Photonic N00N-states, i.e. states of light where N photons are in an extremal superposition between two orthogonal states $\frac{1}{{\sqrt 2 }}\left({\left| {N,0} \right\rangle + \left| {0,N} \right\rangle }\right)$ , have an increased phase-sensitivity in comparison to their classical counterparts. This phase sensitivity has been harnessed in multiple proof-of-principle experiments with one implementation even showing this advantage unconditionally [1] . Using the increased phase sensitivity, that quantum states of light offer, in conjunction with the increased angular sensitivity of states with large orbital angular momentum (OAM) [2] , has been the target of theoretical studies [3] as well experiments utilizing squeezed states [4] and entangled photon pairs [5] . Until recently however [6] , a reliable way of generating two-photon OAM N00N-states, in a single beam-line and for arbitrary OAM-values, had not been demonstrated.
Photonic N00N-states, i.e. states of light where N photons are in an extremal superposition between two orthogonal states 21(∣N,0⟩+∣0,N⟩) , have an increased phase-sensitivity in comparison to their classical counterparts. This phase sensitivity has been harnessed in multiple proof-of-principle experiments with one implementation even showing this advantage unconditionally [1] . Using the increased phase sensitivity, that quantum states of light offer, in conjunction with the increased angular sensitivity of states with large orbital angular momentum (OAM) [2] , has been the target of theoretical studies [3] as well experiments utilizing squeezed states [4] and entangled photon pairs [5] . Until recently however [6] , a reliable way of generating two-photon OAM N00N-states, in a single beam-line and for arbitrary OAM-values, had not been demonstrated.
The increased phase sensitivity of N00N states has been used in many experiments, often involving photon paths or polarization. Here we experimentally combine the phase sensitivity of N00N states with the orbital angular momentum (OAM) of photons up to 100 ℏ, to resolve rotations of a light field around its optical axis. The results show that both a higher photon number and larger OAM increase the resolution and achievable sensitivity. The presented method opens a viable path to unconditional angular supersensitivity and accessible generation of N00N states between any transverse light fields.
Photonic N00N states, i.e., states of light where N photons are in an extremal superposition between two orthogonal states21(∣N,0⟩+∣0,N⟩), have an increased phase-sensitivity in comparison to their classical counterparts. Using the sensitivity offered by N00N states, in conjunction with the intrinsic properties of transverse-spatial modes, enables new measurement schemes with sensitivities beyond the classically allowed limits and opens up possibilities to investigate the behaviour of different quantum states.
Structured photons often serve as physical realizations of high-dimensional quantum states beneficial to quantum information. One popular way of discretizing the space is through Laguerre-Gaussian modes that can have twisted phase front and, thus, orbital angular momentum (OAM). We demonstrate that using multi-plane light-conversion techniques enables the performance of complex unitary transformations between multiple input-modes and output-modes in the quantum regime. We demonstrate various complex two-photon interferences observed in spatial modes, thereby realizing a linear optical network along a single beam path. Finally, we show that using this ability allows the generation of spatial-mode NOON-states, which offer angular super-sensitivity.
Quantum memory is a key component of quantum networks. A successful development in enabling the distribution of quantum information requires the storage of single-photon light. Usually quantum information is encoded using a 2D space, spanned, for example, by the orthogonal polarization states of a photon. In this case, each photon carries a quantum bit of information. If the photon could be encoded in a high-dimensional space instead, the information carried by each photon could be increased from a bit to |log2d| bits, where d is the dimension of the Hilbert space in which the photon is described. The channel capacity of the network and the transmission efficiency would then be greatly enlarged [1]. Moreover, storing high-dimensional states in quantum memory can reduce its sensitivity to memory coherence time [2], leading to significant improvements in storage capacity [3]. It is thus no surprise that many research groups are actively working on different physical systems for storing light encoded using a high-dimensional space. The degrees of freedom for position, linear momentum, time-bin or orbital angular momentum (OAM) of a photon can all be considered as a high-dimensional space for encoding. The photon's OAM has the most potential for encoding [4]. Electromagnetic waves have both spin and OAM. Spin angular momentum produces polarization. Photons with OAM can be regarded as helices with left and right handedness twisted to varying degrees (Fig. 1). Information is encoded using this handedness and the amount of twist. Because of the inherent infinite degrees of freedom for OAM, a photon can in principle carry an arbitrarily large amount of information, and hence the eagerness to store light encoded in OAM space. Although some work on this has been reported for different physical systems, what is lacking is a way of storing and releasing at some later time a true single photon, including its shape and structure [5–7]. Constructing this basic element of quantum memory has been a major challenge. The wavefront of an OAM light is a helical structure (left and center), with an optical vortex at its center in the intensity distribution of light (right). The vortex of light can carry non-zero OAM of any order m. OAM states of a different order are orthogonal. A group at the Key Laboratory of Quantum Information, Chinese Academy of Science, at the University of Science and Technology of China finally resolved this problem [8]. They reported on the first experimental realization of a true single-photon-carrying OAM stored via electromagnetically induced transparency (EIT) in a cold atomic ensemble (Fig. 2). With such a suitable candidate, this work indicates a means of constructing high-dimensional quantum memory. After this, similar results were reported by Laurat's group at Laboratoire Kastler Brossel, at Université Pierre et Marie Curie in France [9], where an extremely weak laser at single-photon level carrying OAM was also stored via EIT in a cold atomic ensemble. Ding et al. [8] first prepared two cold 85Rb atomic clouds in two magnetic-optical traps (MOT) using laser cooling and trapping techniques. They generated non-classical correlated photon pairs using spontaneous four-wave mixing in an atomic cloud. One photon of each pair was used as a trigger; the other mapped and stored in a second atomic cloud via EIT. Each photon to be stored carried one OAM unit. After a programed storage time, the photon was retrieved. What they achieved during storage included (1) proof that the non-classical correlation between the trigger photon and the retrieved photon is retained by demonstrating a strong violation of the Cauchy–Schwarz inequality, (2) a demonstration that the single-photon property of the signal photon is maintained by performing the Hanbury–Brown and Twiss experiment on the trigger photon, (3) proof that the spatial structure of the photon is also very well preserved by showing a high similarity between input and output, and (4) evidence, gathered by Sagnac interferometry, that the coherence of a single photon is also preserved. A heralded single photon is generated through spontaneous four-wave mixing in MOT 1 (a); this single photon carrying OAM is then stored through EIT in MOT 2 (b); (c) shows an image of the photon carrying OAM. Experimental measurements in the transverse position of the image carried by the photon before and after storage are presented in (d) and (e), respectively; (f) shows the simplified experimental setup for storage of a superposition of OAM. Interference patterns taken at different angle settings of the half-wave plate are shown in (g). The left column represents the experimental angle settings of the half-wave and the quarter-wave plates, the middle column gives the experimental results, and the right column gives results from theoretical simulations; (h) and (i) present the interference patterns of the input signal photon and the retrieved signal with plate angle, respectively. This is a significant breakthrough towards the realization of a quantum internet and, potentially, quantum computing. This work addresses the ability to generate, store, retrieve on demand an arbitrary single-photon-level photonic state encoded in OAM space. It signifies an important step in the development of practical quantum-enabled technologies, opens up the possibility for realizing high-dimensional quantum memories based on this degree of freedom of light, and will have a large impact in a broad physical community, especially in the quantum information and quantum optics communities. The Technology Review website of MIT comments on their work very positively with an article entitled ‘First Quantum Memory That Records the Shape of a Single Photon Unveiled in China’. Further, Nature Photonics selected this work as a research highlight. Clearly, memory that can preserve the spatial structure of photons will make the internet far more flexible and capable. Of course, there are still many basic problems remaining that need to be solved to build the future quantum internet, one of which is the construction of quantum memory exploiting entanglement. This derives from the fact that a quantum network needs the distribution of quantum-entangled photons over channels between different nodes [10]. A high-dimensional quantum internet needs to store OAM-entangled states and perform entanglement swapping to efficiently extend the achievable communication distances. While Ding et al. [8] reported the storage of light with OAM at the single-photon level, the photon was, however, still encoded in a 2D space. Therefore, whether it is possible to construct a high-dimensional quantum memory remains an open issue that needs to be investigated further.
Twisted light, or light with orbital angular momentum (OAM), plays an emerging role in both classical and quantum science, with important applications in areas as diverse as biophotonics, micromachines, spintronics, or quantum information. It offers fascinating opportunities for exploring new fundamental ideas in physics, as well as for being used as a tool for practical applications. One important point is to determine how to generate single photons, and two-photon states, with an appropriate OAM content. Here we describe the paraxial orbital angular momentum of entangled photon pairs generated by spontaneous parametric down-conversion (SPDC) in different non-collinear geometries. These geometries introduce a variety of new features. In particular, we find the OAM of entangled pairs generated in purely transverse-emitting configurations, where the entangled photons counter-propagate perpendicularly to the direction of propagation of the pump beam. The spatial walk-off of all interacting waves in the parametric process also determines the OAM content of the down-converted photons, and here its influence is also revealed.
Photons are an ideal candidate for encoding both classical and quantum information. Besides spin angular momentum associated with circular polarization, single photon can also carry other fundamentally new degree of freedom of orbital angular momentum related to the spiral phase structure of light. The key significance of orbital angular momentum lies in its potential in realizing a high-dimensional Hilbert space and in encoding a high-dimensional quantum information. Since Allen et al. [Allen L, Beijersbergen M W, Spreeuw R J C, Woerdman J P 1992 Phys. Rev. A 45 8185] recognized the physical reality of photon orbital angular momentum in 1992, rapidly growing interest has been aroused in orbital angular momentum (OAM) from both classical and quantum points of view. Here we present an overall review on the high-order orbital angular momentum of photon, including its preparation and manipulation based on some specific techniques and also its applications. The spatial light modulator is a commercial device that has been widely employed to generate the OAM beams. We make and identify the optical OAM superposition with very high quantum numbers up to l=360. Recently, the metallic spiral phase mirrors were also developed to produce high-order OAM beams up to l=5050. In addition, the Q-plates made of anisotropic and inhomogeneous liquid crystals were invented to generate high-order OAM beams in a polarization-controllable manner, and the OAM superposition of l=± 50 were achieved. Owing to high rotational symmetry, these high OAM beams have been found to have more and more important applications in the fields of high-sensitivity sensing and high-precision measurements. Two fascinating examples are discussed in detail. The first example is that the research group led by Prof. Zeilinger has prepared and observed the quantum entanglement of high orbital angular momenta up to l=±300 by the technique of polarization-OAM entanglement swapping, and they demonstrated that the angular resolution could be significantly improved by a factor of l. Their result was the first step for entangling and twisting even macroscopic, spatially separated objects in two different directions. The second example is that the research group led by Prof. Padgett has demonstrated an elegant experiment of rotational Doppler effects for visible light with l=±20 OAM superposition. They showed that a spinning object with an optically rough surface might induce a Doppler effect in light reflected from the direction parallel to the rotation axis, and the frequency shift was proportional to both the disk's angular speed and the optical OAM. The potential applications in noncontact measurement of angular speed and in significant improvement of angular resolution for remote sensing will be particularly fascinating.