write-out and read-out cavity modes. Then, the three-mode resonance can be achieved When the cavity mode resonates with the atomic line, it will lead the atomic formants to split. thereby affecting the enhancement effect of retrieval efficiency. In the experiment, the detuning of the read light will affect the frequency of the read-out photon, and further affect the detuning of the cavity mode with the resonance line of the atom. Thus, by increasing the detuning between the reading light and the atomic transition line, the frequency splitting between the two modes can be reduced, then enhance the retrieval efficiency. We study the relation between the enhancement factor of the retrieval efficiency and the detuning amount of the reading light relative to the atomic resonance line. The results show that when the detuning amount of reading light is 80 MHz, the intrinsic readout efficiency is 45%, and the readout efficiency is enhanced by 1.68 times.

DOI
10.7498/aps.71.20210881

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Long-distance entanglement distribution is an important task for quantum communication, but difficult to achieve due to the loss of photons in optical fiber transmission. Quantum repeater is a scheme to solve this problem. In this scheme, the long distance of entanglement distribution is divided into several small parts, the entanglement is established first at both ends of each part, then, the entanglement distance is extended through the entanglement exchange of adjacent interval parts, in order to achieve the long distance entanglement distribution. Of them, the Duan-Lukin-Cirac-Zoller (DLCZ) protocol based on the cold atom ensemble and the linear optics which can generate and store entanglement, is regarded as one of the most potential schemes. In the process of DLCZ, retrieval efficiency is an important index of the quantum repeater, because it will influence each entanglement exchange operation between adjacent quantum repeater nodes. Generally, the retrieval efficiency is improved by optimizing the reading pulse, increasing the optical depth (OD) of the atomic ensemble and the cavity enhancement. The ring cavity constrains the light field to increase the intensity of the interaction between light and atoms, and effectively improve the retrieval efficiency of the quantum memory. In this work, atomic ensembles are placed in a ring cavity. The cavity length is 3.3 m and the fineness is 13.5. The optical loss of all ring cavity is 21%, mainly including 15% loss of other optical elements and 6% loss of the cell. In order to increase the retrieval efficiency, we need to ensure the mode resonance of read-out photon, write-out photon and locking. The cavity needs two input beams of light: one comes from the path of read-out photon and the other from the path of write-out photon in the reverse direction. The two beams are locked at the same frequency as the write-out photon and the read-out photon respectively. The cavity length is adjusted by moving the cavity mirrors’ positions through translating the frame, to make two light modes resonate. The acousto-optic modulator (AOM) is inserted into the path of the locking to control the frequency of the locking. By adjusting the AOM to change the frequency of the locking, the locking can be coincident with the write-out and read-out cavity modes. Then, the three-mode resonance can be achieved When the cavity mode resonates with the atomic line, it will lead the atomic formants to split. thereby affecting the enhancement effect of retrieval efficiency. In the experiment, the detuning of the read light will affect the frequency of the read-out photon, and further affect the detuning of the cavity mode with the resonance line of the atom. Thus, by increasing the detuning between the reading light and the atomic transition line, the frequency splitting between the two modes can be reduced, then enhance the retrieval efficiency. We study the relation between the enhancement factor of the retrieval efficiency and the detuning amount of the reading light relative to the atomic resonance line. The results show that when the detuning amount of reading light is 80 MHz, the intrinsic readout efficiency is 45%, and the readout efficiency is enhanced by 1.68 times.
The Duan-Lukin-Cirac-Zoller (DLCZ) process in the atomic ensemble is an important means to generate quantum correlation and entanglement between photons and atoms (quantum interface). When a write pulse acts on atoms, the DLCZ quantum memory process will be generated, which has been extensively studied. In the process a spontaneous Raman scattering (SRS) of a Stokes photon is generated, and a spin-wave excitation stored in the atomic ensemble is created at the same time. The higher probability of the generation of Stokes photons will cause more noise and reduce entanglement. On the contrary, the low generation probability of Stokes photons affects the success probability of entanglement distribution on a quantum repeater. How to increase generation probability of Stokes photons without causing more noise is an urgent problem to be resolved. In this work, a 87Rb atomic ensemble is placed in a standing wave cavity which resonates with the Stokes photon. This cavity has a trip length of 0.6 m and a free spectral range (FSR) of 256 MHz. The optical loss of all the optical elements in this cavity is 9%, of which 4% loss originates from the other optical elements and 5% loss from the vacuum chamber of the magneto-optical trap (MOT). The fineness of the cavity with the cold atoms is measured to be ~19.1. By calculating the total probability of Stokes photon emission out of the cavity, we derive the enhancement factor of this standing wave cavity when the cavity loss is l. When this cavity is locked with PDH frequency locking technique, we observe that the production probability of the Stokes photons is 8.7 times higher than that without cavity due to the optical cavity enhancement effect. Under this condition, the relationship between the generation probability of Stokes photons and the power of write beam is studied. The write excitation probability changes linearly with the power of write beam. This work provides an experimental solution to reducing the noise caused by time multimode operation in DLCZ scheme.
Duan-Lukin-Cirac-Zoller quantum repeater protocol, which was proposed to realize long distance quantum communication, requires usage of quantum memories. Atomic ensembles interacting with optical beams based on off-resonant Raman scattering serve as convenient on-demand quantum memories. Here, a complete free space, three-dimensional theory of the associated read and write process for this quantum memory is worked out with the aim of understanding intrinsic retrieval efficiency. We develop a formalism to calculate the transverse mode structure for the signal and the idler photons and use the formalism to study the intrinsic retrieval efficiency under various configurations. The effects of atomic density fluctuations and atomic motion are incorporated by numerically simulating this system for a range of realistic experimental parameters. We obtain results that describe the variation in the intrinsic retrieval efficiency as a function of the memory storage time for skewed beam configuration at a finite temperature, which provides valuable information for optimization of the retrieval efficiency in experiments.
Practical realization of quantum repeaters requires quantum memories with high retrieval efficiency, multi-mode storage capacities, and long lifetimes. Here, we report a high-retrieval-efficiency and temporally multiplexed atom-photon entanglement source. A train of 12 write pulses in time is applied to a cold atomic ensemble along different directions, which generates temporally multiplexed pairs of Stokes photons and spin waves via Duan-Lukin-Cirac-Zoller processes. The two arms of a polarization interferometer are used to encode photonic qubits of 12 Stokes temporal modes. The multiplexed spin-wave qubits, each of which is entangled with one Stokes qubit, are stored in a "clock" coherence. A ring cavity that resonates simultaneously with the two arms of the interferometer is used to enhance retrieval from the spin-wave qubits, with the intrinsic retrieval efficiency reaching 70.4%. The multiplexed source gives rise to a ∼12.1-fold increase in atom-photon entanglement-generation probability compared to the single-mode source. The measured Bell parameter for the multiplexed atom-photon entanglement is 2.21(2), along with a memory lifetime of up to ∼125 µs.
Duan-Lukin-Cirac-Zoller quantum repeater protocol provides a feasible scheme to implement long-distance quantum communication and large-scale quantum networks. The elementary link, namely the entanglement between two atomic ensembles, is a fundamental component of quantum repeater. For practical quantum repeater, it is required that the elementary link can be prepared with high yield and the spin waves stored in atoms can be efficiently converted into photons on demand. However, so far, such quantum repeater link has not been demonstrated in experiments. Here, we demonstrate a proof-of-principle multiplexed quantum repeater link by entangling two temporally multiplexed quantum memory. Compared with a single-mode link, the successful preparation rate of the multiplexed link is increased by one order of magnitude. By using the cavity-enhanced scheme, the on-demand retrieval efficiency of atomic spin waves is improved to 70%, which is beneficial for the subsequent entanglement swapping between adjacent links. The realization of temporally multiplexed quantum repeater link with high retrieval efficiency lays a foundation for the development of practical quantum networks.
With the accelerating developments in the field of quantum communication, there will be a need for sources of highly quantum single-photons. In addition to communication applications, the purity, brightness, and fidelity of a given single-photon source are intrinsically linked to the success rate and scalability of a range of photonic technologies in quantum computing, metrology, memory, and cryptography. Further, quantum repeater architectures for maintaining quantum information over long distances will become crucial. In these schemes, end-to-end entanglement is generated by establishing entanglement between the ends of several elementary segments, followed by successive entanglement-swapping operations to increase the entanglement distance until it spans the transmission channel. The most widely studied proposal for the practical implementation of a quantum repeater is the Duan-Lukin-Cirac-Zoller (DLCZ) protocol. This consists of off-resonant Raman excitation by a write pulse, which induces a spin-wave excitation in an atomic ensemble and emits a Stokes photon. At a later time, this spin-wave may be read with a high-power resonant pulse, resulting in the emission of an anti-Stokes photon into a well-defined spatial mode. The Stokes photon may be used for entanglement with another ensemble, while the anti-Stokes may be read out for an entanglement-swapping operation. Notably, in the DLCZ protocol, the atomic ensemble serves as both the quantum memory and a heralded single-photon source. Using atomic ensembles for single-photon sources enables the production of highly pure, indistinguishable photons with minimal spectral broadening; however, the generation rate remains a challenge. In the case of DLCZ, the Raman-scattering step is highly probabilistic, reducing the anti-Stokes generation rate considerably. Furthermore, DLCZ requires operation in the low-excitation-probability regime to avoid multiphoton noise contributions. Additionally, the profile of the induced spin wave is suboptimal for readout. To compensate for these drawbacks, in this thesis we report the experimental realization of a variant of DLCZ that leverages collectively enhanced superradiant (SR) emission. Superradiant emission is characterized by intense bursts of photons emitted in a shorter amount of time than independent atomic state decay. By switching to a resonant excitation and optimizing the write profile, the induced spin-wave is primed for readout, thus increasing retrieval efficiency and the level of quantum correlation. We report data for both the DLCZ and SR schemes under similar optical conditions and compare the two. At high write power, the SR protocol exhibits conditional readout probabilities as high as $\sim$1.2\%, compared to $\sim$0.6\% for the DLCZ protocol under the same conditions. We also analyze the temporal distribution of anti-Stokes emission and find a degree of maintenance of the spin-wave profile, even in the anti-Stokes direction.
Quantum communication deals with absolutely secure transfer of classical messages by means of quantum cryptography or faithful transfer of unknown quantum states by means of quantum teleportation between distant sites. The essential element for quantum communication is to create remote entangled pairs of high fidelity. The main difficulty to create such a distant entangled pair is that both photon loss and decoherence grow exponentially with distance. However, with the help of quantum repeater, it is demonstrated that both the entanglement sources and the time needed to create a single distant entangled pair of high fidelity could scale polynomially with the communication length. Here we propose a robust quantum repeater by extending the original Duan-Lukin-Cirac-Zoller (DLCZ) scheme based on atomic ensembles and linear optics. Our protocol entails the advantage of two photon interference, which is more robust than single photon interference used in the DLCZ scheme. In comparison with our previous proposal, the entangled memory qubits are manipulated across long distance, and local entanglement pairs are avoided. Our proposal provides an exciting possibility for realistic long distance quantum communication.