Photons are elementary particles of light, and their interactions in vacuum are extremely weak. The seclusion of photons makes them perfect carriers of classical and quantum information, but also poses difficulties for employing them in quantum information technologies. Recent years have seen tremendous experimental progress in the development of synthetic quantum systems where strong and controllable coupling between single photons is achieved. In a variety of solid-state and optical platforms, propagating photons are coupled with local emitters such as atoms, quantum dots, NV centers, or superconducting qubits. Despite the different nature of the platforms, many of these systems can be described using the same theoretical framework called waveguide quantum electrodynamics (WQED). Dissipation is an inevitable ingredient of many synthetic quantum systems and is a source of error in quantum information applications. Despite its important role in experimental systems, the implications of dissipation in scattering theory havenot been fully explored. Chapter 2 discusses our discovery of the dissipation-induced bound states in WQED systems. The appearance of these bound states is in a one-to-one correspondence with zeros in the single-photon transmission. We also formulate a dissipative version of Levinson's theorem by looking at the relation between the number of bound states and the winding number of the transmission phases. In Chapter 3, we study three-body loss in Rydberg polaritons. Despite past theoretical and experimental studies of the regime with dispersive interaction, the dissipative regime is still mostly unexplored. Using a renormalization group technique to solve the quantum three-body problem, we show how the shape and strength of dissipative three-body forces can be universally enhanced for Rydberg polaritons. We demonstrate how these interactions relate to the transmission through a single-mode cavity, which can be used as a probe of the three-body physics in current experiments. The high level of control of the synthetic quantum systems behind WQED offers many inspirations for theoretical studies. In Chapter 4 of this dissertation, we explore a new direction of scattering theory motivated by the controllability of dispersion relations in synthetic quantum systems. We study single-particle scattering in one dimension when the dispersion relation is E(k)=k^m, where m>= 2 is an integer. For a large class of interactions, we discover that the S-matrix evaluated at an energy E->0 converges to a universal limit that is only dependent on m. We also give a generalization of Levinson's theorem for these more general dispersion relations in WQED systems.
Photons are elementary particles of light, and their interactions in vacuum are extremely weak. The seclusion of photons makes them perfect carriers of classical and quantum information, but also poses difficulties for employing them in quantum information technologies. Recent years have seen tremendous experimental progress in the development of synthetic quantum systems where strong and controllable coupling between single photons is achieved. In a variety of solid-state and optical platforms, propagating photons are coupled with local emitters such as atoms, quantum dots, NV centers, or superconducting qubits. Despite the different nature of the platforms, many of these systems can be described using the same theoretical framework called waveguide quantum electrodynamics (WQED). Dissipation is an inevitable ingredient of many synthetic quantum systems and is a source of error in quantum information applications. Despite its important role in experimental systems, the implications of dissipation in scattering theory havenot been fully explored. Chapter 2 discusses our discovery of the dissipation-induced bound states in WQED systems. The appearance of these bound states is in a one-to-one correspondence with zeros in the single-photon transmission. We also formulate a dissipative version of Levinson's theorem by looking at the relation between the number of bound states and the winding number of the transmission phases. In Chapter 3, we study three-body loss in Rydberg polaritons. Despite past theoretical and experimental studies of the regime with dispersive interaction, the dissipative regime is still mostly unexplored. Using a renormalization group technique to solve the quantum three-body problem, we show how the shape and strength of dissipative three-body forces can be universally enhanced for Rydberg polaritons. We demonstrate how these interactions relate to the transmission through a single-mode cavity, which can be used as a probe of the three-body physics in current experiments. The high level of control of the synthetic quantum systems behind WQED offers many inspirations for theoretical studies. In Chapter 4 of this dissertation, we explore a new direction of scattering theory motivated by the controllability of dispersion relations in synthetic quantum systems. We study single-particle scattering in one dimension when the dispersion relation is E(k)=k^m, where m>= 2 is an integer. For a large class of interactions, we discover that the S-matrix evaluated at an energy E->0 converges to a universal limit that is only dependent on m. We also give a generalization of Levinson's theorem for these more general dispersion relations in WQED systems.
Rydberg polaritons provide an example of a rare type of system where three-body interactions can be as strong as or even stronger than two-body interactions.The three-body interactions can be either dispersive or dissipative, with both types possibly giving rise to exotic, strongly interacting, and topological phases of matter.Despite past theoretical and experimental studies of the regime with dispersive interaction, the dissipative regime is still mostly unexplored.Using a renormalization group technique to solve the quantum three-body problem, we show how the shape and strength of dissipative three-body forces can be universally enhanced for Rydberg polaritons.We demonstrate how these interactions relate to the transmission through a single-mode cavity, which can be used as a probe of the three-body physics in current experiments.
Strong coupling between light and matter has been demonstrated both in classical cavity quantum electrodynamics (QED) systems and in more recent circuit-QED experiments. This enables the generation of strong nonlinear photon-photon interactions at the single-photon level, which is of great interest for the observation of quantum nonlinear optical phenomena, the control of light quanta in quantum information protocols such as quantum networking, as well as the study of strongly correlated quantum many-body systems using light. Recently, strong coupling has also been realized in a variety of one-dimensional (1D) waveguide- QED experimental systems, which in turn makes them promising candidates for quantum information processing. Compared to cavity-QED systems, there are two new features in waveguide-QED: the existence of a continuum of states and the restricted 1D phase space, which together bring in new physical effects, such as the bound-state effects. This thesis consists of two parts: 1) understanding the fundamental interaction between local quantum objects, such as two-level systems and four-level systems, and photons confined in the waveguide; 2) exploring its implications in quantum information processing, in particular photonic quantum computation and quantum key distribution. First, we demonstrate that by coupling a two-level system (TLS) or three/fourlevel system to a 1D continuum, strongly-correlated photons can be generated inside the waveguide. Photon-photon bound states, which decay exponentially as a function of the relative coordinates of photons, appear in multiphoton scattering processes. As a result, photon bunching and antibunching can be observed in the photon-photon correlation function, and nonclassical light source can be generated on demand. In the case of an N-type four-level system, we show that the effective photon-photon interaction mediated by the four-level system, gives rise to a variety of nonlinear optical phenomena, including photon blockade, photon-induced tunneling, and creation of single-photon states and photon pairs with a high degree of spectral entanglement, all in the absence of a cavity. However, to enable greater quantum networking potential using waveguide- QED, it is important to study systems having more than just one TLS/qubit. We develop a numerical Green function method to study cooperative effects in a system of two qubits coupled to a 1D waveguide. Quantum beats emerge in photon-photon correlations, and persist to much longer time scales because of non-Markovian processes. In addition, this system can be used to generate a high-degree of long-distance entanglement when one of the two qubits is driven by an on-resonance laser, further paving the way toward waveguide-QED-based quantum networks. Furthermore, based on our study of light-matter interactions in waveguide- QED, we investigate its implications in quantum information processing. First, we study quantum key distribution using the sub-Possonian single photon source obtained by scattering a coherent state off a two-level system. The rate for key generation is found to be twice as large as for other sources. Second, we propose a new scheme for scalable quantum computation using flying qubits--propagating photons in a one-dimensional waveguide--interacting with matter qubits. Photonphoton interactions are mediated by the coupling to a three- or four-level system, based on which photon-photon -phase gates (Controlled-NOT) can be implemented for universal quantum computation. We show that high gate fidelity is possible given recent dramatic experimental progress in superconducting circuits and photonic-crystal waveguides. The proposed system can be an important building block for future on-chip quantum networks.
Waveguide quantum electrodynamics (waveguide QED) describes the interaction between an electromagnetic field confined to a one-dimensional waveguide with atom-like quantum emitters close by. The characteristics of these kinds of systems are the possibility for strong and even ultrastrong interactions between the photonic and atom-like systems, and practically infinite range interactions between the emitters. These properties are valuable for a wide range of quantum optical applications, like quantum communication, quantum networks and quantum metrology. In this thesis we focus on two challenges in quantum optics, namely the generation and scattering of multiphoton states. In the first part of this thesis we demonstrate how waveguide QED systems can be exploited for the generation of multiphoton states, in particular of single-mode Fock states and superpositions thereof as well as multi-mode photonic states with metrological applications. The basic setup for this goal is an ensemble of quantum emitters coupled to a waveguide. In the so-called atomic mirror configuration symmetric Dicke states (or a superposition thereof) decay superradiantly to the ground state and emit the desired multiphoton state, which can be efficiently collected at the ends of the waveguide. We propose various protocols for the preparation of these Dicke states in waveguide QED systems and characterize the emitted photonic state. It turns out that in the low excitation regime, that is, if the number of photons is much lower than the ensemble size, the photonic state is emitted into a single mode. This single-mode structure is fundamental to current proposals for applications in quantum metrology with optical interferometers. Outside the low excitation regime, a multi-mode photonic state is generated, for which the metrological capabilities were unknown. We were able to show that these states still lead to quantum-enhanced optical interferometry. In the second part of this thesis we demonstrate how the scattering of multiphoton states on a single quantum emitter coupled to the waveguide can be used for testing the limits of the light-matter interaction strength. In particular, we investigate systems in the so-called ultrastrong coupling regime, where the coupling strength between the photonic and atom-like system is of the order of the emitter's transition energy. In this regime, many methods and approximations used in quantum optics, especially the Rotating Wave Approximation, break down and one needs to develop new analytical and numerical methods to study these systems. One approach is the so-called polaron Transformation. We show how this transformation can be applied for predicting the scattering amplitude of few photons scattering on the emitter. The comparison of these results with numerical simulations using matrix product states shows a good agreement for moderate coupling strengths. Both parts together show that waveguide QED systems are promising candidates for the generation of multiphoton states as well as for the investigation of fundamental limits probed through the scattering of multiphoton states. The latter also finds application in the implementation of photon-photon nonlinearities induced by the interaction with the quantum emitters. Apart from these and many other theoretical predictions, waveguide QED systems are also undergoing rapid progress in experiments. Therefore, we expect these kinds of systems to bring forth several advances in the field of quantum optics.
At the quantum many-body level, atom-light interfaces generally remain challenging to solve for or understand in a nonperturbative fashion. Here we consider a waveguide quantum electrodynamics model, where two-level atoms interact with and via propagating photons in a one-dimensional waveguide, and specifically investigate the interplay of atomic position disorder, multiple scattering of light, quantum nonlinear interactions, and dissipation. We develop qualitative arguments and present numerical evidence that such a system exhibits a many-body localized (MBL) phase, provided that atoms are less than half excited. Interestingly, while MBL is originally formulated with respect to closed systems, this system is intrinsically open. However, as dissipation originates from transport of energy to the system boundaries and the subsequent radiative loss, the lack of transport in the MBL phase makes the waveguide QED system look essentially closed and makes applicable the notions of MBL. Conversely, we show that if the system is initially in a delocalized phase due to a large excitation density, then rapid initial dissipation can leave the system unable to efficiently transport energy at later times, resulting in a dynamical transition to an MBL phase. These phenomena can be feasibly realized in state-of-the-art experimental setups.
This review describes the emerging field of waveguide quantum electrodynamics (WQED) concerned with the interaction of photons propagating in a waveguide with localized quantum emitters. The collective emitter-photon interactions can lead to both enhanced and suppressed coupling compared to the case of independent emitters. Here, we focus on guided photons and ordered arrays, leading to super- and sub-radiant states, bound photon states and quantum correlations with promising quantum information applications. We highlight recent groundbreaking experiments performed with different quantum platforms, including cold atoms, superconducting qubits, semiconductor quantum dots, quantum solid-state defects, and we provide a comprehensive introduction to theoretical techniques to study the interactions and dynamics of these emitters and the photons in the waveguide.
Understanding physical properties of quantum emitters strongly interacting with quantized electromagnetic modes is one of the primary goals in the emergent field of waveguide quantum electrodynamics (QED). When the light-matter coupling strength is comparable to or even exceeds energies of elementary excitations, conventional approaches based on perturbative treatment of light-matter interactions, two-level description of matter excitations, and photon-number truncation are no longer sufficient. Here we study in and out of equilibrium properties of waveguide QED in such nonperturbative regimes on the basis of a comprehensive and rigorous theoretical approach using an asymptotic decoupling unitary transformation. We uncover several surprising features ranging from symmetry-protected many-body bound states in the continuum to strong renormalization of the effective mass and potential; the latter may explain recent experiments demonstrating cavity-induced changes in chemical reactivity as well as enhancements of ferromagnetism or superconductivity. To illustrate our general results with concrete examples, we use our formalism to study a model of coupled cavity arrays, which is relevant to experiments in superconducting qubits interacting with microwave resonators or atoms coupled to photonic crystals. We examine the relation between our results and delocalization-localization transition in the spin-boson model; notably, we point out that a reentrant transition can occur in the regimes where the coupling strength becomes the dominant energy scale. We also discuss applications of our results to other problems in different fields, including quantum optics, condensed matter physics, and quantum chemistry.