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Nature Photonics

Nanoscale atomic suspended waveguides for improved vapour coherence times and optical frequency referencing

Roy Zektzer, Noa Mazurski, Yefim Barash, Uriel Levy

Published Aug 2, 2021• 44 citations
Publisher
DOI
10.1038/s41566-021-00853-4

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In recent years, there has been marked increase in research aimed to introduce alkali vapours into guided-wave configurations. Owing to the significant reduction in device dimensions, the increase in density of states, the interaction with surfaces and primarily the high intensities carried along the structure, a plethora of light-vapour interactions can be studied. Moreover, such platform may exhibit new functionalities such as low-power nonlinear light-matter interactions. One immense challenge is to study the effects of quantum coherence and shifts in nanoscale waveguides, characterized by ultra-small mode areas and fast dynamics. Here, we construct a highly compact 17 mm long serpentine silicon-nitride atomic vapour cladding waveguide. Fascinating and important phenomena such as van-der-Waals shifts, dynamical stark shifts and coherent effects such as strong coupling (in the form of Autler-Townes splitting) are observed. Some of these effects may play an important role in applications such as all-optical switching, frequency referencing and magnetometry.
In this work, we demonstrate - for the first time, to the best of our knowledge - electromagnetically induced transparency (EIT) on a fully integrated, chip-scale platform based on nanoscale tapered suspended waveguides surrounded by hot rubidium vapour. We further show that these waveguides enable the excitation of rubidium atoms to Rydberg states, and implement an electric readout scheme to detect these atoms by their ionisation currents. The fabrication workflow for standard ridge waveguides made of silicon nitride (Si3N4) is optimised, leading to significantly improved optical quality. Building on this, different techniques for locally suspending photonic structures out of Si3N4 are developed, allowing us to retain the waveguide interconnects between the structures on a conventional SiO2 layer for full chip integration. The use of a sacrificial silicon layer proves to be advantageous for suspending resonator structures, as this method does not change the optical properties of the device, as opposed to other established suspension methods. With these fabrication techniques, high quality suspended tapered waveguides are realised. Spectroscopy measurements on the D2 transition of rubidium confirm that the Doppler and transit time broadening are significantly reduced compared to standard ridge waveguides, owing to the extended evanescent field of the tapered geometry. After this, EIT is demonstrated on the tapered waveguides using a three level ladder scheme, benefiting from the longer atomic interaction times enabled by the extended evanescent field. The experimental results are compared to numerical simulations, showing good agreement. Finally, the excitation to Rydberg levels in the evanescent field of the tapered waveguide is investigated. An electrically contacted vapour cell is designed to detect the current from excited Rydberg atoms, ionised through collisions with ground-state atoms or perturber gases in the cell. Clear Rydberg signals are observed and compared with simulations modelling excitation and ionisation in the confined geometry of the evanescent field. The results indicate that the excitation can indeed occur within the guided mode and that the corresponding ionisation currents are of the same order of magnitude as those measured experimentally. However, strong scattering of the guided light is also observed at the transitions to the underetched regions, suggesting that a fraction of the Rydberg excitation may originate from this scattered light rather than from the evanescent field alone. Further investigations are ongoing at the time of writing to quantify this contribution.