Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Strain tuning of single-molecule-based single photon sources

Anastasios Fasoulakis, Kyle D. Major, Rowan A. Hoggarth, Alex S. Clark

Published Jun 21, 2021• 0 citations

Abstract

Dibenzoterrylene (DBT) molecules embedded in an anthracene host crystal are promising sources of single photons. They have high photostability and can be readily included in photonic structures [1] . Furthermore, when cooled to cryogenic temperatures they are spectrally stable and display fully coherent, lifetime-limited emission in the zero-phonon line (ZPL) [2] , and have a large branching ratio for this decay compared to incoherent decay involving molecular vibrations [3] . Another key characteristic of DBT-based photon sources is the proximity of their emission wavelength compared to rubidium atoms [4] , which can be exploited for quantum technology applications. However, so far fine-tuning of the emission of DBT has mainly been achieved using Stark tuning with a static electric field.

DOI: 10.1109/cleo/europe-eqec52157.2021.9541855

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