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Physical Review A

Insights into Fano-type resonance fluorescence from quantum-dot–metal-nanoparticle molecules with a squeezed vacuum

Shu-Ting Shen, Zhiming Wu, Jiahua Li, Ying Wu

Published Jul 21, 2021• 23 citations

Abstract

Metal nanoparticles (MNPs) possess the intriguing property of enhancing and limiting the energy of light field to subwavelength scale, which have attracted extensive attention in physics, chemistry, and life sciences. Meanwhile, squeezing is a general concept in quantum optics and can be used to engineer matter interaction scenarios. Here we consider an artificial hybrid molecule consisting of an MNP interacting with a semiconductor quantum dot (QD), combining with a squeezed reservoir. Using experimentally realistic parameters for the MNP-QD architecture and fully quantized approach, we theoretically explore the optical properties of the hybrid molecule driven by an external applied laser field via probing the resonance fluorescence in the steady state. We show that in this way it is possible to engineer and control the peak-value magnitudes, widths, and shapes of the resonance fluorescence spectra under the influence of the squeezed vacuum field without the need for the strong-coupling condition between the MNP and QD. In particular, some interesting phenomena in rich spectral responses are attainable, including Fano-type resonance fluorescence, fluorescence quenching, fluorescence narrowing, and fluorescence enhancement. Our method can also be extended to other nanoscopic structures, such as a plasmonic nanoantenna coupled to an emitter. These unique line shapes obtained here may have potential applications in developing quantum plasmonic platforms and sensitive on-chip devices such as optical switches and sensors.

DOI: 10.1103/physreva.104.013717

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We study theoretically the quantum optical properties of hybrid molecules composed of an individual quantum dot and a metallic nanoparticle. We calculate the resonance fluorescence of this composite system. Its incoherent part, arising from nonlinear quantum processes, is enhanced by more than 2 orders of magnitude as compared to that of the dot alone. The coupling between the two systems gives rise to a Fano interference effect which strongly influences the quantum statistical properties of the scattered photons: a small frequency shift of the incident light field may cause changes in the intensity correlation function of the scattered field of orders of magnitude. The system opens a good perspective for applications in active metamaterials and ultracompact single-photon devices.

In the present work, we investigate the modified nonlinear pump-probe optical properties due to the excitonic–plasmonic interaction of a double semiconductor quantum dot (SQD) molecule coupled to a metal nanoparticle (MNP). More specifically, we study the absorption and the dispersion spectra of a weak electromagnetic field in a hybrid structure with two counterparts, a molecule of two coupled SQDs, and a spherical MNP driven by a field of high intensity. We solve the relevant density matrix equations, calculate the first-order optical susceptibility of the probe field in the strong pumping regime, and investigate the way in which the distance between the two counterparts modifies the optical response, for a variety of values of the physical constants of the system, including the pump-field detuning, the tunnelling rate, and the energy separation gap associated with the excited states of the coupled SQDs.

The emergence of hybrid nanostructures has paved a novel path for the development of nanotechnology and next-generation quantum devices.In this study, we report a remarkable enhancement of nonlinear diffraction achieved within a hybrid artificial molecule consisting of a semiconductor quantum dot (SQD) and a metal nanoparticle (MNP).Our findings reveal that the optical nonlinear properties of the hybrid system can be substantially enhanced due to the plasmon resonance of MNP.Specifically, reducing the interparticle distance and the SQD's size while increasing the MNP's size leads to a significant enhancement in the nonlinear phase modulation of the hybrid system.Meanwhile, the absorption spectra exhibit a redshift accompanied by linewidth broadening under the SQD-MNP coupling interaction controlled by geometric parameters, indicating plasmon-exciton energy transfer.On this basis, it is validated that the enhanced nonlinear phase modulation greatly improves the self-imaging visibility and the signal-to-noise ratio, and extends the near-field pattern over more Talbot lengths.We also demonstrate that the far-field diffraction efficiency is tunable via the coupling interaction between the artificial molecule and external fields, which is determined by the geometric structure, photon detuning, and Rabi frequency.For instance, the first-order diffraction efficiency can be increased from 39.58% to 55% if the geometric parameters of the hybrid system satisfy the threshold in non-resonance conditions.Such plasmon-enhanced optical lattices show potential for applications in all-optical modulators and all-optical switches operating at few-photon levels, and may also afford a novel perspective for the design and development of nanophotonics circuits and topological photonic devices.

Abstract We theoretically demonstrate the Fano resonance and the conversion from fast to slow light in a hybrid semiconductor quantum dot (SQDs)-metal nanoparticle (MNPs) with cavity quantum electrodynamics treatment. The absorption spectra of the weak probe field exhibit a series of asymmetric Fano line shapes and their related optical propagation properties, such as fast and slow light effects, are investigated based on the hybrid system for suitable parametric regimes. Further, the transparency windows (i.e. the absorption dip approaches zero) in the probe absorption spectra are accompanied by the rapid steep dispersion of the Fano resonance profile, which promises the slow or fast light effect, and even tunable fast-to-slow light propagation (or vice versa) can be achieved by controlling different parameter regimes. Therefore the investigation may indicate promising applications in quantum information processing based on the hybrid SQD-MNP system.

We theoretically study the interaction between two semiconductor quantum dots (SQDs) and a metal nanoparticle\ (MNP) within the quantum description. The plasmon field produced in the MNP excited by the external field can play the platform of F\"{o}rster energy transfer between two SQDs which gives rise to the generation of entangled states. The Fano effect can be shown in the energy absorption spectrum of MNP, which originates from constructive or destructive interference between two competing optical pathways. Since the generated entangled state is in one pathway, the steady-state concurrence of entanglement can be evaluated by the observation of Fano profile. Because the concurrence of two SQDs is determined by both the pump intensity and the energy difference, one can properly choose these two parameters for detecting the non-negligible entanglement. When the pump intensity is very strong, there is no entanglement. The method to observe entanglement with the Fano profile, so, has a limited range of applicability. The optical observation is a novel approach to reveal entanglement. It may be used to optically detect quantum entanglement in many solid-state systems.