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Physical review. E

Subharmonics and superharmonics of the weak field in a driven two-level quantum system: Vibrational resonance enhancement

Prasun Sarkar, Shibashis Paul, Deb Shankar Ray

Published Jul 2, 2021• 8 citations
Publisher

Abstract

We consider a quantum two-level system in bichromatic classical time-periodic fields, the frequency of one of which far exceeds that of the other. Based on systematic separation of timescales and averaging over the fast motion a reduced quantum dynamics in the form of a nonlinear forced Mathieu equation is derived to identify the stable oscillatory resonance zones intercepted by unstable zones in the frequency-amplitude plot. We show how this forcing of the dressed two-level system may generate the subharmonics and superharmonics of the weak field in the stable region, which can be amplified by optimization of the strength of the high frequency field. We have carried out detailed numerical simulations of the driven quantum dynamics to corroborate the theoretical analysis.

DOI
10.1103/physreve.104.014202

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Physical Review A•Oct 1, 1993•110 citations
We consider a quantum two-level system in bichromatic classical time-periodic fields, the frequency of one of which far exceeds that of the other. Based on systematic separation of timescales and averaging over the fast motion a reduced quantum dynamics in the form of a nonlinear forced Mathieu equation is derived to identify the stable oscillatory resonance zones intercepted by unstable zones in the frequency-amplitude plot. We show how this forcing of the dressed two-level system may generate the subharmonics and superharmonics of the weak field in the stable region, which can be amplified by optimization of the strength of the high frequency field. We have carried out detailed numerical simulations of the driven quantum dynamics to corroborate the theoretical analysis.
We consider a two-level quantum system interacting with two classical time-periodic electromagnetic fields. The frequency of one of the fields far exceeds that of the other. The effect of the high-frequency field can be averaged out of the dynamics to realize an effective transition frequency of the field-dressed two-level system. We examine the linear response, second harmonic response and Stokes and anti-Stokes Raman response of the dressed two-level system, to the weak frequency field. The vibrational resonance enhancement in each case is demonstrated for optimal strength of the high-frequency field. Our theoretical scheme is corroborated by full numerical simulation of the two-level, two-field dynamics governed by loss-free Bloch equations. We suggest that quantum optics can offer an interesting arena for the study of the vibrational resonance. This article is part of the theme issue 'Vibrational and stochastic resonance in driven nonlinear systems (part 1)'.
Resonances of the six-wave mixing susceptibility χ(5)(ω1, ω1, ω1,-ω2,-ω2) at frequency 3ω1-2ω2 of a system of two-level atoms dissipating through the spontaneous emission and collisions and driven by a weak bichromatic external field of frequencies ω1 and ω2 in a finite Q cavity are analyzed. It is shown that the atomic collisions not only induce the usual Bloembergen resonances but that they also play a major role in enhancing the transitions among the higher-order dressed states, thereby bringing out some of the quantum resonances that are suppressed in the absence of collisions. The important contribution of collisions in this higher-order nonlinear process is the generation of the subharmonic resonances at ±1/2 times the hyperfine splitting of the first and the second excited manifolds.
We study the behavior of a two-level atom that is driven by a bichromatic field consisting of a strong resonant component and a weaker tunable component. In addition to the splitting of the energy levels (the multiphoton AC Stark effect), we find that the weaker component also shifts the subharmonic resonances, an effect we attribute to a dynamic Stark shift. When the weaker component is tuned to a shifted resonance, no fluorescence occurs at either the frequency of the strong component or the three-photon mixing frequency. Results are obtained with numerical techniques and explained in terms of the dressed-atom model of the system.
The quantum trajectories method is illustrated for the resonance fluorescence of a two-level atom driven by a multichromatic field. We discuss the method for the time evolution of the fluorescence intensity in the presence of bichromatic and trichromatic driving fields. We consider the special case wherein one multichromatic field component is strong and resonant with the atomic transition whereas the other components are much weaker and arbitrarily detuned from the atomic resonance. We find that the phase-dependent modulations of the Rabi oscillations, recently observed experimentally [Q. Wu, D. J. Gauthier, and T. W. Mossberg, Phys. Rev. A 49, R1519 (1994)] for the special case when the weaker component of a bichromatic driving field is detuned from the atomic resonance by the strong-field Rabi frequency, appear also for detunings close to the subharmonics of the Rabi frequency. Furthermore, we show that for the atom initially prepared in one of the dressed states of the strong field component the modulations are not sensitive to the phase. We extend the calculations to the case of a trichromatic driving field and find that apart from the modulations of the amplitude there is a modulation of the frequency of the Rabi oscillations. Moreover, the time evolution of the fluorescence intensity depends on the phase regardless of the initial conditions and a phase-dependent suppression of the Rabi oscillations can be observed when the sideband fields are tuned to the subharmonics of the strong-field Rabi frequency.
We have studied the transient response of undamped two-level atoms to excitation by a classical bichromatic field consisting of a strong resonant component and a moderate-strength, tunable, ``perturber'' component. It is found that the strong field tends to stabilize the atom against the influence of the perturber field. Exceptions to this general result occur when the perturber is detuned from the strong field by the Rabi frequency of the latter or its subharmonics. We believe this stabilization phenomenon is a semiclassical analog of the effect that leads to the dynamical modification of spontaneous emission [M. Lewenstein and T. W. Mossberg, Phys. Rev. Lett. 59, 775 (1987)], and the presence of detunings at which the stabilization fails provides a simple motivation for the Rabi subharmonic resonances found in certain cw bichromatic spectra. Interestingly, when the perturber field is relatively weak, detuned from the atomic resonance by the strong-field Rabi frequency, and turned on with a specific initial phase relative to the strong field, one finds that the bichromatic field can be employed to dressed-state polarize initially ground-state atoms. In a related vein, we find that perturbations at the subharmonic detunings lead to interesting phase-dependent atomic dynamics. Results were obtained using both numerical and approximate analytical techniques entirely within the context of the rotating-wave approximation. The validity of the latter is ensured by demanding that all detunings and Rabi frequencies are vanishingly small compared to the atomic transition frequency.
We examine the radiative properties of a two-level atom driven by a strong bichromatic field with frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$=${\mathrm{\ensuremath{\omega}}}_{0}$-${\mathrm{\ensuremath{\delta}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{2}$=${\mathrm{\ensuremath{\omega}}}_{0}$+${\mathrm{\ensuremath{\delta}}}_{2}$, which can be asymmetrically placed about the atomic transition frequency ${\mathrm{\ensuremath{\omega}}}_{0}$ and can have different Rabi frequencies ${\mathrm{\ensuremath{\Omega}}}_{1}$ and ${\mathrm{\ensuremath{\Omega}}}_{2}$. Applying the optical Bloch equations for the bichromatic excitation, we derive an infinite set of equations of motion for the time evolution of the atomic variables. The equations are solved numerically by matrix inversion and Laplace transforms. Using the quantum regression theorem, we then solve for the steady-state total fluorescence intensity, and the resonance-fluorescence and absorption spectra. The spectra are found to depend on the frequency difference 2\ensuremath{\delta}=${\mathrm{\ensuremath{\delta}}}_{1}$+${\mathrm{\ensuremath{\delta}}}_{2}$, the average detuning \ensuremath{\Delta}=${\mathrm{\ensuremath{\omega}}}_{0}$-1/2(${\mathrm{\ensuremath{\omega}}}_{1}$+${\mathrm{\ensuremath{\omega}}}_{2}$), and the Rabi frequencies of the driving fields. For ${\mathrm{\ensuremath{\Omega}}}_{1}$=${\mathrm{\ensuremath{\Omega}}}_{2}$=\ensuremath{\Omega}, the total fluorescent intensity displays a series of maxima for \ensuremath{\Delta}=\ifmmode\pm\else\textpm\fi{}n\ensuremath{\delta}\ensuremath{\mp}${\mathrm{\ensuremath{\Omega}}}^{2}$/4\ensuremath{\delta}, where the n are the odd integers. The intensity-dependent shift from the resonances n\ensuremath{\delta} is explained as an analog of the generalized Bloch-Siegert shift. The resonance-fluorescence spectrum for \ensuremath{\Delta}\ensuremath{\ne}0 appears to contain more peaks than that for \ensuremath{\Delta}=0.This is due to the splitting of the central peak and the even sidebands into doublets. The absorption spectrum of a weak-probe beam for \ensuremath{\Delta}=0 and equal Rabi frequencies consists of a symmetric series of dispersionlike sidebands separated from ${\mathrm{\ensuremath{\omega}}}_{0}$ by integer multiples of \ensuremath{\delta}, together with a central absorption peak at ${\mathrm{\ensuremath{\omega}}}_{0}$, whose amplitude oscillates with \ensuremath{\Omega}. For \ensuremath{\Delta}\ensuremath{\ne}0 and/or ${\mathrm{\ensuremath{\Omega}}}_{1}$\ensuremath{\ne}${\mathrm{\ensuremath{\Omega}}}_{2}$, the odd sidebands remain dispersionlike, while the central peak and the even sidebands split into absorption-emission doublets. A simple physical interpretation of the spectral features is given in terms of the dressed-atom model.