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Science Advances

Controlling the uncontrollable: Quantum control of open-system dynamics

Shimshon Kallush, Roie Dann, Ronnie Kosloff

Published Nov 2, 2022• 30 citations
Publisher

Abstract

Control of open quantum systems is essential for the realization of contemporary quantum science and technology. We demonstrate such control using a thermodynamically consistent framework, taking into account the fact that the drive can modify the system's interaction with the environment. Such an effect is incorporated within the dynamical equation, leading to control-dependent dissipation. This relation serves as the key element for open-system control. The control paradigm is displayed by analyzing entropy-changing state-to-state transformations, such as heating and cooling. The difficult task of controlling quantum gates is achieved for nonunitary reset maps with complete memory loss. In addition, we identify a mechanism for controlling unitary gates by actively removing entropy from the system to the environment. We demonstrate a universal set of single- and double-qubit unitary gates under dissipation.

DOI
10.1126/sciadv.add0828

Related papers

Controlling the uncontrollable: Quantum control of open system dynamics

Shimshon Kallush, Roie Dann, Ronnie Kosloff

Control of open quantum systems is an essential ingredient to the realization of contemporary quantum science and technology. We demonstrate such control by employing a thermodynamically consistent framework, taking into account the fact that the drive can modify the interaction with environment. Such an effect is incorporated within the dynamical equation, leading to control dependent dissipation, this relation serves as the key element for open system control. Thermodynamics of the control process is reflected by a unidirectional flow of energy to the environment resulting in large entropy production. The control paradigm is displayed by analyzing entropy changing state to state transformations, such as heating and cooling. In addition, the generation of quantum gates under dissipative conditions is demonstrated for both non-unitary reset maps with complete memory loss and a universal set of single and double qubit unitary gates.

arXiv:2205.05971•May 12, 2022•2 citations

Controlling the uncontrollable: Quantum control of open system dynamics

Shimshon Kallush, Roie Dann, Ronnie Kosloff

Quantum control of an open system is demonstrated employing a thermodynamically consistent master equation. In this framework, the open system dynamics depend on the control protocol due to the dressing of the system by the drive. This interrelation serves as the key element for control. The influence of the external drive is incorporated within the dynamical equation, enabling an indirect control of the dissipation. The control paradigm is displayed by analyzing entropy changing state to state transformations, heating and cooling N-level systems. Following, we study the generation of quantum non-unitary maps via coherent control. These include both reset maps with complete memory loss and single-qubit unitary maps under dissipative conditions.

arXiv:2107.11767•Jul 25, 2021•1 citation

Controlling open quantum systems

Benjamin Dive

All physical quantum systems are in contact with the external world which is inevitably a source of noise. It is therefore necessary to take into account this dissipation when designing controls that accomplish useful tasks in quantum information processing. This thesis is on that overlap of open quantum systems and control theory; it looks at what dynamics can happen with the use of external driving, and how this driving can be chosen to accomplish a desired goal. The first result looks at how a given quantum dissipator can be manipulated, using coherent controls, into replicating the action of a different type of noise. This results in no-go theorems for how noise can be transformed based on its isotropy, with applications in simulating open systems. Another way of doing simulations is to use only unitary dynamics over the system and a finite dimensional ancilla, and it is proved that there always exists a dilation Hamiltonian that replicates the noisy dynamics continuously in time. This also highlights the fact that adding controls on noise can result in a different evolution than if the controls were done on the under- lying system-environment level. A conjecture is introduced and studied which states that both approaches are equivalent in the special case of the controls commuting with the Lindbladian. A way around this difficulty is to use a quantum system to compute in situ which controls are best for achieving a desired task on itself. This problem is studied in the context of reaching entangling gates on a quantum simulator in order to upgrade it into a quantum computer. The experimental cost of doing so is found to be polynomial in the number of qubits in simulations. The same underlying principle is also used to find error correcting codes tailored to the dissipation in a system.

•Sep 1, 2017•2 citations

Effectiveness of the Krotov method in controlling open quantum systems

Marllos E. Fonseca, F. F. Fanchini, Emanuel F. de Lima +1 more

We apply the Krotov method for open and closed quantum systems with the objective of finding optimized controls to manipulate qubit/qutrit systems in the presence of the external environment. In the case of unitary optimization, the Krotov method is first applied to a quantum system neglecting its interaction with the environment. The resulting controls from the unitary optimization are then used to drive the system along with the environmental noise. In the case of non-unitary optimization, the Krotov method already takes into account the noise during the optimization process. We consider two distinct computational task: target-state preparation and quantum gate implementation. These tasks are carried out in simple qubit/qutrit systems and also in systems presenting leakage states. For the state-preparation cases, the controls from the non-unitary optimization outperform the controls from the unitary optimization. However, as we show here, this is not always true for the implementation of quantum gates. There are some situations where the unitary optimization performs equally well compared to the non-unitary optimization. We verify that these situations corresponds to either the absence of leakage states or to the effects of dissipation being spread uniformly over the system, including non-computational levels. For such cases, the quantum gate implementation must cover the entire Hilbert space and there is no way to dodge dissipation. On the other hand, if the subspace containing the computational levels and its complement are differently affected by dissipation, the non-unitary optimization becomes effective.

arXiv:2208.03114•Aug 5, 2022•0 citations

Universal Dynamical Control of Open Quantum Systems

Gershon Kurizki

Due to increasing demands on speed and security of data processing, along with requirements on measurement precision in fundamental research, quantum phenomena are expected to play an increasing role in future technologies. Special attention must hence be paid to omnipresent decoherence effects, which hamper quantumness. Their consequence is always a deviation of the quantum state evolution (error) with respect to the expected unitary evolution if these effects are absent. In operational tasks such as the preparation, transformation, transmission, and detection of quantum states, these effects are detrimental and must be suppressed by strategies known as dynamical decoupling, or the more general dynamical control by modulation developed by us. The underlying dynamics must be Zeno-like, yielding suppressed coupling to the bath. There are, however, tasks which cannot be implemented by unitary evolution, in particular those involving a change of the system’s state entropy. Such tasks necessitate efficient coupling to a bath for their implementation. Examples include the use of measurements to cool (purify) a system, to equilibrate it, or to harvest and convert energy from the environment. If the underlying dynamics is anti-Zeno like, enhancement of this coupling to the bath will occur and thereby facilitate the task, as discovered by us. A general task may also require state and energy transfer, or entanglement of noninteracting parties via shared modes of the bath which call for maximizing the shared (two-partite) couplings with the bath, but suppressing the single-partite couplings. For such tasks, a more subtle interplay of Zeno and anti-Zeno dynamics may be optimal. We have therefore constructed a general framework for optimizing the way a system interacts with its environment to achieve a desired task. This optimization consists in adjusting a given “score” that quantifies the success of the task, such as the targeted fidelity, purity, entropy, entanglement, or energy by dynamical modification of the system-bath coupling spectrum on demand.

ISRN Optics•Sep 19, 2013•8 citations

Quantum control theory for coherence and information dynamics

Lorenza Viola, David J. Tannor

Precisely characterizing and controlling the dynamics of realistic open quantum systems has emerged in recent years as a key challenge across contemporary quantum sciences and technologies, with implications ranging from physics, chemistry and applied mathematics to quantum information processing (QIP) and quantum engineering. Quantum control theory aims to provide both a general dynamical-system framework and a constructive toolbox to meet this challenge. The purpose of this special issue of Journal of Physics B: Atomic, Molecular and Optical Physics is to present a state-of-the-art account of recent advances and current trends in the field, as reflected in two international meetings that were held on the subject over the last summer and which motivated in part the compilation of this volume—the Topical Group: Frontiers in Open Quantum Systems and Quantum Control Theory , held at the Institute for Theoretical Atomic, Molecular and Optical Physics (ITAMP) in Cambridge, Massachusetts (USA), from 1–14 August 2010, and the Safed Workshop on Quantum Decoherence and Thermodynamics Control , held in Safed (Israel), from 22–27 August 2010. Initial developments in quantum control theory date back to (at least) the early 1980s, and have been largely inspired by the well-established mathematical framework for classical dynamical systems. As the above-mentioned meetings made clear, and as the burgeoning body of literature on the subject testifies, quantum control has grown since then well beyond its original boundaries, and has by now evolved into a highly cross-disciplinary field which, while still fast-moving, is also entering a new phase of maturity, sophistication, and integration. Two trends deserve special attention: on the one hand, a growing emphasis on control tasks and methodologies that are specifically motivated by QIP, in addition and in parallel to applications in more traditional areas where quantum coherence is nevertheless vital (such as, for instance, quantum control of chemical reactions or high-resolution magnetic resonance spectroscopy); on the other hand, an unprecedented demand for close coupling between theory and experiment , with theoretical developments becoming more and more attuned to and driven by experimental advances as different quantum technologies continue to evolve at an impressive pace in the laboratory. Altogether, these two trends account for several of the recurrent themes in this volume, as well as in the current quantum control literature as a whole: namely, the quest for control strategies that can attain the highest degree of precision and robustness possible, while striving for efficiency and, ultimately, optimality in achieving the intended control task under realistic operational constraints. From a theory standpoint, this makes it imperative to take into account increasingly more realistic control settings; to assess the quantitative impact of limited control resources and/or system knowledge; and to provide a rigorous and general foundation for existing experimental approaches in order to further enhance applicability and performance. From an experimental standpoint, renewed emphasis is in turn placed on validating theoretical predictions and benchmarking performance, so that the limiting constraints can be singled out for additional theoretical analysis and guidance. This ongoing cross-talk is clearly reflected in this collection, which brings together theoreticians and experimentalists, with a significant fraction of the papers reporting on combined quantum control theory–experiment efforts. While a precise categorization would neither be possible nor desirable, contributions to this volume have been loosely grouped into five broad sections. This grouping has been made in the hope that connections between different problems and/or technical approaches will become more transparent, facilitating the transfer of concepts and methods. The special issue opens with a section devoted to open-loop control methods, with special emphasis on dynamical decoupling (DD), which is becoming an increasingly important tool for decoherence control at the physical 'quantum firmware' level. In addition to including original research results, the first two articles, by Brion et al and Biercuk et al , also serve to pedagogically review some background in their respective subjects. In particular, Brion et al revisit one of the conceptually simplest approaches to open-loop manipulation of both closed and open quantum systems, nonholonomic control , motivated by its broad applicability to QIP settings. A special instance of open-loop control based on sequences of (nearly) instantaneous `bang-bang' pulses is addressed by Biercuk et al , who reformulate the simplest DD scenario, suppression of phase decoherence in a single qubit, as a filter-design problem. Peng et al report on the implementation of 'concatenated' DD for arbitrary single-qubit decoherence in the context of nuclear magnetic resonance QIP. A dedicated analysis of the performance of different DD schemes in the presence of realistic pulse errors is given by Wang and Dobrovitski. DD is also one of the strategies used by Lucamarini et al to reduce polarization decoherence in a photon qubit. These authors additionally report on the use of active feedback to counter transmission noise, effectively setting the stage for the second section, which is centered on closed-loop control. Unlike in open-loop control, measurement is an essential ingredient in closed-loop schemes aimed at both reliably identifying features of the target quantum system and further modifying its dynamics. The importance of directly measuring the spectrum of the underlying system-environment coupling is stressed by Almog et al , who show how this knowledge is crucial, in particular, for predicting the performance of DD sequences in experiments and for optimizing performance. Riofrio et al address a weak-measurement protocol for implementing quantum state tomography , which is a necessary 'primitive' for inferring the target quantum state and thereby diagnosing the control performance. Next, the impact of realistic control and system imperfections in continuous-time Markovian feedback strategies for rapid state preparation is analyzed by Combes and Wiseman. A prominent role is played in the special issue by optimal control (OC) approaches, reflecting their central importance for quantum control and QIP. The OC contributions have been divided into two separate sections, depending on whether the target dynamics is modeled as Hamiltonian (section 3) or dissipative (section 4), respectively. The contribution by Beltrani et al deals with `control landscapes', which provide a foundation for analyzing the performance of numerical OC algorithms and their robustness against control errors. Specifically, this paper characterizes geometric properties of the control landscape, relevant to the optimal control of state-to-state transitions. Application of OC theory to the problem of population transfer and coherence enhancement in Λ-systems is studied by Kumar et al , whereas Goerz et al report on the OC-design of a high-fidelity controlled phase-gate in atomic qubits. The robustness of an OC solution is specifically addressed by Negretti et al , along with an approach for identifying easily implementable while still 'close-to-optimal' control pulses. Powerful relaxation-optimized OC schemes (based on so-called opengrape algorithms) for generating unitary target gates in the presence of known dissipation parameters are discussed by Schulte-Herbrüggen et al . Next, Lapert et al report on the problem of time-optimal control of spin-1/2 systems undergoing Bloch relaxation dynamics, highlighting the crucial role played by singular extremals in the control synthesis. Alternative approaches for optimized control of qubits exposed to various decoherence processes are developed by Esher et al and Xue et al , based on a perturbative 'bath-optimized' formalism and on numerical optimization via a genetic algorithm, respectively. Testifying to the richness of the field, the volume concludes with four contributions that address a diverse range of problems. The exploitation of properties of adiabatic quantum evolutions is common to the first two papers. In particular, Legthtas et al offer a rigorous explanation for the robustness of a control protocol, chirped pulsing , that is widely employed in 'adiabatic rapid passage' experiments, while Han et al present a theoretical framework for adiabatic Raman photo-association schemes relevant to ultracold atomic systems. In the context of cavity quantum electrodynamics, Montenegro and Orszag describe how to engineer a system of two atoms coupled to distant lossy cavities so that stable atomic entanglement is generated. Finally, still very little is known about the physical mechanisms that are responsible for and control the experimentally observed 'coherent' features of transport phenomena in biological systems. The last contribution by Alicki and Giraldi analyzes energy transport in dynamical systems that can be modeled as 'quantum networks', and points to this fascinating emerging frontier. It is our hope that the above papers may help readers to gain an overview of some of the main trends in current quantum control efforts, both theoretical and experimental. In closing, we take the opportunity to thank the organizations which sponsored the above-mentioned ITAMP Topical Group (the United States National Science Foundation and Harvard University) and the Safed Workshop (the Israeli Science Foundation, the Safed Scientific Workshop program, CECAM and ACAM). Last but not least our sincere gratitude goes to all of the contributors to the volume and the reviewers as well as the J. Phys. B staff, for their respective efforts in preparing the papers and ensuring the overall quality of this special issue.

Journal of Physics B Atomic Molecular and Optical Physics•Jul 25, 2011•6 citations
Control of open quantum systems is essential for the realization of contemporary quantum science and technology. We demonstrate such control using a thermodynamically consistent framework, taking into account the fact that the drive can modify the system's interaction with the environment. Such an effect is incorporated within the dynamical equation, leading to control-dependent dissipation. This relation serves as the key element for open-system control. The control paradigm is displayed by analyzing entropy-changing state-to-state transformations, such as heating and cooling. The difficult task of controlling quantum gates is achieved for nonunitary reset maps with complete memory loss. In addition, we identify a mechanism for controlling unitary gates by actively removing entropy from the system to the environment. We demonstrate a universal set of single- and double-qubit unitary gates under dissipation.
Control of open quantum systems is an essential ingredient to the realization of contemporary quantum science and technology. We demonstrate such control by employing a thermodynamically consistent framework, taking into account the fact that the drive can modify the interaction with environment. Such an effect is incorporated within the dynamical equation, leading to control dependent dissipation, this relation serves as the key element for open system control. Thermodynamics of the control process is reflected by a unidirectional flow of energy to the environment resulting in large entropy production. The control paradigm is displayed by analyzing entropy changing state to state transformations, such as heating and cooling. In addition, the generation of quantum gates under dissipative conditions is demonstrated for both non-unitary reset maps with complete memory loss and a universal set of single and double qubit unitary gates.
Quantum control of an open system is demonstrated employing a thermodynamically consistent master equation. In this framework, the open system dynamics depend on the control protocol due to the dressing of the system by the drive. This interrelation serves as the key element for control. The influence of the external drive is incorporated within the dynamical equation, enabling an indirect control of the dissipation. The control paradigm is displayed by analyzing entropy changing state to state transformations, heating and cooling N-level systems. Following, we study the generation of quantum non-unitary maps via coherent control. These include both reset maps with complete memory loss and single-qubit unitary maps under dissipative conditions.
All physical quantum systems are in contact with the external world which is inevitably a source of noise. It is therefore necessary to take into account this dissipation when designing controls that accomplish useful tasks in quantum information processing. This thesis is on that overlap of open quantum systems and control theory; it looks at what dynamics can happen with the use of external driving, and how this driving can be chosen to accomplish a desired goal. The first result looks at how a given quantum dissipator can be manipulated, using coherent controls, into replicating the action of a different type of noise. This results in no-go theorems for how noise can be transformed based on its isotropy, with applications in simulating open systems. Another way of doing simulations is to use only unitary dynamics over the system and a finite dimensional ancilla, and it is proved that there always exists a dilation Hamiltonian that replicates the noisy dynamics continuously in time. This also highlights the fact that adding controls on noise can result in a different evolution than if the controls were done on the under- lying system-environment level. A conjecture is introduced and studied which states that both approaches are equivalent in the special case of the controls commuting with the Lindbladian. A way around this difficulty is to use a quantum system to compute in situ which controls are best for achieving a desired task on itself. This problem is studied in the context of reaching entangling gates on a quantum simulator in order to upgrade it into a quantum computer. The experimental cost of doing so is found to be polynomial in the number of qubits in simulations. The same underlying principle is also used to find error correcting codes tailored to the dissipation in a system.
We apply the Krotov method for open and closed quantum systems with the objective of finding optimized controls to manipulate qubit/qutrit systems in the presence of the external environment. In the case of unitary optimization, the Krotov method is first applied to a quantum system neglecting its interaction with the environment. The resulting controls from the unitary optimization are then used to drive the system along with the environmental noise. In the case of non-unitary optimization, the Krotov method already takes into account the noise during the optimization process. We consider two distinct computational task: target-state preparation and quantum gate implementation. These tasks are carried out in simple qubit/qutrit systems and also in systems presenting leakage states. For the state-preparation cases, the controls from the non-unitary optimization outperform the controls from the unitary optimization. However, as we show here, this is not always true for the implementation of quantum gates. There are some situations where the unitary optimization performs equally well compared to the non-unitary optimization. We verify that these situations corresponds to either the absence of leakage states or to the effects of dissipation being spread uniformly over the system, including non-computational levels. For such cases, the quantum gate implementation must cover the entire Hilbert space and there is no way to dodge dissipation. On the other hand, if the subspace containing the computational levels and its complement are differently affected by dissipation, the non-unitary optimization becomes effective.
Due to increasing demands on speed and security of data processing, along with requirements on measurement precision in fundamental research, quantum phenomena are expected to play an increasing role in future technologies. Special attention must hence be paid to omnipresent decoherence effects, which hamper quantumness. Their consequence is always a deviation of the quantum state evolution (error) with respect to the expected unitary evolution if these effects are absent. In operational tasks such as the preparation, transformation, transmission, and detection of quantum states, these effects are detrimental and must be suppressed by strategies known as dynamical decoupling, or the more general dynamical control by modulation developed by us. The underlying dynamics must be Zeno-like, yielding suppressed coupling to the bath. There are, however, tasks which cannot be implemented by unitary evolution, in particular those involving a change of the system’s state entropy. Such tasks necessitate efficient coupling to a bath for their implementation. Examples include the use of measurements to cool (purify) a system, to equilibrate it, or to harvest and convert energy from the environment. If the underlying dynamics is anti-Zeno like, enhancement of this coupling to the bath will occur and thereby facilitate the task, as discovered by us. A general task may also require state and energy transfer, or entanglement of noninteracting parties via shared modes of the bath which call for maximizing the shared (two-partite) couplings with the bath, but suppressing the single-partite couplings. For such tasks, a more subtle interplay of Zeno and anti-Zeno dynamics may be optimal. We have therefore constructed a general framework for optimizing the way a system interacts with its environment to achieve a desired task. This optimization consists in adjusting a given “score” that quantifies the success of the task, such as the targeted fidelity, purity, entropy, entanglement, or energy by dynamical modification of the system-bath coupling spectrum on demand.
Precisely characterizing and controlling the dynamics of realistic open quantum systems has emerged in recent years as a key challenge across contemporary quantum sciences and technologies, with implications ranging from physics, chemistry and applied mathematics to quantum information processing (QIP) and quantum engineering. Quantum control theory aims to provide both a general dynamical-system framework and a constructive toolbox to meet this challenge. The purpose of this special issue of Journal of Physics B: Atomic, Molecular and Optical Physics is to present a state-of-the-art account of recent advances and current trends in the field, as reflected in two international meetings that were held on the subject over the last summer and which motivated in part the compilation of this volume—the Topical Group: Frontiers in Open Quantum Systems and Quantum Control Theory , held at the Institute for Theoretical Atomic, Molecular and Optical Physics (ITAMP) in Cambridge, Massachusetts (USA), from 1–14 August 2010, and the Safed Workshop on Quantum Decoherence and Thermodynamics Control , held in Safed (Israel), from 22–27 August 2010. Initial developments in quantum control theory date back to (at least) the early 1980s, and have been largely inspired by the well-established mathematical framework for classical dynamical systems. As the above-mentioned meetings made clear, and as the burgeoning body of literature on the subject testifies, quantum control has grown since then well beyond its original boundaries, and has by now evolved into a highly cross-disciplinary field which, while still fast-moving, is also entering a new phase of maturity, sophistication, and integration. Two trends deserve special attention: on the one hand, a growing emphasis on control tasks and methodologies that are specifically motivated by QIP, in addition and in parallel to applications in more traditional areas where quantum coherence is nevertheless vital (such as, for instance, quantum control of chemical reactions or high-resolution magnetic resonance spectroscopy); on the other hand, an unprecedented demand for close coupling between theory and experiment , with theoretical developments becoming more and more attuned to and driven by experimental advances as different quantum technologies continue to evolve at an impressive pace in the laboratory. Altogether, these two trends account for several of the recurrent themes in this volume, as well as in the current quantum control literature as a whole: namely, the quest for control strategies that can attain the highest degree of precision and robustness possible, while striving for efficiency and, ultimately, optimality in achieving the intended control task under realistic operational constraints. From a theory standpoint, this makes it imperative to take into account increasingly more realistic control settings; to assess the quantitative impact of limited control resources and/or system knowledge; and to provide a rigorous and general foundation for existing experimental approaches in order to further enhance applicability and performance. From an experimental standpoint, renewed emphasis is in turn placed on validating theoretical predictions and benchmarking performance, so that the limiting constraints can be singled out for additional theoretical analysis and guidance. This ongoing cross-talk is clearly reflected in this collection, which brings together theoreticians and experimentalists, with a significant fraction of the papers reporting on combined quantum control theory–experiment efforts. While a precise categorization would neither be possible nor desirable, contributions to this volume have been loosely grouped into five broad sections. This grouping has been made in the hope that connections between different problems and/or technical approaches will become more transparent, facilitating the transfer of concepts and methods. The special issue opens with a section devoted to open-loop control methods, with special emphasis on dynamical decoupling (DD), which is becoming an increasingly important tool for decoherence control at the physical 'quantum firmware' level. In addition to including original research results, the first two articles, by Brion et al and Biercuk et al , also serve to pedagogically review some background in their respective subjects. In particular, Brion et al revisit one of the conceptually simplest approaches to open-loop manipulation of both closed and open quantum systems, nonholonomic control , motivated by its broad applicability to QIP settings. A special instance of open-loop control based on sequences of (nearly) instantaneous `bang-bang' pulses is addressed by Biercuk et al , who reformulate the simplest DD scenario, suppression of phase decoherence in a single qubit, as a filter-design problem. Peng et al report on the implementation of 'concatenated' DD for arbitrary single-qubit decoherence in the context of nuclear magnetic resonance QIP. A dedicated analysis of the performance of different DD schemes in the presence of realistic pulse errors is given by Wang and Dobrovitski. DD is also one of the strategies used by Lucamarini et al to reduce polarization decoherence in a photon qubit. These authors additionally report on the use of active feedback to counter transmission noise, effectively setting the stage for the second section, which is centered on closed-loop control. Unlike in open-loop control, measurement is an essential ingredient in closed-loop schemes aimed at both reliably identifying features of the target quantum system and further modifying its dynamics. The importance of directly measuring the spectrum of the underlying system-environment coupling is stressed by Almog et al , who show how this knowledge is crucial, in particular, for predicting the performance of DD sequences in experiments and for optimizing performance. Riofrio et al address a weak-measurement protocol for implementing quantum state tomography , which is a necessary 'primitive' for inferring the target quantum state and thereby diagnosing the control performance. Next, the impact of realistic control and system imperfections in continuous-time Markovian feedback strategies for rapid state preparation is analyzed by Combes and Wiseman. A prominent role is played in the special issue by optimal control (OC) approaches, reflecting their central importance for quantum control and QIP. The OC contributions have been divided into two separate sections, depending on whether the target dynamics is modeled as Hamiltonian (section 3) or dissipative (section 4), respectively. The contribution by Beltrani et al deals with `control landscapes', which provide a foundation for analyzing the performance of numerical OC algorithms and their robustness against control errors. Specifically, this paper characterizes geometric properties of the control landscape, relevant to the optimal control of state-to-state transitions. Application of OC theory to the problem of population transfer and coherence enhancement in Λ-systems is studied by Kumar et al , whereas Goerz et al report on the OC-design of a high-fidelity controlled phase-gate in atomic qubits. The robustness of an OC solution is specifically addressed by Negretti et al , along with an approach for identifying easily implementable while still 'close-to-optimal' control pulses. Powerful relaxation-optimized OC schemes (based on so-called opengrape algorithms) for generating unitary target gates in the presence of known dissipation parameters are discussed by Schulte-Herbrüggen et al . Next, Lapert et al report on the problem of time-optimal control of spin-1/2 systems undergoing Bloch relaxation dynamics, highlighting the crucial role played by singular extremals in the control synthesis. Alternative approaches for optimized control of qubits exposed to various decoherence processes are developed by Esher et al and Xue et al , based on a perturbative 'bath-optimized' formalism and on numerical optimization via a genetic algorithm, respectively. Testifying to the richness of the field, the volume concludes with four contributions that address a diverse range of problems. The exploitation of properties of adiabatic quantum evolutions is common to the first two papers. In particular, Legthtas et al offer a rigorous explanation for the robustness of a control protocol, chirped pulsing , that is widely employed in 'adiabatic rapid passage' experiments, while Han et al present a theoretical framework for adiabatic Raman photo-association schemes relevant to ultracold atomic systems. In the context of cavity quantum electrodynamics, Montenegro and Orszag describe how to engineer a system of two atoms coupled to distant lossy cavities so that stable atomic entanglement is generated. Finally, still very little is known about the physical mechanisms that are responsible for and control the experimentally observed 'coherent' features of transport phenomena in biological systems. The last contribution by Alicki and Giraldi analyzes energy transport in dynamical systems that can be modeled as 'quantum networks', and points to this fascinating emerging frontier. It is our hope that the above papers may help readers to gain an overview of some of the main trends in current quantum control efforts, both theoretical and experimental. In closing, we take the opportunity to thank the organizations which sponsored the above-mentioned ITAMP Topical Group (the United States National Science Foundation and Harvard University) and the Safed Workshop (the Israeli Science Foundation, the Safed Scientific Workshop program, CECAM and ACAM). Last but not least our sincere gratitude goes to all of the contributors to the volume and the reviewers as well as the J. Phys. B staff, for their respective efforts in preparing the papers and ensuring the overall quality of this special issue.