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Physical review. B./Physical review. B

Dissipative quantum transport in a nanowire

Malay Bandyopadhyay, Sushanta Dattagupta

Published Sep 1, 2021• 7 citations
Publisher

Abstract

The coherence-to-decoherence transition is studied in a nanowire modeled as a one-dimensional tight-binding lattice in the presence of an external field and in linear interaction with a boson heat bath, characterized by Ohmic dissipation. The focus of attention is the probability propagator which quantifies the likelihood of a quantum particle, such as an electron to end up at an arbitrary site at a time $t$, given that it was at the origin initially---and from it---the particle-current and the mean-squared displacement. If the bath is absent, the probability operator exhibits quantum coherence as can be captured by say, Bloch oscillation and Wannier-Stark (dynamic) localization. The coupling with the bath---which can be weak or strong---leads to decoherence that will be quantified in the text. The Ohmic model of the spectral function of bath excitations contains a cutoff frequency, which if greater than the temperature (in energy units) defines the ``low-temperature'' regime, whereas the opposite limit implies ``high temperatures.'' Results will be presented in both these regimes separately.

DOI
10.1103/physrevb.104.125401

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In this PhD thesis we have been concerned with dissipative and decoherence processes which take place specifically for quantum systems in a dissipative bistable potential. This potential describes a Hamiltonian system whose spectrum is composed by a ladder of levels, grouped as doublets under the potential barrier and being almost equally spaced above it. The system interacts with a thermal environment, fully characterized by the so-called bath spectral density. The dynamical quantity we looked at is the so-called reduced density matrix (RDM), obtained by tracing out the full density matrix the environmental degrees of freedom. The matrix elements for the RDM are exactly evaluated by means of the Feynman-Vernon real-time path-integral technique. Depending on which regime of parameters we are interested in, i.e. temperature and coupling strength with the reservoir, a few or several energy levels contribute to the dynamics. In particular, a two-level system (TLS) is first analyzed, corresponding to the regime where only the lowest doublet is energetically accessible. We discussed in the beginning the case of a TLS interacting with Ohmic and super-Ohmic baths and then the situation in which a symmetric TLS is assumed to be coupled with an external detector, like a dc-SQUID, the latter being coupled to an Ohmic environment. This model provides a better description of a real qubit, as frequently discussed in various experiments. In the former case, we developed a theory called Weakly-Interacting Blip Approximation (WIBA), which is nonperturbative in the coupling strength as well as in the tunneling frequency and gives reliable results over a wide range of temperatures and coupling strength to the thermal environment. In the latter case, the dynamics was evaluated upon starting from the Non-Interacting Blip Approximation (NIBA) and approximating the NIBA kernels up to first order in the detector-bath coupling strength. Analytical results, valid also at finite detuning, were obtained and we showed that our theory correctly reproduces the onset of multiple oscillation frequencies in the dynamics due to the entanglement between TLS and detector. Finally, we discussed the more general case of an M-level system coupled with an Ohmic environment. This situation describes the case of a bistable potential where the temperature is high enough that higher-lying energy levels are being populated and the system cannot be reduced to a simple TLS. Many are the experimental situations which can be described by our theory. We developed a novel approximation called Weakly-Interacting VR-Blip Approximation (VR-WIBA) for the dynamics in a driven dissipative bistable potential. In the regimes of low to moderate temperatures and coupling strengths, we exploited a separation of time scales between tunneling and vibrational relaxation events and we could derive analytical kernels for the intra- and inter-well dynamics.

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Quantum dissipation has been the object of study within the physics and chemistry communities for many years. Despite this, the field is in constant evolution, largely due to the fact that novel systems where the understanding of dissipation and dephasing processes is of crucial importance have become experimentally accessible in recent years. Among the ongoing research themes, we mention the defeat of decoherence in solid state-based quantum bits (qubits) (e.g. superconducting qubits or quantum dot based qubits), or dissipation due to non-equilibrium Fermi reservoirs, as is the case for quantum transport through meso- and nanoscale structures. A close inspection of dissipation in such systems reveals that one has to deal with 'unconventional' environments, where common assumptions of, for example, linearity of the bath and/or equilibrium reservoir have to be abandoned. Even for linear baths at equilibrium it might occur that the bath presents some internal structure, due, for example, to the presence of localized bath modes. A large part of this focus issue is devoted to topics related to the rapidly developing fields of quantum computation and information with solid state nanodevices. In these implementations, single and two-qubit gates as well as quantum information transmission takes place in the presence of broadband noise that is typically non-Markovian and nonlinear. On both the experimental and theory side, understanding and defeating such noise sources has become a crucial step towards the implementation of efficient nanodevices. On a more fundamental level, electron and spin transport through quantum dot nanostructures may suffer from 'unconventional' dissipation mechanisms such as the simultaneous presence of spin relaxation and fermionic dissipation, or may represent themselves out of equilibrium baths for nearby mesoscopic systems. Finally, although not expected from the outset, the present collection of articles has revealed that different 'unconventional' questions were still open on the standard harmonic oscillator and spin baths. This includes both fundamental issues, such as the possibility of estimating the specific heat for a free particle in the presence of dissipation, and the development of methods suitable to dealing with long range correlations at zero temperature and with quantum chaotic environments. We believe that the present focus issue on Quantum Dissipation in Unconventional Environments , although certainly not exhaustive, provides an important open-access resource that presents the latest state of the art of research in this field along its different lines. Focus on Quantum Dissipation in Unconventional Environments Contents Coherent control of an effective two-level system in a non-Markovian biomolecular environment J Eckel, J H Reina and M Thorwart Charge transfer dynamics in driven molecular ratchets: quantum Monte Carlo results and rate models L Mühlbacher and J Ankerhold Decoherence in qubits due to low-frequency noise J Bergli, Y M Galperin and B L Altshuler Dephasing by electron–electron interactions in a ballistic Mach–Zehnder interferometer Clemens Neuenhahn and Florian Marquardt Quantum frustration of dissipation by a spin bath D D Bhaktavatsala Rao, Heiner Kohler and Fernando Sols A random matrix theory of decoherence T Gorin, C Pineda, H Kohler and T H Seligman Dissipative dynamics of a biased qubit coupled to a harmonic oscillator: analytical results beyond the rotating wave approximation Johannes Hausinger and Milena Grifoni Dissipative dynamics of a two-level system resonantly coupled to a harmonic mode Frederico Brito and Amir O Caldeira Spin correlations in spin blockade Rafael Sánchez, Sigmund Kohler and Gloria Platero Landau–Zener tunnelling in dissipative circuit QED David Zueco, Peter Hänggi and Sigmund Kohler Quantum oscillations in the spin-boson model: reduced visibility from non-Markovian effects and initial entanglement F K Wilhelm Dynamics of dissipative coupled spins: decoherence, relaxation and effects of a spin-boson bath P Nägele, G Campagnano and U Weiss Spin chain model for correlated quantum channels Davide Rossini, Vittorio Giovannetti and Simone Montangero Finite quantum dissipation: the challenge of obtaining specific heat Peter Hänggi, Gert-Ludwig Ingold and Peter Talkner Dynamics of large anisotropic spin in a sub-ohmic dissipative environment close to a quantum-phase transition Frithjof B Anders Effects of low-frequency noise cross-correlations in coupled superconducting qubits A D'Arrigo, A Mastellone, E Paladino and G Falci From coherent motion to localization: dynamics of the spin-boson model at zero temperature Haobin Wang and Michael Thoss Phonon distributions of a single-bath mode coupled to a quantum dot F Cavaliere, G Piovano, E Paladino and M Sassetti

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The dissipative dynamics of a quantum bistable system coupled to a Ohmic heat bath is investigated beyond the spin-boson approximation. Within the path-integral approach to quantum dissipation, we propose an approximation scheme which exploits the separation of time scales between intra- and interwell (tunneling) dynamics. The resulting generalized master equation for the populations in a space localized basis enables us to investigate a wide range of temperatures and system-environment coupling strengths. A phase diagram in the coupling-temperature space is provided to give a comprehensive account of the different dynamical regimes.

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Zhiguo Lü, Hang Zheng

The decoherence of a two-state system coupled with a sub-Ohmic bath is investigated theoretically by means of the perturbation approach based on a unitary transformation. It is shown that the decoherence depends strongly and sensitively on the structure of environment. Nonadiabatic effect is treated through the introduction of a function ${\ensuremath{\xi}}_{k}$ which depends on the boson frequency and renormalized tunneling. The results are as follows: (i) the nonequilibrium correlation function $P(t)$, the dynamical susceptibility ${\ensuremath{\chi}}^{\ensuremath{''}}(\ensuremath{\omega})$, and the equilibrium correlation function $C(t)$ are analytically obtained for $s\ensuremath{\leqslant}1$; (ii) the phase diagram of thermodynamic transition shows the delocalized-localized transition point ${\ensuremath{\alpha}}_{l}$ which agrees with exact results and numerical data from the numerical renormalization group; (iii) the dynamical transition point ${\ensuremath{\alpha}}_{c}$ between coherent and incoherent phase is explicitly given. A crossover from the coherent oscillation to incoherent relaxation appears with increasing coupling (for $\ensuremath{\alpha}>{\ensuremath{\alpha}}_{c}$, the coherent dynamics disappear); (iv) the Shiba's relation and sum rule are exactly satisfied when $\ensuremath{\alpha}\ensuremath{\leqslant}{\ensuremath{\alpha}}_{c}$; (v) an underdamping-overdamping transition point ${\ensuremath{\alpha}}_{c}^{*}$ exists in the function $S(\ensuremath{\omega})$. Consequently, the dynamical phase diagrams in both ohmic and sub-Ohmic case are mapped out. For $\ensuremath{\Delta}⪡{\ensuremath{\omega}}_{c}$, the critical couplings (${\ensuremath{\alpha}}_{l},{\ensuremath{\alpha}}_{c}$, and ${\ensuremath{\alpha}}_{c}^{*}$) are proportional to ${\ensuremath{\Delta}}^{1\ensuremath{-}s}$.

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The coherence-to-decoherence transition is studied in a nanowire modeled as a one-dimensional tight-binding lattice in the presence of an external field and in linear interaction with a boson heat bath, characterized by Ohmic dissipation. The focus of attention is the probability propagator which quantifies the likelihood of a quantum particle, such as an electron to end up at an arbitrary site at a time ttt, given that it was at the origin initially---and from it---the particle-current and the mean-squared displacement. If the bath is absent, the probability operator exhibits quantum coherence as can be captured by say, Bloch oscillation and Wannier-Stark (dynamic) localization. The coupling with the bath---which can be weak or strong---leads to decoherence that will be quantified in the text. The Ohmic model of the spectral function of bath excitations contains a cutoff frequency, which if greater than the temperature (in energy units) defines the low-temperature'' regime, whereas the opposite limit implies high temperatures.'' Results will be presented in both these regimes separately.
Abstract The quantum dissipative dynamics of a particle which tunnels through the barrier of a double well potential and is coupled to an Ohmic heat bath is studied. Exact formal expressions for correlation functions are presented and examined. Attention is focused on the region in which coherence effects are important, and on the algebraic long‐time tails at zero temperature. Coherence effects in the dissipative quantum transport of a particle in a tight‐binding lattice are also investigated.
Abstract We derive a non-Markovian master equation for a charged particle in a magnetic field coupled to a bath and study decoherence by analyzing the temporal decay of the off-diagonal elements of the reduced density matrix in the position basis. The coherent oscillations characterized by the cyclotron frequency get suppressed as a result of decoherence due to coupling with the environment. We consider an Ohmic bath with three distinct models for the high-frequency cutoff for the spectral density of the bath and compare the three cases. As expected, the three cutoff models converge in the limit of the uppermost frequency of the bath tending to infinity. We notice a dramatic slowing down of loss of coherence in the low-temperature limit dominated by zero point quantum fluctuations compared to the high-temperature classical limit dominated by thermal fluctuations. We also go beyond the Ohmic model and study super-Ohmic and sub-Ohmic baths with the spectral densities deviating from a linear dependence on the frequency. Our results are testable in a state of the art cold atom laboratory.
In this PhD thesis we have been concerned with dissipative and decoherence processes which take place specifically for quantum systems in a dissipative bistable potential. This potential describes a Hamiltonian system whose spectrum is composed by a ladder of levels, grouped as doublets under the potential barrier and being almost equally spaced above it. The system interacts with a thermal environment, fully characterized by the so-called bath spectral density. The dynamical quantity we looked at is the so-called reduced density matrix (RDM), obtained by tracing out the full density matrix the environmental degrees of freedom. The matrix elements for the RDM are exactly evaluated by means of the Feynman-Vernon real-time path-integral technique. Depending on which regime of parameters we are interested in, i.e. temperature and coupling strength with the reservoir, a few or several energy levels contribute to the dynamics. In particular, a two-level system (TLS) is first analyzed, corresponding to the regime where only the lowest doublet is energetically accessible. We discussed in the beginning the case of a TLS interacting with Ohmic and super-Ohmic baths and then the situation in which a symmetric TLS is assumed to be coupled with an external detector, like a dc-SQUID, the latter being coupled to an Ohmic environment. This model provides a better description of a real qubit, as frequently discussed in various experiments. In the former case, we developed a theory called Weakly-Interacting Blip Approximation (WIBA), which is nonperturbative in the coupling strength as well as in the tunneling frequency and gives reliable results over a wide range of temperatures and coupling strength to the thermal environment. In the latter case, the dynamics was evaluated upon starting from the Non-Interacting Blip Approximation (NIBA) and approximating the NIBA kernels up to first order in the detector-bath coupling strength. Analytical results, valid also at finite detuning, were obtained and we showed that our theory correctly reproduces the onset of multiple oscillation frequencies in the dynamics due to the entanglement between TLS and detector. Finally, we discussed the more general case of an M-level system coupled with an Ohmic environment. This situation describes the case of a bistable potential where the temperature is high enough that higher-lying energy levels are being populated and the system cannot be reduced to a simple TLS. Many are the experimental situations which can be described by our theory. We developed a novel approximation called Weakly-Interacting VR-Blip Approximation (VR-WIBA) for the dynamics in a driven dissipative bistable potential. In the regimes of low to moderate temperatures and coupling strengths, we exploited a separation of time scales between tunneling and vibrational relaxation events and we could derive analytical kernels for the intra- and inter-well dynamics.
Quantum dissipation has been the object of study within the physics and chemistry communities for many years. Despite this, the field is in constant evolution, largely due to the fact that novel systems where the understanding of dissipation and dephasing processes is of crucial importance have become experimentally accessible in recent years. Among the ongoing research themes, we mention the defeat of decoherence in solid state-based quantum bits (qubits) (e.g. superconducting qubits or quantum dot based qubits), or dissipation due to non-equilibrium Fermi reservoirs, as is the case for quantum transport through meso- and nanoscale structures. A close inspection of dissipation in such systems reveals that one has to deal with 'unconventional' environments, where common assumptions of, for example, linearity of the bath and/or equilibrium reservoir have to be abandoned. Even for linear baths at equilibrium it might occur that the bath presents some internal structure, due, for example, to the presence of localized bath modes. A large part of this focus issue is devoted to topics related to the rapidly developing fields of quantum computation and information with solid state nanodevices. In these implementations, single and two-qubit gates as well as quantum information transmission takes place in the presence of broadband noise that is typically non-Markovian and nonlinear. On both the experimental and theory side, understanding and defeating such noise sources has become a crucial step towards the implementation of efficient nanodevices. On a more fundamental level, electron and spin transport through quantum dot nanostructures may suffer from 'unconventional' dissipation mechanisms such as the simultaneous presence of spin relaxation and fermionic dissipation, or may represent themselves out of equilibrium baths for nearby mesoscopic systems. Finally, although not expected from the outset, the present collection of articles has revealed that different 'unconventional' questions were still open on the standard harmonic oscillator and spin baths. This includes both fundamental issues, such as the possibility of estimating the specific heat for a free particle in the presence of dissipation, and the development of methods suitable to dealing with long range correlations at zero temperature and with quantum chaotic environments. We believe that the present focus issue on Quantum Dissipation in Unconventional Environments , although certainly not exhaustive, provides an important open-access resource that presents the latest state of the art of research in this field along its different lines. Focus on Quantum Dissipation in Unconventional Environments Contents Coherent control of an effective two-level system in a non-Markovian biomolecular environment J Eckel, J H Reina and M Thorwart Charge transfer dynamics in driven molecular ratchets: quantum Monte Carlo results and rate models L Mühlbacher and J Ankerhold Decoherence in qubits due to low-frequency noise J Bergli, Y M Galperin and B L Altshuler Dephasing by electron–electron interactions in a ballistic Mach–Zehnder interferometer Clemens Neuenhahn and Florian Marquardt Quantum frustration of dissipation by a spin bath D D Bhaktavatsala Rao, Heiner Kohler and Fernando Sols A random matrix theory of decoherence T Gorin, C Pineda, H Kohler and T H Seligman Dissipative dynamics of a biased qubit coupled to a harmonic oscillator: analytical results beyond the rotating wave approximation Johannes Hausinger and Milena Grifoni Dissipative dynamics of a two-level system resonantly coupled to a harmonic mode Frederico Brito and Amir O Caldeira Spin correlations in spin blockade Rafael Sánchez, Sigmund Kohler and Gloria Platero Landau–Zener tunnelling in dissipative circuit QED David Zueco, Peter Hänggi and Sigmund Kohler Quantum oscillations in the spin-boson model: reduced visibility from non-Markovian effects and initial entanglement F K Wilhelm Dynamics of dissipative coupled spins: decoherence, relaxation and effects of a spin-boson bath P Nägele, G Campagnano and U Weiss Spin chain model for correlated quantum channels Davide Rossini, Vittorio Giovannetti and Simone Montangero Finite quantum dissipation: the challenge of obtaining specific heat Peter Hänggi, Gert-Ludwig Ingold and Peter Talkner Dynamics of large anisotropic spin in a sub-ohmic dissipative environment close to a quantum-phase transition Frithjof B Anders Effects of low-frequency noise cross-correlations in coupled superconducting qubits A D'Arrigo, A Mastellone, E Paladino and G Falci From coherent motion to localization: dynamics of the spin-boson model at zero temperature Haobin Wang and Michael Thoss Phonon distributions of a single-bath mode coupled to a quantum dot F Cavaliere, G Piovano, E Paladino and M Sassetti
The dissipative dynamics of a quantum bistable system coupled to a Ohmic heat bath is investigated beyond the spin-boson approximation. Within the path-integral approach to quantum dissipation, we propose an approximation scheme which exploits the separation of time scales between intra- and interwell (tunneling) dynamics. The resulting generalized master equation for the populations in a space localized basis enables us to investigate a wide range of temperatures and system-environment coupling strengths. A phase diagram in the coupling-temperature space is provided to give a comprehensive account of the different dynamical regimes.
The decoherence of a two-state system coupled with a sub-Ohmic bath is investigated theoretically by means of the perturbation approach based on a unitary transformation. It is shown that the decoherence depends strongly and sensitively on the structure of environment. Nonadiabatic effect is treated through the introduction of a function ${\ensuremath{\xi}}_{k}$ which depends on the boson frequency and renormalized tunneling. The results are as follows: (i) the nonequilibrium correlation function P(t)P(t)P(t), the dynamical susceptibility ${\ensuremath{\chi}}^{\ensuremath{''}}(\ensuremath{\omega})$, and the equilibrium correlation function C(t)C(t)C(t) are analytically obtained for $s\ensuremath{\leqslant}1$; (ii) the phase diagram of thermodynamic transition shows the delocalized-localized transition point ${\ensuremath{\alpha}}_{l}$ which agrees with exact results and numerical data from the numerical renormalization group; (iii) the dynamical transition point ${\ensuremath{\alpha}}_{c}$ between coherent and incoherent phase is explicitly given. A crossover from the coherent oscillation to incoherent relaxation appears with increasing coupling (for $\ensuremath{\alpha}>{\ensuremath{\alpha}}_{c}$, the coherent dynamics disappear); (iv) the Shiba's relation and sum rule are exactly satisfied when $\ensuremath{\alpha}\ensuremath{\leqslant}{\ensuremath{\alpha}}_{c}$; (v) an underdamping-overdamping transition point ${\ensuremath{\alpha}}_{c}^{*}$ exists in the function $S(\ensuremath{\omega})$. Consequently, the dynamical phase diagrams in both ohmic and sub-Ohmic case are mapped out. For $\ensuremath{\Delta}⪡{\ensuremath{\omega}}_{c}$, the critical couplings (${\ensuremath{\alpha}}_{l},{\ensuremath{\alpha}}_{c}$, and ${\ensuremath{\alpha}}_{c}^{*}$) are proportional to ${\ensuremath{\Delta}}^{1\ensuremath{-}s}$.