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Orbital order and chiral currents of interacting bosons with $\pi$-flux

Marco Fedele Di Liberto, Nathan Goldman

Published Nov 26, 2021• 0 citations
OpenAlex

Abstract

Higher Bloch bands provide a remarkable setting for realizing many-body states that spontaneously break time-reversal symmetry, offering a promising path towards the realization of interacting topological phases. Here, we propose a different approach by which chiral orbital order effectively emerges in the low-energy physics of interacting bosons moving on a square plaquette pierced by a $\pi$-flux. We analyze the low-energy excitations of the condensate in terms of two orbital degrees of freedom and identify a gapped collective mode corresponding to the out-of-phase oscillations of the relative density and phase of the two orbitals. We further highlight the chiral nature of the ground state by revealing the cyclotron-like dynamics of the density upon quenching an impurity potential on a single site. Our single-plaquette results can be used as building blocks for extended dimerized lattices, as we exemplify using the BBH model of higher-order topological insulators. Our results provide a distinct direction to realize interacting orbital-like models that spontaneously break time-reversal symmetry, without resorting to higher bands nor to external drives.

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Ultracold atoms loaded into higher Bloch bands provide an elegant setting for realizing many-body quantum states that spontaneously break time-reversal symmetry through the formation of chiral orbital order. The applicability of this strategy remains nonetheless limited due to the finite lifetime of atoms in high-energy bands. Here we introduce an alternative framework, suitable for bosonic gases, which builds on assembling square plaquettes pierced by a $\ensuremath{\pi}$ flux (half a magnetic-flux quantum). This setting is shown to be formally equivalent to an interacting bosonic gas loaded into $p$ orbitals, and we explore the consequences of the resulting chiral orbital order, both for weak and strong on-site interactions. We demonstrate the emergence of a chiral superfluid vortex lattice, exhibiting a long-lived gapped collective mode that is characterized by local chiral currents. This chiral superfluid phase is shown to undergo a phase transition to a chiral Mott insulator for sufficiently strong interactions. Our work establishes coupled $\ensuremath{\pi}$-flux plaquettes as a practical route for the emergence of orbital order and chiral phases of matter.

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Orbital order and chiral currents of interacting bosons with π\piπ-flux
Higher Bloch bands provide a remarkable setting for realizing many-body states that spontaneously break time-reversal symmetry, offering a promising path towards the realization of interacting topological phases. Here, we propose a different approach by which chiral orbital order effectively emerges in the low-energy physics of interacting bosons moving on a square plaquette pierced by a π\piπ-flux. We analyze the low-energy excitations of the condensate in terms of two orbital degrees of freedom and identify a gapped collective mode corresponding to the out-of-phase oscillations of the relative density and phase of the two orbitals. We further highlight the chiral nature of the ground state by revealing the cyclotron-like dynamics of the density upon quenching an impurity potential on a single site. Our single-plaquette results can be used as building blocks for extended dimerized lattices, as we exemplify using the BBH model of higher-order topological insulators. Our results provide a distinct direction to realize interacting orbital-like models that spontaneously break time-reversal symmetry, without resorting to higher bands nor to external drives.
Ultracold atoms loaded into higher Bloch bands provide an elegant setting for realizing many-body quantum states that spontaneously break time-reversal symmetry through the formation of chiral orbital order. The applicability of this strategy remains nonetheless limited due to the finite lifetime of atoms in high-energy bands. Here we introduce an alternative framework, suitable for bosonic gases, which builds on assembling square plaquettes pierced by a $\ensuremath{\pi}$ flux (half a magnetic-flux quantum). This setting is shown to be formally equivalent to an interacting bosonic gas loaded into ppp orbitals, and we explore the consequences of the resulting chiral orbital order, both for weak and strong on-site interactions. We demonstrate the emergence of a chiral superfluid vortex lattice, exhibiting a long-lived gapped collective mode that is characterized by local chiral currents. This chiral superfluid phase is shown to undergo a phase transition to a chiral Mott insulator for sufficiently strong interactions. Our work establishes coupled $\ensuremath{\pi}$-flux plaquettes as a practical route for the emergence of orbital order and chiral phases of matter.
Neutral-atom quantum simulators provide a powerful platform for realizing strongly correlated phases, enabling access to dynamical signatures of quasiparticles and symmetry breaking processes. Motivated by recent observations of quantum phases in flux-frustrated ladders with non-vanishing ground state currents, we investigate interacting bosons on the dimerized BBH lattice in two dimensions-originally introduced in the context of higher-order topology. After mapping out the phase diagram, which includes vortex superfluid (V-SF), vortex Mott insulator (V-MI), and featureless Mott insulator (MI) phases, we focus on the integer filling case. There, the MI/V-SF transition simultaneously breaks the Z2T\mathbb Z_2^{T}Z2T​ and U(1) symmetries, where Z2T\mathbb Z_2^{T}Z2T​ corresponds to time-reversal symmetry (TRS). Using a slave-boson description, we resolve the excitation spectrum across the transition and uncover a chiral Higgs mode whose mass softens at criticality, providing a dynamical hallmark of emergent chirality that manifests via the oscillation of the loop currents in quench dynamics. Our results establish an experimentally realistic setting for probing unconventional TRS-broken phases and quasiparticles with intrinsic chirality in strongly interacting quantum matter.
Interacting bosons on a single plaquette threaded by a $\ensuremath{\pi}$ flux can spontaneously break time-reversal symmetry, resulting in a chiral loop current. Connecting such bosonic $\ensuremath{\pi}$-flux plaquettes in a dispersive configuration was recently shown to lead to long-range chiral order. Here, instead, we design a chain of $\ensuremath{\pi}$-flux plaquettes that exhibits an all-flat-bands single-particle energy spectrum and an extensive set of local symmetries. Using Elitzur's theorem, we show that these local symmetries prevent the emergence of long-range chiral order. Moreover, projecting the dynamics to a Creutz ladder model with an effective intrarung interaction allows one to derive simple spin Hamiltonians capturing the ground-state degeneracy and the low-energy excitations, and to confirm the absence of chiral order. Nevertheless, we show how to obtain gauge-invariant information from a mean-field approach, which explicitly breaks gauge-invariance. Finally, we observe an impurity self-pinning phenomenon, when an extra boson is added on top of a ground state at integer filling, resulting in a nondispersive density peak. Exact diagonalization benchmarks are also provided, and experimental perspectives are discussed.
Abstract Topological superfluidity is an important concept in electronic materials as well as ultracold atomic gases1. However, although progress has been made by hybridizing superconductors with topological substrates, the search for a material—natural or artificial—that intrinsically exhibits topological superfluidity has been ongoing since the discovery of the superfluid 3He-A phase2. Here we report evidence for a globally chiral atomic superfluid, induced by interaction-driven time-reversal symmetry breaking in the second Bloch band of an optical lattice with hexagonal boron nitride geometry. This realizes a long-lived Bose–Einstein condensate of 87Rb atoms beyond present limits to orbitally featureless scenarios in the lowest Bloch band. Time-of-flight and band mapping measurements reveal that the local phases and orbital rotations of atoms are spontaneously ordered into a vortex array, showing evidence of the emergence of global angular momentum across the entire lattice. A phenomenological effective model is used to capture the dynamics of Bogoliubov quasi-particle excitations above the ground state, which are shown to exhibit a topological band structure. The observed bosonic phase is expected to exhibit phenomena that are conceptually distinct from, but related to, the quantum anomalous Hall effect3–7 in electronic condensed matter.
Topological edge states and Dirac fermions are fascinating phenomena known for fermionic systems. Whether similar phenomena can occur for interacting bosons is an open question in fundamental science. The recent observation of 87^{87}87Rb chiral px±ipyp_x\pm ip_ypx​±ipy​ condensates in a checkerboard optical lattice further raises the question whether a bosonic superfluid can be topological. Here we show that Dirac bosons experiencing a π\piπ Berry flux emerge in the elementary excitation spectra of this experimentally realized Bose system. Tuning a population bias between the observed px+ipyp_x+ip_ypx​+ipy​ and px−ipyp_x-ip_ypx​−ipy​ condensate components opens an energy gap in the bulk, which results in Chern invariant and topologically protected Bogoliubov edge modes. Different from previous topological scenarios that employ the concept of engineered spin-orbit coupling or the equivalent in single-particle Bloch bands, spontaneous chiral orbital order driven by many-body interaction is a crucial ingredient in our finding.
The breaking of time-reversal symmetry via the spontaneous formation of chiral order is ubiquitous in nature. Here, we present an unambiguous demonstration of this phenomenon for atoms Bose-Einstein condensed in the second Bloch band of an optical lattice. As a key tool, we use a matter-wave interference technique, which lets us directly observe the phase properties of the superfluid order parameter and allows us to reconstruct the spatial geometry of certain low-energy excitations, associated with the formation of domains of different chirality. Our work marks a new era of optical lattices where orbital degrees of freedom play an essential role for the formation of exotic quantum matter, similarly as in electronic systems.