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Electron Phase Coherence and Correlations Probed in Electronic Interferometers

장동인

Published Jan 1, 2008• 0 citations
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Electronic and vibrational coherences of Cl2 embedded in solid Ar are investigated by exciting to the B state with a phase-locked pulse pair from an unbalanced Michelson interferometer, where the chirp difference matches the B state anharmonicity. Recording the A' --> X fluorescence after relaxation is compared to probing to charge transfer states by a third pulse. The three-pulse experiment delivers more details on the decoherence processes. The signal modulation due to phase tuning up to the third vibrational round-trip time indicates that the electronic coherence in the B <-- X transition is preserved for more than 660 fs in the solid Ar environment where many body electronic interactions take place. Vibrational coherence lasts longer than 3 ps according to the observed half revival of the wavepacket. Control of the coupling between wavepacket motion and lattice oscillation is demonstrated by tuning the relative phase between the phase-locked pulses, preparing wavepackets predominantly composed of either zero-phonon lines or phonon side bands.
The quantum correlation of light and atomic collective excitation can be used to compose an SU(1,1)-type hybrid light-atom interferometer, where one arm in the optical SU(1,1) interferometer is replaced by the atomic collective excitation. The phase-sensing probes include not only the photon field but also the atomic collective excitation inside the interferometer. For a coherent squeezed state as the phase-sensing field, the phase sensitivity can approach the Heisenberg limit under the optimal conditions. We also study the effects of the loss of light field and the dephasing of atomic excitation on the phase sensitivity. This kind of active SU(1,1) interferometer can also be realized in other systems, such as circuit quantum electrodynamics in microwave systems, which provides a different method for basic measurement using the hybrid interferometers.
An experiment is described which is an analog of Young's double-slit interferometer using an atomic electron instead of light. Two phase-coherent laser pulses are used to excite a single electron into a state of the form of a pair of Rydberg wave packets that are initially on opposite sides of the orbit. The two wave packets propagate and spread until they completely overlap, then a third phase-coherent laser pulse probes the resulting fringe pattern. The relative phase of the two wave packets is varied so that the interference produces a single localized electron wave packet on one side of the orbit or the other.