Path integrals for open quantum systems: General theory and dynamical simulation

Amartya Bose

Path integrals offer a robust approach for simulating open quantum dynamics with advancements transcending initial system size limitations. However, accurately modeling systems governed by mechanisms that do not conserve the number of quantum particles, such as lossy cavity modes, remains a challenge. We present a method to incorporate such empirical source and drain mechanisms within a path integral framework using quantum master equations. This technique facilitates rigorous inclusion of bath degrees of freedom while accommodating empirical time scales via Lindbladian dynamics. Computational costs are primarily driven by the path integral method with minimal overhead from Lindbladian terms. We use it to study exciton transport in a four-site Fenna-Matthews-Olson model, examining the potential loss of the exciton to the reaction center. This path integral Lindblad method promises an enhanced ability to simulate dynamics and will be fundamental to simulation of spectra in diverse quantum processes in open systems.

Michael B. Mensky

Antonio Camurati, Felipe Sobrero, Bruno Suassuna +1 more

We establish a direct connection between the Feynman-Vernon path integral formalism for open quantum systems and the Wiener path integral used in classical stochastic dynamics. By considering a generalized influence functional in the strong decoherence limit, we demonstrate that integrating over the quantum coherence length leads to a derivation of stochastic Langevin dynamics. Specifically, we show that the quantum Feynman measure transforms into the stochastic Wiener measure. Applying this framework to the Wigner function representation, we show that the system follows a stochastic path interpretable via classical probability theory. Finally, we address the inverse problem: constructing an equivalent quantum influence functional from a given classical Langevin equation.

Ruofan Chen

M. S. Marinov

Antonio Camurati, Felipe Sobrero, Bruno B. Suassuna +1 more

Abstract We establish a formal connection between the Feynman–Vernon path integral formalism for open quantum systems and the Wiener path integral used in classical stochastic dynamics, further exploring its applications. By considering a generalized influence functional in the strong decoherence limit, we demonstrate that integrating over the quantum coherence length leads to stochastic Langevin dynamics. Specifically, under our model, we show that the quantum Feynman differential transforms into an underdamped multiplicative non-Markovian Langevin dynamics. Applying this framework to the Wigner function representation, we show that the system follows a stochastic path interpretable via classical probability theory, allowing for the investigation of decoherence through classical dynamics. Finally, we address the inverse problem: constructing an equivalent quantum influence functional from a given classical Langevin equation.