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Annalen der Physik

Spatially Structured Optical Effects in a Four‐Level Quantum System Near a Plasmonic Nanostructure

Hamid Reza Hamedi, Vassilios Yannopapas, Emmanuel Paspalakis

Published Jul 24, 2021• 16 citations
Publisher

Abstract

Abstract The light–matter interaction for a four‐level double‐V‐type quantum system interacting with a pair of weak probe fields while located near a 2D array of metal‐coated dielectric nanospheres is studied. A situation is considered in which one of the probe field carries an optical vortex, that is, an electromagnetic field with optical angular momentum, and the other probe field has no vortex. It is demonstrated that due to the phase sensitivity of the closed‐loop double V‐type quantum system, the linear and nonlinear susceptibility of the non‐vortex probe beam depends on the azimuthal angle and orbital angular momentum (OAM) of the vortex probe beam. This feature is missing in an open four‐level double V‐type quantum system interacting with free‐space vacuum, as no quantum interference occurs in this case. The azimuthal dependence of optical susceptibility of the quantum system is used to determine the regions of spatially structured transparency.

DOI
10.1002/andp.202100117

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Physical review. B./Physical review. B•May 11, 2017•39 citations
Abstract The light–matter interaction for a four‐level double‐V‐type quantum system interacting with a pair of weak probe fields while located near a 2D array of metal‐coated dielectric nanospheres is studied. A situation is considered in which one of the probe field carries an optical vortex, that is, an electromagnetic field with optical angular momentum, and the other probe field has no vortex. It is demonstrated that due to the phase sensitivity of the closed‐loop double V‐type quantum system, the linear and nonlinear susceptibility of the non‐vortex probe beam depends on the azimuthal angle and orbital angular momentum (OAM) of the vortex probe beam. This feature is missing in an open four‐level double V‐type quantum system interacting with free‐space vacuum, as no quantum interference occurs in this case. The azimuthal dependence of optical susceptibility of the quantum system is used to determine the regions of spatially structured transparency.
We investigate the nonlinear optical response of a four-level double-V-type quantum system interacting with a pair of weak probe fields while located near a two-dimensional array of metal-coated dielectric nanospheres. Such a quantum system contains a V-type subsystem interacting with surface plasmons, and another V-type subsystem interacting with the free-space vacuum. A distinctive feature of the proposed setup is its sensitivity to the relative phase of the applied fields when placed near the plasmonic nanostructure. We demonstrate that due to the presence of the plasmonic nanostructure, the third-order (Kerr-type) susceptibility for one of the laser fields can be significantly modified while another probe field is acting. Moreover, the Kerr nonlinearity of the system can be controlled and even enhanced by varying the distance of the quantum system from the plasmonic nanostructure.We also show that the Kerr nonlinearity of such a system can be controlled by adjusting the relative phase of the applied fields. The results obtained may find potential applications in on-chip nanoscale photonic devices. We also study the light-matter interaction in the case where one probe field carries an optical vortex, and another probe field has no vortex. We demonstrate that due to the phase sensitivity of the closed-loop double V-type quantum system, the linear and nonlinear susceptibility of the nonvortex probe beam depends on the azimuthal angle and orbital angular momentum (OAM) of the vortex probe beam. This feature is missing in open four-level double V-type quantum system interacting with free-space vacuum, as no quantum interference occurs in this case. We use the azimuthal dependence of optical susceptibility of the quantum system to determine the regions of spatially-structured transmittance.
We study theoretically the effects of a plasmonic nanostructure on the linear absorption and dispersion spectrum of a four-level double- V\mathsf{V}V-type quantum system. In the quantum system under study one V\mathsf{V}V-type transition is influenced by the interaction with surface plasmons while the other V\mathsf{V}V-type transition interacts with free-space vacuum. As plasmonic nanostructure we consider a two-dimensional array of metal-coated dielectric nanospheres. We analyze the optical properties of a linearly polarized laser field that couples the lowest state with the upper states in the free-space transitions. We show that, due to the presence of the plasmonic nanostructure, effects of optical transparency are created. These effects are also complemented by the existence of slow light.
Recently, the generation and detection of structured light field have drawn a great deal of attention, due to their importance in high-capacity optical data storage and quantum technology. In this letter, we explore the azimuthal modulation of optical transparency in a four-level double-V type quantum system near a plasmonic nanostructure. A Laguerre-Gaussian beam and the interaction of the system with free-space vacuum modes have been employed to create the phase-dependent absorption of a non-vortex probe field. First, we demonstrate how to identify the azimuthal index associated with the conventional LG beam via measuring the probe absorption so that the phase information of such a beam gets encoded on the spatially-dependent absorption profile with angularly-distributed lobes. Also, a spatially-varying optical transparency can be formed, due to the periodic variation of the absorption spectrum. Then, asymmetrical Laguerre-Gaussian beams are used to extend the selective spatial transparency mechanism to asymmetric spatially-structured windows, allowing for optical manipulation of spatial modes at arbitrary positions. Moreover, we investigate the influence of the asymmetric parameter on the features of the spatial inhomogeneities and show how the beams enable us to imprint the phase information of the orbital angular momentum at a desired position.
We present a theoretical study for the Kerr nonlinearity of a four-level double-V-type quantum system near a two-dimensional array of metal-coated dielectric nanospheres. In the quantum system under study one V-type transition is influenced by the interaction with surface plasmons while the other V-type transition interacts with free-space vacuum. The quantum system interacts with a linearly polarized weak laser field that couples the lowest state with the upper states in the free-space transitions. We show that the Kerr nonlinearity is strongly influenced by the presence of the plasmonic nanostructure and is particularly sensitive to the distance between the quantum system and the plasmonic nanostructure.
Abstract We present an azimuthal phase-dependent scheme to study the spatially dependent electromagnetically induced transparency (EIT) and the generation of spatial light in a closed-loop four-level Y-type system. A structured control beam and a microwave (MW) field are adopted in the closed-loop structure. Interestingly, the weak non-vortex probe beam responses explicitly depend on the orbital angular momentum (OAM) of the control beam along with the MW-assisted quantum interference. The regions of spatially dependent EIT are demonstrated at different azimuthal angles. It is found that the intensity of the structured control beam and the relative phase arising out of the beams participating in the closed-loop can be used as the controlling knobs to tailor the shape and the angular location of the spatially dependent EIT.
We study the optical response of a four-level double-V-type quantum system which interacts simultaneously with probe and pump laser fields and is located near a two-dimensional array of metal-coated dielectric nanospheres. By considering different coupling configurations for the pump/probe laser fields and analyzing the resulting probe absorption spectrum we reveal a variety of phenomena, such as huge enhancement of the absorption at the central line, gain without inversion, and a phase-dependent absorption spectrum. We also show that the enhancement of probe absorption or the gain can be controlled by varying the distance of the quantum system from the plasmonic nanostructure, the intensity of the pump field(s), and, when applicable, their relative phase. Our results can find applications in on-chip nanoscale photonic devices.