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Nano Letters

Strain-Controlled Quantum Dot Fine Structure for Entangled Photon Generation at 1550 nm

Thomas Lettner, Samuel Gyger, Katharina D. Zeuner, Lucas Schweickert, Stephan Steinhauer, Carl Reuterskiöld-Hedlund, Sandra Stroj, Armando Rastelli, Mattias Hammar, Rinaldo Trotta, Klaus D. Jöns, Val Zwiller

Published Dec 13, 2021• 43 citations
Publisher

Abstract

Entangled photon generation at 1550 nm in the telecom C-band is of critical importance as it enables the realization of quantum communication protocols over long distance using deployed telecommunication infrastructure. InAs epitaxial quantum dots have recently enabled on-demand generation of entangled photons in this wavelength range. However, time-dependent state evolution, caused by the fine-structure splitting, currently limits the fidelity to a specific entangled state. Here, we show fine-structure suppression for InAs quantum dots using micromachined piezoelectric actuators and demonstrate generation of highly entangled photons at 1550 nm. At the lowest fine-structure setting, we obtain a maximum fidelity of 90.0 ± 2.7% (concurrence of 87.5 ± 3.1%). The concurrence remains high also for moderate (weak) temporal filtering, with values close to 80% (50%), corresponding to 30% (80%) of collected photons, respectively. The presented fine-structure control opens the way for exploiting entangled photons from quantum dots in fiber-based quantum communication protocols.

DOI
10.1021/acs.nanolett.1c04024

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Entangled photon generation at 1550 nm in the telecom C-band is of critical importance as it enables the realization of quantum communication protocols over long distance using deployed telecommunication infrastructure. InAs epitaxial quantum dots have recently enabled on-demand generation of entangled photons in this wavelength range. However, time-dependent state evolution, caused by the fine-structure splitting, currently limits the fidelity to a specific entangled state. Here, we show fine-structure suppression for InAs quantum dots using micromachined piezoelectric actuators and demonstrate generation of highly entangled photons at 1550 nm. At the lowest fine-structure setting, we obtain a maximum fidelity of 90.0 ± 2.7% (concurrence of 87.5 ± 3.1%). The concurrence remains high also for moderate (weak) temporal filtering, with values close to 80% (50%), corresponding to 30% (80%) of collected photons, respectively. The presented fine-structure control opens the way for exploiting entangled photons from quantum dots in fiber-based quantum communication protocols.
Entanglement resources are key ingredients of future quantum technologies. If they could be efficiently integrated into a semiconductor platform, a new generation of devices could be envisioned, whose quantum-mechanical functionalities are controlled via the mature semiconductor technology. Epitaxial quantum dots (QDs) embedded in diodes would embody such ideal quantum devices, but a fine-structure splitting (FSS) between the bright exciton states lowers dramatically the degree of entanglement of the sources and hampers severely their real exploitation in the foreseen applications. In this work, we overcome this hurdle using strain-tunable optoelectronic devices, where any QD can be tuned for the emission of photon pairs featuring the highest degree of entanglement ever reported for QDs, with concurrence as high as 0.75 ± 0.02. Furthermore, we study the evolution of Bell's parameters as a function of FSS and demonstrate for the first time that filtering-free violation of Bell's inequalities requires the FSS to be smaller than 1 μeV. This upper limit for the FSS also sets the tuning range of exciton energies (∼1 meV) over which our device operates as an energy-tunable source of highly entangled photons. A moderate temporal filtering further increases the concurrence and the tunability of exciton energies up to 0.82 and 2 meV, respectively, though at the expense of 60% reduction of count rate.
High Resolution Image Download MS PowerPoint Slide Entangled photons are an integral part in quantum optics experiments and a key resource in quantum imaging, quantum communication, and photonic quantum information processing. Making this resource available on-demand has been an ongoing scientific challenge with enormous progress in recent years. Of particular interest is the potential to transmit quantum information over long distances, making photons the only reliable flying qubit. Entangled photons at the telecom C-band could be directly launched into single-mode optical fibers, enabling worldwide quantum communication via existing telecommunication infrastructure. However, the on-demand generation of entangled photons at this desired wavelength window has been elusive. Here, we show a photon pair generation efficiency of 69.9 ± 3.6% in the telecom C-band by an InAs/GaAs semiconductor quantum dot on a metamorphic buffer layer. Using a robust phonon-assisted two-photon excitation scheme we measure a maximum concurrence of 91.4 ± 3.8% and a peak fidelity to the Φ + state of 95.2 ± 1.1%, verifying on-demand generation of strongly entangled photon pairs and marking an important milestone for interfacing quantum light sources with our classical fiber networks.
Fiber-based quantum networks require on-demand sources of entangled photons in the telecom C-band for long distance information transfer. Historically, the field of in-fiber entanglement distribution has been dominated by photons provided via spontaneous processes. In recent years, semiconductor quantum dots have emerged as strong competitors in terms of generating single and entangled photons due to their promise of deterministic qubit generation in the NIR wavelength region. Here, we show the on-demand generation of polarization entangled photons in the telecom C-band based on InAs/GaAs quantum dots grown via metal-organic vapor-phase epitaxy. By employing a robust phonon-assisted two-photon excitation scheme, we are able to generate pairs of entangled photons with a concurrence of 91.4 ± 3.8 % and a maximum fidelity to the Bell state Φ+ of 95.2 ± 1.1 %.
We report on the observation of nearly maximally entangled photon pairs from semiconductor quantum dots, without resorting to postselection techniques. We use GaAs quantum dots integrated on a patterned piezoelectric actuator capable of suppressing the exciton fine structure splitting. By using a resonant two-photon excitation, we coherently drive the biexciton state and demonstrate experimentally that our device generates polarization-entangled photons with a fidelity of 0.978(5) and a concurrence of 0.97(1) taking into account the nonidealities stemming from the experimental setup. By combining fine-structure-dependent fidelity measurements and a theoretical model, we identify an exciton spin-scattering process as a possible residual decoherence mechanism. We suggest that this imperfection may be overcome using a modest Purcell enhancement so as to achieve fidelities >0.99, thus making quantum dots evenly matched with the best probabilistic entangled photon sources.
Abstract Long-distance quantum communication and computation is based on the exchange of information via photons as flying qubits. In all foreseen implementations, from quantum relays and networks to remote quantum computing, the photons must be able to propagate over long distances, in silica fibers, with limited absorption and wave packet dispersion. When propagating into silica fibers, photons in the so-called telecom C-band (i.e. wavelength around 1550 nm) will experience the absolute minimum of absorption, together with a limited photon wave packet dispersion. This implies that losses of information will be minimized and additionally, the capability of the photons to quantum interfere (the so-called Hong–Ou–Mandel effect) will be negligibly affected. This motivated the search for efficient non-classical light sources in this wavelength range. In the present review, we discuss the approaches followed to red-shift the emission wavelength from the near-infrared (NIR) to telecom wavelengths. In particular, the use of metamorphic buffers (MMBs) enabled the use of highly developed InAs/GaAs systems, engineering the dots to emit single and entangled photons in the telecom C-band. The main advantage of this approach is set by the choice of the material system: being the same as state-of-the-art structures emitting in the NIR range, it opens the possibility of achieving comparable performances even at telecommunication wavelengths. Here we will discuss the current state-of-the-art in the generation of non-classical photons, comparing the properties and performances of MMB-based results with other competing quantum dot (QD) platforms. We report in particular that very low fine-structure splitting can be observed with conservative values, on average well below 10 μ eV. This allowed for the observation of post-selected entanglement fidelity higher than 0.6. Additionally, on-demand single-photon emission with g ( 0 ) 2 = 0.184 ± 0.002 was observed in addition to a very low emitter density of ≈ 10 7 cm − 2 and a decay time of τ ≈ 1.2 ns comparable to standard InAs QDs emitting in the NIR range. A final highlight on approaches to further improve the current device performances will also be reported.
High Resolution Image Download MS PowerPoint Slide Entangled photon pairs at telecom wavelengths are essential for quantum communication, distributed computing, and quantum-enhanced sensing. The telecom O-band offers low chromatic dispersion and fiber loss, which is ideal for long-distance networks. Site-controlled nanowire quantum dots have emerged as a promising platform for generating single and entangled photons, offering high extraction efficiency and scalability. However, their operation has largely been restricted to the visible and first near-infrared (NIR-I) windows. Here, we demonstrate a bright source of entangled photon pairs in the telecom O-band based on site-controlled nanowire quantum dots. We measure a fine-structure splitting of 4.6 μeV, confirming suitability for high-fidelity polarization entanglement. Quantum-state tomography of the biexciton–exciton cascade reveals a maximum fidelity of 85.8 ± 1.1% to the Φ + Bell state and a maximum concurrence of 75.1 ± 2.1%. This work establishes nanowire quantum dots as viable entangled photon sources at telecom, advancing scalable quantum technologies for fiber-based networks.