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Field Theories of Interacting and Disordered Dirac Fermions in Graphene

Christian Fräßdorf

Published Jan 1, 2019• 0 citations
Publisher

Abstract

After its first isolation by Geim and Novoselov in 2004, graphene has grown quickly into an independent subfield of contemporary condensed matter physics, counting thousands of publications. This material has attracted so much attention not only because it is truly two-dimensional -- a feature long thought to be impossible to be realized in nature -- but also because it is the prime representative of a new class of condensed matter systems, the Dirac materials, whose electronic spectrum disperses linearly around isolated points in the Brillouin zone. An outstanding consequence of this linear energy-momentum dispersion is the collapse of the Fermi surface to isolated points at charge neutrality, accompanied by a vanishing single-particle density of states. While this feature of the noninteracting model is what separates graphene from most other, more conventional condensed matter systems, giving rise to many of its astounding physical properties, it leads to severe computational complications when extending the model to contain two-body interactions and/or disorder. In this thesis we consider both extensions separately. After rigorously deriving the low-energy quantum field theory from a tight-binding model and establishing the one-particle irreducible (1PI) vertex functions as the fundamental building blocks of correlation functions, we construct a nonperturbative formalism for the calculation of these vertex functions using the well-established functional renormalization group (fRG). By combining the fRG with the Keldysh formalism, accounting for possible external electromagnetic fields and nontrivial initial correlations, this framework is capable of handling thermal equilibrium and true nonequilibrium alike. To circumvent some of the technical problems of the standard fRG formalism when treating fermionic systems at finite density, we also explore a variant of the fRG, where the chemical potential is interpreted as a flow parameter. We obtain hierarchical sets of flow equations, which describe the change of the 1PI vertex functions upon varying an artificial cutoff scale or the chemical potential, respectively. These nonperturbative formalisms have been used to calculate the renormalization of the Fermi velocity and the static dielectric function at finite temperature and density in the strong coupling regime as an explicit demonstration of their capabilities. Since the Keldysh fRG is an exact formulation of quantum field theory, in particular when external magnetic fields are present, it should be possible to describe the fractional quantum Hall effect in this framework. However, the typical truncation schemes that are currently available to approximately solve the fRG flow equation fail to account for the nontrivial correlation effects necessary to access the fractional quantum Hall regime. To circumvent this problem we consider a modified field theory, where these correlations are implemented ``by hand'' via a Chern-Simons gauge field, coupling to the fermions in addition to the Coulomb interaction term. This modified field theory is analyzed in a stationary phase approximation including Gaussian fluctuations. The electromagnetic response tensor is calculated in the random phase approximation, yielding the Hall conductivities. In the second part of this thesis we consider disordered Dirac fermions in the absence of two-particle interactions. After sketching how the most general disorder potential for Dirac fermions arises from a tight-binding model, we first consider an explicit physical scenario, a disordered graphene pn junction in the presence of a quantizing magnetic field perpendicular to the graphene sheet. We derive an effective one-dimensional theory for the chiral states that propagate along the junction interface and calculate the full conductance distribution in the crossover between the clean and the strong-disorder limit, via an exact solution of a Fokker-Planck equation. Lastly, we develop a nonperturbative approach to calculate the disorder induced self-energy that is based on exact Schwinger-Dyson equations and Ward identities, not only for graphene, but also for other paradigmatic semimetals with a nodal point dispersion.

DOI
10.17169/refubium-2153

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After its first isolation by Geim and Novoselov in 2004, graphene has grown quickly into an independent subfield of contemporary condensed matter physics, counting thousands of publications. This material has attracted so much attention not only because it is truly two-dimensional -- a feature long thought to be impossible to be realized in nature -- but also because it is the prime representative of a new class of condensed matter systems, the Dirac materials, whose electronic spectrum disperses linearly around isolated points in the Brillouin zone. An outstanding consequence of this linear energy-momentum dispersion is the collapse of the Fermi surface to isolated points at charge neutrality, accompanied by a vanishing single-particle density of states. While this feature of the noninteracting model is what separates graphene from most other, more conventional condensed matter systems, giving rise to many of its astounding physical properties, it leads to severe computational complications when extending the model to contain two-body interactions and/or disorder. In this thesis we consider both extensions separately. After rigorously deriving the low-energy quantum field theory from a tight-binding model and establishing the one-particle irreducible (1PI) vertex functions as the fundamental building blocks of correlation functions, we construct a nonperturbative formalism for the calculation of these vertex functions using the well-established functional renormalization group (fRG). By combining the fRG with the Keldysh formalism, accounting for possible external electromagnetic fields and nontrivial initial correlations, this framework is capable of handling thermal equilibrium and true nonequilibrium alike. To circumvent some of the technical problems of the standard fRG formalism when treating fermionic systems at finite density, we also explore a variant of the fRG, where the chemical potential is interpreted as a flow parameter. We obtain hierarchical sets of flow equations, which describe the change of the 1PI vertex functions upon varying an artificial cutoff scale or the chemical potential, respectively. These nonperturbative formalisms have been used to calculate the renormalization of the Fermi velocity and the static dielectric function at finite temperature and density in the strong coupling regime as an explicit demonstration of their capabilities. Since the Keldysh fRG is an exact formulation of quantum field theory, in particular when external magnetic fields are present, it should be possible to describe the fractional quantum Hall effect in this framework. However, the typical truncation schemes that are currently available to approximately solve the fRG flow equation fail to account for the nontrivial correlation effects necessary to access the fractional quantum Hall regime. To circumvent this problem we consider a modified field theory, where these correlations are implemented ``by hand'' via a Chern-Simons gauge field, coupling to the fermions in addition to the Coulomb interaction term. This modified field theory is analyzed in a stationary phase approximation including Gaussian fluctuations. The electromagnetic response tensor is calculated in the random phase approximation, yielding the Hall conductivities. In the second part of this thesis we consider disordered Dirac fermions in the absence of two-particle interactions. After sketching how the most general disorder potential for Dirac fermions arises from a tight-binding model, we first consider an explicit physical scenario, a disordered graphene pn junction in the presence of a quantizing magnetic field perpendicular to the graphene sheet. We derive an effective one-dimensional theory for the chiral states that propagate along the junction interface and calculate the full conductance distribution in the crossover between the clean and the strong-disorder limit, via an exact solution of a Fokker-Planck equation. Lastly, we develop a nonperturbative approach to calculate the disorder induced self-energy that is based on exact Schwinger-Dyson equations and Ward identities, not only for graphene, but also for other paradigmatic semimetals with a nodal point dispersion.
This thesis aims at developing new schemes for the treatment of correlation effects in condensed matter systems using quantum field theoretical approaches. In particular, our goal is to extend the description of correlation physics at the two-particle level. This is necessary for an unbiased treatment of condensed matter systems that exhibit electronic correlations and competing ordering tendencies. In this respect, the functional renormalization group (fRG) approaches have surely contributed substantially over the last years, as they account for all scattering channels and their mutual feedback effects in an unbiased way. In spite of its flexibility, the application of the fRG is limited by its inherent perturbative nature. To go beyond the conventional weak-coupling implementations, we discuss the general idea to extend fRG based computational schemes by using an exactly solvable interacting reference problem as starting point for the RG flow. The systematic expansion around this solution accounts for a non-perturbative inclusion of correlations at both, the one-particle (self-energy) and two-particle (vertex functions) level. The full treatment of the two-particle vertex functions, however, poses a huge limitation to the numerical performance, not only in the fRG, but in several forefront many-body algorithms. In this perspective, we provide a detailed diagrammatic analysis of the frequency and momentum structures of the vertex functions, together with their physical interpretation. This constitutes the basis for sophisticated parametrization schemes. We then explain the technical details necessary for cutting-edge numerical implementations, and further benchmark our ideas using refined implementations of both, the fRG and the parquet approximation (PA).
The progress in micro-fabrication technologies makes it possible to address individual, tailored, mesoscopic structures with sizes on a nanometer to micrometer scale. The transport properties of such quasi zero- or one-dimensional systems are considerably influenced by the electron-electron interaction. In theoretical studies this often becomes apparent in the emergence of divergences in a perturbative treatment of the interaction. A successful approach may then be given by renormalization group (RG) methods which are based on the idea of treating energy scales successively from high to low. In the functional RG (fRG) an exact infinite hierarchy of flow equations for multi-particle Green or vertex functions is derived, that allows for systematic approximations on different levels. In numerous studies the fRG has been found to be a powerful tool for the investigation of low dimensional Fermi systems. Usually it is formulated within Matsubara formalism which applies to a system in thermal equilibrium. A central topic of this thesis is the implementation of the fRG within Keldysh formalism, providing the possibility to treat equilibrium and non-equilibrium situations on equal footing. The resulting Keldysh fRG is used in this thesis to explore the transport properties of quantum wires with several barriers and of the single impurity Anderson model. The thesis starts with an introduction to Keldysh formalism and to related concepts. Then the structure of the Green and vertex functions of Keldysh formalism is investigated. This includes studying the consequences of causality, characterizing thermal equilibrium, and formulating corresponding relations for the multi-particle functions. After that, the implementation of the fRG within Keldysh formalism is presented in detail. The flow equations for the vertex functions are derived via their diagrammatic expansion. Two especially useful flow parameters are determined: one of them cuts off the imaginary frequencies that appear as poles of the Fermi functions of the reservoirs. The second flow parameter is an artificially enhanced reservoir hybridization; on one hand it has the advantage to preserve the fluctuation dissipation theorem in equilibrium even in frequency dependent approximations; on the other hand, its use can be more cumbersome. One of the models studied in this thesis is a tight-binding chain with nearest-neighbour interaction. At weak and intermediate interactions it belongs to the class of Luttinger liquids (LLs) whose low energy properties are characterized by power laws. The transport properties of LLs have been studied experimentally for example on carbon nanotubes. However, the presence of transport barriers at the contacts make the interpretation of the experimental data difficult. A theoretical treatment with the fRG permits a rather large flexibility to model the barrier configuration. In this thesis the fRG is first used in its equilibrium Matsubara implementation in order to analyse the temperature dependence of the linear conductance in the presence of two, three or four barriers. It is shown that temperature induces an averaging over quantum phases of propagation, leading to combinations of the power law exponents of the individual barriers. An experimental set-up that allows to verify this behaviour is proposed. In a second step the Keldysh version of the fRG is applied to the problem of transport through a quantum wire at finite bias voltage. For a wire with two high contact barriers it is found that the non-equilibrium particle distribution in the wire is responsible for the appearance of a two-fold power law in the density of states. An additional weakly attached probe lead can be used to make the two different power laws visible in the conductance. The second model which is analysed is the one of the single Anderson impurity, often considered as a paradigm for the investigation of strong local electron correlations. The latter become noticeable in the appearance of the Kondo scale, an energy exponentially small in the interaction strength, that characterizes the low energy physics of the model in the regime of spin fluctuations. On the basis of this model an advanced frequency dependent approximation for the Keldysh fRG is developed in this thesis. Such an approximation can account for subleading effects of the interaction, namely the fact that two-particle interactions can generate decay rates for single-particle states. The derivation of a consistent approximation scheme is presented, that turns out to yield a good description of the model at moderate interaction strength.
Studying the strong correlation effects in interacting Dirac fermion systems is one of the most challenging problems in modern condensed matter physics. The long-range Coulomb interaction and the fermion-phonon interaction can lead to a variety of intriguing properties. In the strong-coupling regime, weak-coupling perturbation theory breaks down. The validity of 1/N1/N1/N expansion with NNN being the fermion flavor is also in doubt since NNN equals to 2 or 4 in realistic systems. Here, we investigate the interaction between (1+2)(1+2)(1+2)- and (1+3)(1+3)(1+3)-dimensional massless Dirac fermions and a generic scalar boson, and develop an efficient nonperturbative approach to access the strong-coupling regime. We first derive a number of self-consistently coupled Ward-Takahashi identities based on a careful symmetry analysis and then use these identities to show that the full fermion-boson vertex function is solely determined by the full fermion propagator. Making use of this result, we rigorously prove that the full fermion propagator satisfies an exact and self-closed Dyson-Schwinger integral equation, which can be solved by employing numerical methods. A major advantage of our nonperturbative approach is that there is no need to employ any small expansion parameter. Our approach provides a unified theoretical framework for studying strong Coulomb and fermion-phonon interactions. It may also be used to approximately handle the Yukawa coupling between fermions and order-parameter fluctuations around continuous quantum critical points. Our approach is applied to treat the Coulomb interaction in undoped graphene. We find that the renormalized fermion velocity exhibits a logarithmic momentum dependence but is nearly energy independent, and that no excitonic gap is generated by the Coulomb interaction. These theoretical results are consistent with experiments in graphene.
We present a nonperturbative study of the quantum many-body effects caused by the long-range Coulomb interaction in a two-dimensional semi-Dirac semimetal. This kind of semimetal may be realized in deformed graphene and a class of other realistic materials. In the noninteracting limit, the dispersion of semi-Dirac fermion is linear in one direction and quadratic in the other direction. When the impact of Coulomb interaction is taken into account, such a dispersion can be significantly modified. To reveal the correlation effects, we first obtain the exact self-consistent Dyson-Schwinger equation of the full fermion propagator and then extract the momentum dependence of the renormalized fermion dispersion from the numerical solutions. Our results show that the fermion dispersion becomes linear in two directions. These results are compared to previous theoretical works on semi-Dirac semimetals.
We investigate nonequilibrium properties of the single-impurity Anderson model by means of the functional renormalization group (fRG) within Keldysh formalism. We present how the level broadening $\ensuremath{\Gamma}/2$ can be used as flow parameter for the fRG. This choice preserves important aspects of the Fermi-liquid behavior that the model exhibits in case of particle-hole symmetry. An approximation scheme for the Keldysh fRG is developed which accounts for the frequency dependence of the two-particle vertex in a way similar but not equivalent to a recently published approximation to the equilibrium Matsubara fRG. Our method turns out to be a flexible tool for the study of weak to intermediate on-site interactions $U\ensuremath{\lesssim}3\ensuremath{\Gamma}$. In equilibrium we find excellent agreement with numerical RG results for the linear conductance at finite gate voltage, magnetic field, and temperature. In nonequilibrium, our results for the current agree well with time-dependent density-matrix RG. For the nonlinear conductance as function of the bias voltage, we propose reliable results at finite magnetic field and finite temperature. Furthermore, we demonstrate the exponentially small scale of the Kondo temperature to appear in the second-order derivative of the self-energy. We show that the approximation is, however, not able to reproduce the scaling of the effective mass at large interactions.
The topic of this thesis is the functional renormalization group. We discuss some approximations schemes. Thereafter we apply these approximations to study different fields of condensed matter physics. Generally we have to evaluate an infinite set of vertex functions describing the scattering of particles. These vertex functions get renormalized away from their bare values governed by an infinite hierarchy of flow equations. We cannot expect to actually solve these equations but have to apply a couple of approximations. The aim is to somehow separate relevant contributions from irrelevant ones. One possible scheme opens up if we rescale fields and vertices. Here "relevance" is used in a quantitative way to describe the scaling behaviour of vertices close to a fixed point of the RG. One disadvantage of describing the system in terms of infinitely many vertices is that the majority of these vertices we have to evaluate are not of interest to us. In most cases we are just looking for the self-energy or the two-particle effective interaction. However there might be contributions to the flow of these vertices that are generated by irrelevant vertices. We generally assume that we can express irrelevant vertices in terms of the relevant and marginal ones. Then in turn it should be possible to write the contributions of these irrelevant vertices to the flow of relevant and marginal ones in terms of relevant and marginal vertices as well. We show how this can be achieved by what we term the adiabatic approximation. We now consider weakly interacting bosons at the critical point of Bose-Einstein condensation. As the transition takes place at a finite temperature this temperature defines an effective ultraviolet cut-off. For the investigation of physical properties that depend on momenta smaller than this cut-off it is therefore sufficient to describe the system by a classical field theory. Our central topic here is the self-energy of the bosons and we are able to evaluate it with the full momentum dependence. For small momenta it approaches a scaling form and as the momentum is gradually increased we observe a crossover to the perturbative regime. As a test for the reliability of our expression for the selfenergy we investigate the interaction induced shift of the critical. Our results compare quite satisfactory to the best available estimates for this shift. For the anomalous dimension our approach predicts the correct order of magnitude however with a considerable error. As an improvement we include more vertices into our calculations. Here we observe that our fixed point estimates indeed approach the best known results but this convergence is quite weak. We turn toward systems of interacting fermions. The formulation of the functional renormalization group implicitly requires knowledge of the true Fermi surface of the full interacting system. In general however we can just calculate it a-posteriori from the self-energy. The requirement to flow into a fixed point can be translated into a fine-tuning of the frequency/momentum independent part r_0 of the rescaled 2-point function. We show how this bare value is related to the momentum dependent effective interaction along the complete trajectory of the RG. On the other hand r_0 expresses the difference between the bare and the true Fermi surface. Putting both equations together results into an exact selfconsistency equation for the Fermi surface. We apply our self-consistency equation above to tackle the problem of finding the true Fermi surface of interacting fermions in low dimensions. The most simple non-trivial model with an inhomogeneous Fermi surface is a system of two coupled metallic chains. The process of interband backward scattering leads to a smoothing of the Fermi surface. Of special interest is if the Fermi momenta of the two bands collapse into just one value. We propose the term confinement transition for this behaviour. We bosonize the interband backward scattering by means of a Hubbard-Stratonovich transformation and treat our system as a single channel problem. This bosonization together with the adiabatic approximation allows us to investigate the system even at strong coupling. Within a simple one-loop treatment our method predicts a confinement transition at strong coupling. However taken vertex renormalizations into account we observe that this confinement is destroyed by fluctuations beyond one-loop. Actually we observe how the confined phase can be stabilized by the inclusion of interband umklapp scattering. Thereafter we consider the physically more relevant case of a two-dimensional system of infinitely many coupled metallic chains. Here the Fermi surface consists of two disconnected weakly curved sheets. We are able to repeat the calculations we have performed for our toy model. Within a self-consistent 2-loop calculation indeed signs for a confinement transition at finite coupling strength emerge.