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Superconducting nanowire single photon detectors for high-rate quantum communication

Matthieu Perrenoud

Published Jan 1, 2021• 0 citations
Publisher

Abstract

The important development of quantum technologies during the past decade brought the need for efficient, fast and precise single-photon detection. Superconducting Nanowire Single-Photon Detectors (SNSPDs) are currently considered as the detection method of choice when extreme performances are required. This thesis aimed at investigating this technology, with the objective of improving existing detectors for high-rate applications in quantum communication. This document presents the work and result achieved over four years dedicated to the subject. During this thesis, single-photon detection based on superconducting nanowire has been investigated, with a particular focus on specific requirements for high speed quantum communication applications. The work achieved ranges from the design and nano-fabrication of the structures, to the characterization and the understanding of the physics, detection models and fundamental limits of the devices.

DOI
10.13097/archive-ouverte/unige:153779

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The important development of quantum technologies during the past decade brought the need for efficient, fast and precise single-photon detection. Superconducting Nanowire Single-Photon Detectors (SNSPDs) are currently considered as the detection method of choice when extreme performances are required. This thesis aimed at investigating this technology, with the objective of improving existing detectors for high-rate applications in quantum communication. This document presents the work and result achieved over four years dedicated to the subject. During this thesis, single-photon detection based on superconducting nanowire has been investigated, with a particular focus on specific requirements for high speed quantum communication applications. The work achieved ranges from the design and nano-fabrication of the structures, to the characterization and the understanding of the physics, detection models and fundamental limits of the devices.
Single photon detection advanced rapidly in the last decade. The superconducting nanowire single-photon detector (SNSPD) is an emerging technology, which offers low dark count rates, broadband sensitivity from visible to mid-infrared wavelengths and very high quantum efficiency. All these features are appealing for future emerging applications in remote gas sensing, quantum key distribution and quantum information processing. By enclosing the detector in an optical cavity, tuned to the operating wavelength, the total system detection of the SNSPD is improved. Based on the cavity design, the detector absorption is boosted at the desired experimental wavelength. Devices have been fabricated and tested, in this thesis, with enhanced detection efficiency at near-infrared, infrared and mid-infrared wavelengths. NbTiN detectors fabricated on Ta2O5 / SiO2 distributed Bragg reflectors (DBR) for front-side coupling exhibit a system detection efficiency of ≈ 90% at λ = 940 nm for the best device measured. SNSPDs were also fabricated in NbTiN on metallic mirrors for back-side coupling for 1550 and 2333 nm experimental wavelengths. The first design exhibited a system detection efficiency of ≈ 84.5%, at λ = 1550 nm for the best device measured. The second exhibited low system detection efficiency since the device suffered from unexpectedly high dark count rate mainly due to blackbody radiation at 2.2 K. However, it was possible to measure the timing jitter of this device at 350 mK indicating a FWHM of 84 ps. Another technique to improve the total system detection efficiency of the SNSPD, is by fabricating a hairpin-shaped nanowire atop a single mode waveguide. In this design, photons travel through the waveguide and via evanescent coupling are absorbed in the nanowire. These SNSPD devices have been designed to thread along single mode Si ridge waveguides using a hairpin-shaped nanowire structure, which offers enhanced coupling and absorption efficiency via evanescent coupling. These ultra-thin superconducting MoSi detectors are precisely patterned on top of a single mode Si waveguide (600 nm) with alignment error less than 40 nm. Low temperature electrical and nano-optical characterization was carried out using a two-stage pulse tube (PT) coldhead, using an additional 4He / 3He sorption pump, low vibration characterization of SNSPD devices at 350 mK was carried out. Characterised devices exhibit low dark count rate <5 counts per second and timing jitter of ≈ 83 ps full width half maximum (FWHM) at wavelength (λ) = 1550 nm and at critical current ≈ 30 µA.
Superconducting nanowire single-photon detectors (SNSPDs) are renowned for their high detection efficiency, low dark count rate, and fast timing resolution, which have emerged as an essential device in quantum technologies, including quantum computing and communication, which also significantly benefits classical applications such as deep-space communication, neuromorphic computing, and light detection and ranging (LiDAR). However, designing and customizing SNSPD into versatile functionalities to satisfy these intensive requirements poses significant challenges, including thin-film deposition, nanofabrication, electrical integration, and light delivery strategies. While prior work has typically optimized individual steps – such as fabrication or characterization – there is a lack of reported systematic, integrated frameworks that span all stages from device design to performance benchmarking. This gap hinders broader adoption of the technology across scientific and industrial communities and limits the rigorous exploration of advanced detection concepts. This thesis aims to establish an end-to-end workflow for the customizable fabrication and comprehensive characterization of superconducting nanowire single-photon detectors, and to demonstrate that such a platform is essential for the investigation of diverse single-photon detection architectures. It begins with the optimization of NbTiN thin-film deposition utilizing an ultrahigh vacuum sputtering system. By systematically identifying and optimizing key deposition parameters, we achieve NbTiN films with targeted superconducting properties along with high uniformity and reproducibility. This fast and reliable workflow establishes a solid foundation for detector fabrication and provides instructions for flexible control over film properties. Furthermore, effective nanofabrication protocols for the high-quality SNSPDs were elaborated, along with the specialized cryogenic packaging techniques for reliable electrical and optical integration. The achieved devices demonstrated performance metrics comparable to commercial systems. The implementation of this full fabrication—characterization cycle also enabled flexible exploration of advanced detector architectures. For example, we investigated superconducting microbridge single-photon detectors (SMSPDs) as a complementary platform, demonstrating a fivefold enhancement in signal-to-noise ratio and a tenfold reduction in recovery time relative to conventional SNSPDs. These results provide quantitative insight into detector design trade-offs. Within this framework, photon-number-resolving (PNR) detection using SNSPDs was further investigated as an essential function for advanced quantum and classical applications. We presented innovative detector architectures—interleaved multi-pixel arrays and multilayer coherent absorption structures—to overcome limitations inherent in conventional multiplexing methods, such as nonuniform detection, temporal degradation, and crosstalk. An interleaved multi-pixel SNSPD array with up to four-photon resolution was achieved with uniform detection, as well as a multilayer architecture based on coherent absorption with uniform and near-unity absorption efficiency. Importantly, a theoretical comparison between these two architectures was conducted to evaluate their absorption efficiency and PNR performance, offering insights into structural optimization and device scalability for advanced PNR detectors. Overall, this thesis establishes a fully in-house SNSPD fabrication and characterization capability, providing a robust foundation for the development, customization, and evaluation of high-performance superconducting single-photon detectors. This platform enables reproducible design optimization, quantitative performance benchmarking, and systematic exploration of detector architectures. By integrating fabrication, characterization, and architectural innovation within a consistent workflow, it facilitates both fundamental investigation and application-driven advancement of single-photon detection technologies in our laboratory and the broader research community in Singapore.
Superconducting Nanowire Single Photon Detectors (SNSPDs) excel at a wide variety of performance criteria for single photon counting. They combine unprecedented high detection efficiency, high timing resolution, high count rates, low intrinsic dark count rates, and are sensitive to ultraviolet through mid-infrared single-photons. At JPL, we are working on several projects to push the performance limits of SNSPDs to achieve higher maximum count rates, larger active areas, higher timing resolution, and a wider spectral range. Our recent advances enable new applications for dark matter detection, imaging, and space-to-ground communication and provide insight into the fundamental physics of single-photon detection in superconducting nanowires.
Abstract Single‐photon detectors and nanoscale superconducting devices are two major candidates for realizing quantum technologies. Superconducting‐nanowire single‐photon detectors (SNSPDs) comprise these two solid‐state and optic aspects enabling high‐rate (1.3 Gb s −1 ) quantum key distribution over long distances (>400 km), long‐range quantum communication (>1200 km), as well as space communication (239 000 miles). The attractiveness of SNSPDs stems from competitive performance in the four single‐photon relevant characteristics at wavelengths ranges from UV to the mid‐IR: high detection efficiency, low false‐signal rate, low uncertainty in photon time arrival, and fast reset time. However, to date, these characteristics cannot be optimized simultaneously. In this review, the mechanisms that govern these four characteristics are presented, and it is demonstrated how they are affected by material properties and device design as well as by the operating conditions, allowing aware optimization of SNSPDs. Based on the evolution in the existing literature and state of the art, it is proposed how to choose or design the material and device for optimizing SNSPD performance, while possible future opportunities in the SNSPD technology are also highlighted.
Superconducting nanowire single-photon detectors (SNSPDs) have abstracted widespread attention in the fields of quantum information and quantum photonics due to their high detection efficiency and low dark count rates (DCR). However, single-pixel SNSPDs exist the notable limitations in detection speed and photon number resolution (PNR) capabilities, which pose challenges for practical applications. In this study, we propose a design of a series four-pixel SNSPD that incorporates a SPICE circuit simulation model to achieve PNR and spatial resolution of the four photons in an ideal state, and then determine the optical cavity structure of the detector at the highest light absorption of up to 97% through optical simulation. This design provides a theoretical foundation for the subsequent fabrication of large-area SNSPD with PNR and spatial resolution, significantly improving the flexibility and adaptability of SNSPDs to meet diverse detection requirements. Furthermore, our work also lays a research foundation for multi-photon detection in quantum communication and quantum computing.
Single photon detectors are a vital part of many emerging technologies which harness the quantum properties of light to benefit the fields of communication, computation and sensing. Superconducting nanowire single photon detectors (SNSPDs) offer high detection efficiency, low dark count rates, low timing jitter, and infrared sensitivity that are required by the most demanding single photon counting applications. This thesis presents SNSPDs fabricated and tested at the University of Glasgow that are integrated with optical structures which enable enhanced detection efficiency and integration with waveguide circuit technology. The monolithic integration of waveguide circuit components presents a route towards realisation of an optical quantum information processor that has the stability and scalability to perform the demanding tasks of quantum computation. A novel process is introduced for incorporating superconducting detectors with single mode gallium arsenide waveguides and quantum dot single photon sources. Together these elements would enable the generation of quantum states of light which could be manipulated and detected on a single chip. Detectors are patterned in NbTiN thin superconducting films on to suspended nanobeam waveguides with better than 50 nm alignment accuracy. Low temperature electrical and optical testing confirms the detectors’ single photon sensitivity under direct illumination as well as to waveguide coupled light. Measured detectors were found to have internal registering efficiencies of 6.8 ± 2.4%. Enhancing absorption of photons into thin superconducting films is vital to the creation of high efficiency superconducting single photon detectors. Fabricating an SNSPD on a dielectric mirror creates a partial cavity that can be tailored to enhance detection of light at specific wavelengths. Devices have been fabricated and tested in this thesis with enhanced detection efficiency at infrared and visible wavelengths for quantum cryptography, remote sensing and life science applications. Detectors fabricated in NbTiN on GaAs/AlGaAs Bragg mirrors exhibited a system detection efficiency of 1.5% at 1500 nm wavelength for the best device measured. SNSPDs were also fabricated in NbN on aperiodic dielectric mirrors with a range of different bandwidths. A peak system detection efficiency of 82.7% at 808 nm wavelength was recorded.