Interacting ultracold atomic quantum gases provide an ideal test bed to study strongly correlated quantum matter. The interactions between atoms in such an ultracold quantum gas are typically short-ranged and well described by an effective contact potential. Introducing longer-range interactions promises the realization of novel quantum phases which are absent in systems with only short-range interactions. Trapped atoms, resonantly laser-coupled to highly excited, strongly interacting Rydberg states have been proposed as a versatile platform to realize such long-range interacting quantum matter. In a first experiment presented in this thesis, we combined the single-atom-sensitive local preparation and detection enabled by a quantum gas microscope to prepare and microscopically characterize an ensemble of rubidium-87 atoms trapped in an optical lattice in the regime of strong Rydberg blockade. There, we observe collectively enhanced optical coupling in an effective two-level system, the so-called “superatom”, and infer the presence of entanglement. Detuned optical coupling to Rydberg states, termed “Rydberg dressing”, has been proposed as an alternative approach to induce long-range interactions. Rather than directly exciting an atom to a Rydberg state, the properties of the latter are admixed to a ground state, which consequently acquires long-range interactions. In the context of this thesis, we have designed a laser system in the ultraviolet spectral range to admix Rydberg P-state character to the ground state of atoms in an optical lattice. In an emerging Ising quantum magnet, the presence of Rydberg-dressed interactions was demonstrated by an interferometric technique combined with spatially resolved spin correlation measurements. The theoretically predicted tunability of the isotropy and range of the interaction were confirmed experimentally. While these initial measurements exhibited unexpected dissipation, in a subsequent experiment in a one-dimensional spin chain this dissipation was overcome. We substantiated the improved coherence times by tracking the time evolution of the magnetization upon suddenly switching on interactions and observing coherent collapse and revival dynamics, one of the hallmarks of coherent quantum evolution. Our results establish Rydberg-dressed interactions in ultracold gases and pave the way to realize and study novel exotic quantum phases.
We use 40K atoms trapped in a cubic optical lattice to simulate the Fermi-Hubbard model. The work in this thesis focuses on investigating dynamics in the Fermi-Hubbard model and developing techniques for engineering Hamiltonians beyond the minimal Hubbard model. We discussed three experiments. In the first, we investigated the transport properties of a Fermi lattice gas by directly measuring the transport lifetime at various interaction strengths and temperatures. The resistivity is inferred from the measured transport lifetime. We observe anomalous transport behavior, which is analogous to bad-metal behavior in strongly correlated electronic materials. The second experiment presents the first realization of correlated, density-dependent tunneling in a Fermi-Hubbard optical lattice model by applied Raman laser fields. This correlated tunneling involves spin-flips and the generation of doublons, which have been observed experimentally. We also confirmed that the amplitude of correlated tunneling is suppressed when neighboring lattice sites are unoccupied. The last experiment explores the possibility to introduce long-range interactions for fermions trapped in optical lattices via Rydberg-dressed states. We developed a novel velocity-selective spectroscopy method to measure the transition between the 5P_1/2 and Rydberg states via electromagnetically induced transparency. This measurement is a first step toward inducing Rydberg-dressed interactions in optical lattices.
We study theoretically the deformation of the Fermi surface (FS) of a three-dimensional gas of Rydberg-dressed
6Li atoms. The laser dressing to high-lying Rydberg
D states results in angle-dependent soft-core-shaped interactions whose anisotropy is described by multiple spherical harmonics. We show that this can drastically modify the shape of the FS and that its deformation depends on the interplay between the Fermi momentum
kF and the reciprocal momentum
k corresponding to the characteristic soft-core radius of the dressing-induced potential. When
kF<k, the dressed interaction stretches a spherical FS into an ellipsoid. When ${k}_{F}\ensuremath{\gtrsim}\overline{k}$, complex deformations are encountered which exhibit multipolar characteristics. We analyze the formation of Cooper pairs around the deformed FS and show that they occupy large orbital angular momentum states (
p,f, and
h wave) coherently. Our study demonstrates that Rydberg dressing to high angular momentum states may pave a route toward the investigation of unconventional Fermi gases and multiwave superconductivity.