Photon correlation: Using photon statistics to probe dynamic systems

Dale W. Schaefer

F. Shikerman, Eli Barkai

A two level model of a single molecule undergoing spectral diffusion dynamics and interacting with a sequence of two short laser pulses is investigated. Analytical solution for the probability of n=0,1,2 photon emission events for the telegraph and Gaussian processes is obtained. We examine under what circumstances the photon statistics emerging from such pump-probe setup provides new information on the stochastic process parameters and what are the measurement limitations of this technique. The impulsive and selective limits, the semiclassical approximation, and the fast modulation limit exhibit general behaviors of this new type of spectroscopy. We show that in the fast modulation limit, where one has to use impulsive pulses in order to obtain meaningful results, the information on the photon statistics is contained in the molecule's dipole correlation function, equivalently to continuous wave experiments. In contrast, the photon statistics obtained within the selective limit depends on the both spectral shifts and rates and exhibits oscillations, which are not found in the corresponding line shape.

Edward R. Pike, Eric Jakeman

Julien Gabelli, Laure-Hélène Reydellet, Gwendal Fève +4 more

We present the first study of the statistics of GHz photons in quantum circuits, using Hanbury Brown and Twiss correlations. The super-Poissonian and Poissonian photon statistics of thermal and coherent sources, respectively, made of a resistor and a radio frequency generator, are measured down to the quantum regime at milli-Kelvin temperatures. As photon correlations are linked to the second and fourth moments of current fluctuations, this experiment, which is based on current cryogenic electronics, may become a standard for probing electron/photon statistics in quantum conductors.

Swati Singh, Yiwen Chu, Adi Pick +3 more

Edward R. Pike