Ultracold neutral plasmas 1 (UNPs) are strongly coupled, non- equilibrium systems created by photoionizing laser cooled atoms in a vacuum. As a result, experimental platforms are developed to elucidate the properties of UNPs such as their spatial expansion and temperature relaxation 2 . Data from these experiments are used to validate theories and computational models that aim to model UNPs. One such computational model derived from a multi-species BGK kinetic theory 3 .
Ultracold neutral plasmas 1 (UNPs) are strongly coupled, non- equilibrium systems created by photoionizing laser cooled atoms in a vacuum. As a result, experimental platforms are developed to elucidate the properties of UNPs such as their spatial expansion and temperature relaxation 2 . Data from these experiments are used to validate theories and computational models that aim to model UNPs. One such computational model derived from a multi-species BGK kinetic theory 3 .
Ultracold neutral plasmas (UNPs) are created in a vacuum by photoionizing laser-cooled atoms. The expansion of UNPs begins as a non-equilibrium system that quickly relaxes to a local equilibrium state [1] . We aim to quantify and compare the transport processes that govern the relaxation to equilibrium in the expanding UNP. Using a 1D-1V kinetic code in spherical coordinates, we model the radial expansion of an UNP. We compare our simulation results against analytic expressions to determine where the expansion of the UNP is adiabatic or isothermal. We carry out simulations for various initial density distributions such as an exponentially decaying density distribution [2] . We ultimately aim to extend this approach to a 1D-3V multi-component kinetic code that incudes collisions [3] .
By photoionizing samples of laser-cooled atoms with laser light tuned just above the ionization limit, plasmas can be created with electron and ion temperatures below 10 K. These ultracold neutral plasmas have extended the temperature bounds of plasma physics by two orders of magnitude. Table-top experiments, using many of the tools from atomic physics, allow for the study of plasma phenomena in this new regime with independent control over the density and temperature of the plasma through the excitation process. Characteristic of these systems is an inhomogeneous density profile, inherited from the density distribution of the laser-cooled neutral atom sample. Most work has dealt with unconfined plasmas in vacuum, which expand outward at velocities of order 100 m/s, governed by electron pressure, and with lifetimes of order 100 μs, limited by stray electric fields. Using detection of charged particles and optical detection techniques, a wide variety of properties and phenomena have been observed, including expansion dynamics, collective excitations in both the electrons and ions, and collisional properties. Through three-body recombination collisions, the plasmas rapidly form Rydberg atoms, and clouds of cold Rydberg atoms have been observed to spontaneously avalanche ionize to form plasmas. Of particular interest is the possibility of the formation of strongly coupled plasmas, where Coulomb forces dominate thermal motion and correlations become important. The strongest impediment to strong coupling is disorder-induced heating, a process in which Coulomb energy from an initially disordered sample is converted into thermal energy. This restricts electrons to a weakly coupled regime and leaves the ions barely within the strongly coupled regime. This review will give an overview of the field of ultracold neutral plasmas, from its inception in 1999 to current work, including efforts to increase strong coupling and effects on plasma properties due to strong coupling.
Ultracold neutral plasmas (UNPs) are highly correlated, charged-particle systems studied in standard atomic-molecular optical physics laboratories. Advances in ultracold physics techniques have led to the development of magneto-optical traps that permit the localization of micro-Kelvin temperature atomic samples (10⁸ - 10¹⁰ cm -³ that can be photoionized with a defined excess laser energy. Magneto-optical trapping of molecules proves difficult, and to date, lags in reaching conditions attainable for atoms. Molecules possess additional degrees of freedom where energy can flow during laser trapping and cooling. Alternatively, elastic collisions with inert gases offer another route to low temperatures. Super-sonic expansions of target molecules seeded in a noble gas can reduced the translational temperature to values as low as 0.1 K. Here I report on the formation of a molecular ultracold plasma in a molecular beam of nitric oxide seeded in an inert gas. Our method does not directly form a plasma, but instead, I create a Rydberg gas that spontaneously evolves to a plasma. I have verified the transition to a collective plasma state by applying pulsed-fields to the field-free flight region, and observe a signal that persists well beyond classical field amplitudes required to ionize individual Rydberg states. Electric field screening is a collective effect occurring over a characteristic distance, quantified by the Debye length, λ_D. Molecular ultracold plasmas described here exhibit Debye lengths smaller than the overall size, λ_D<<σ. Plasmas of this nature offer an exotic environment for which to study fundamental phenomena. While plasmas are generally thought of as hot, UNPs exist at low enough temperatures that electrostatic interaction energy between particles is greater than their kinetic energy. At this point, charged particles begin to find themselves in local potential energy minima. Over the entire sample this translates to long-range order, or correlation. It is of great interest for researchers studying UNPs to maximize particle correlation, which requires UNPs to remain very cold, and dense through their lifetime.
This thesis describes the measurements of collective effects in strongly coupled ultra-cold neutral plasmas (UNPs). It shows the implementation of experimental techniques that perturb either the density or velocity distribution of the plasma and it describes the subsequent excitation, observation and analysis of the aforementioned collective phenomena. UNPs are interesting in that they display physics of strongly coupled systems. For most plasma systems, collective effects are well described with classical hydrodynamic or kinetic descriptions. However, for strongly coupled systems, the Coulomb interaction energy between nearest neighbors exceeds the kinetic energy, and these descriptions must be modified as the plasma crosses over from a gas-like to liquid-like behavior. Strongly coupling can be found in exotic plasma systems found astrophysics, dusty plasmas, non-neutral trapped ion plasmas, intense-laser/matter interactions and inertial confinement fusion experiments. Compared to other strongly coupled plasmas, UNPs are ideal for studying collective effects in this regime since they have lower timescales, precisely controllable initial conditions and non-invasive diagnostics. Previous studies of UNPs concentrated on plasma expansion dynamics and some collective effects such as disorder induced heating, but little work had been done in relaxation or collision rates and collective modes in UNPs. This thesis presents a method for measuring collision rates by perturbing the velocity distribution of the plasma, observing plasma relaxation and measuring the relaxation rate. It also presents a new technique for observing collective modes in the plasma by perturbing the initial density of the plasma and how this results in the excitation of ion acoustic waves and a measurement of its dispersion relation. Finally, this thesis presents how this last technique can be used to create a gap in the center of the plasma and how this leads to hole propagation and plasma streaming and presents a characterization of both phenomena. The result of these experiments will be valuable for predicting the behavior of collective effects in other strongly coupled plasmas and for comparison with theories that describe them.
Ultracold neutral plasmas are formed by photoionizing laser-cooled atoms near the ionization threshold. Through the application of atomic physics techniques and diagnostics, these experiments stretch the boundaries of traditional neutral plasma physics. The electron temperature in these plasmas ranges from 1-1000 K and the ion temperature is around 1 K. The density can approach 1011 cm−3. Fundamental interest stems from the possibility of creating strongly-coupled plasmas, but recombination, collective modes, and thermalization in these systems have also been studied. Optical absorption images of a strontium plasma, using the Sr+2S1/2−>2P1/2 transition at 422 nm, depict the density profile of the plasma, and probe kinetics on a 50 ns time-scale. The Doppler-broadened ion absorption spectrum measures the ion velocity distribution, which gives an accurate measure of the ion dynamics in the first microsecond after photoionization.
Using high-resolution laser-induced fluorescence spectroscopy, ion dynamics in\nan expanding ultracold neutral plasma (UNP) have been studied in unprecedented\ndetail. The evolution of the ion temperature is of great interest because the ions in\nan ultracold neutral plasma are strongly coupled, meaning their Coulomb interaction\nenergy exceeds the thermal energy. This leads to novel plasma properties that are\nhard to describe theoretically. Understanding all the factors that contribute to ion\ntemperature evolution is critical for designing schemes to cool the ions and achieve\neven stronger Coulomb coupling.\nThis work has also observed several phenomena that have not previously been\nstudied in ultracold plasmas. Ion adiabatic cooling has been observed in a UNP for\nthe first time, resulting in ion temperatures as low as 100mK and up to a tripling of\nthe Coulomb coupling parameter. The importance of electron-ion energy transfer is\ndemonstrated with the first observations of electron-ion collisional heating. Inclusion\nof this effect into existing numerical models provides better agreement with experimental\nresults. Results of molecular dynamics simulations of equilibrating plasmas\nhave been compared to early time experimental data, which provides a new method\nof density determination that is much less sensitive to experimental systematics and\nis accurate to within 10%. This improved certainty in the density allows accurate\ncomparison between data and a theoretical model of the plasma dynamics. The\nagreement is excellent, but on a hydrodynamic time scale a small amount of extra\nheat (on order of 100mK), not ascribable to electron-ion collisions or other sources in\nthe model, is detected in the ion component. Potential sources are discussed within\nas well as proposals for further studies and improvements.