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Zhurnal Eksperimentalnoi i Teoreticheskoi Fiziki

Resonance effects in the interaction between a two-level system and intense polychromatic radiation

O. A. Kocharovskaia, Ia. I. Khanin, V. B. Tsaregradskii

Published Feb 1, 1984• 0 citations
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Fluorescence by a polar quantum system in a polychromatic field

Jr. Bogolyubov, Andrey Vladimirovich Soldatov

Spectral properties of fluorescent radiation from a two-level quantum system with broken inversion spatial symmetry, which can be described by a model of an one-electron two-level atom whose electric dipole moment operator has permanent unequal diagonal matrix elements, were studied. The case of the excitation of this system by a polychromatic laser field, comprised of $N-1$ high-frequency components with the frequencies close to or being in resonance with the atomic transition frequency, and a low-frequency component whose frequency coincides with the Rabi frequency of the high-frequency components, was considered. Special attention was given to the resonant bichromatic and nearly resonant trichromatic excitation. In the former case it was shown that by changing the intensity of the low-frequency component, one can efficiently alter spectral properties of the fluorescent radiation of the system in the high-frequency range, while in the latter case it was found that the fluorescent behavior of the system in question reveals a kind of an optoelectronic transistor effect. Options for the experimental detection and practical usage of the effects under study were discussed.

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Spectroscopy of a resonance medium based on the use of nonlinear absorption of strong polychromatic radiation with equidistant spectrum

G. I. Toptygina, Evald E. Fradkin

Let us consider preliminary two situations. In the first of them the monochromatic radiation is absorbing. The increase of its intensity leads to the diminution of an absorption down to zero in a limiting case, i.e. to the effect of saturated absorption. In the second case an absorption of test radiation with a small intensity is observing, while two—level atom is strongly interacting with a perturbing field. This case is characterized by asymmetric dependence of absorption on the frequency difference w- w = A, where w and w are the frequencies of two light waves. As it was shown by Rautian and Sobelman in 19611, the amplification of test radiation arises in a certain range of frequency offsets A instead of the absorption, and the energy transfers from a strong wave to a weak one. In this paper we study the problem which appears from the above situation, when the intensity of test radiation increases. Such an increase leads to new maxima in absorption spectra of test radiation at frequencies A = i n = 2, 3 4 . . . which are additional to the main maxima at n R A = where R the Rabi frequency. These new resonances were observed by Bonch-Bruevich, Vartanyan, and Chigir in 19792 and cal led the subradiat ive structure. We have the following simple approximate expression for R obtained in the case of interaction with two fields: Q =d(?+E2)1"2/h. (1) R 0 1 There are two essential effects in the described situation: the saturation of absorption and the nonlinear interference effect. The last causes the redistribution of an absorbed energy between radiation components, the negative absorption (amplification) without population inversion, and the multiphoton parametric resonances at difference frequencies. The laser generation on the base7of the negative absorption without population inversion was obtained in 1989. The following problems arise from the facts reviewed above: 1. The calculation of absorption coefficients for individual components of a strong polychromatic radiation with an equidistant spectrum. 2. Determining of a generalized Rabi frequency and verification of the simple formula A = In for maxima of resonances. n R The aim of this paper is to solve these problems.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Jul 1, 1992•1 citation

OPTICAL PROPERTIES OF TWO-LEVEL MEDIA EXCITED BY AN INTENSE POLYCHROMATIC FIELD

V. Alekseev, Yu. A. Zinin, E. D. Kholodkevich

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Laser-induced collective interactions under propagation of polychromatic radiation pulse through resonant optically dense extended medium without population inversion

Sergei N Bagayev, V. S. Egorov, Igor B. Mekhov +5 more

Experimental and theoretical investigation of the coherent propagation and amplification of polychromatic broadband laser pulses in optically dense resonant media without population inversion was carried out for the cases of plasma in a Ne glow discharge and a pulse discharge in Hg-Ar mixture. High density of Ne and Hg atoms in the metastable state (about 1012 cm-3), which was chosen to be the ground state of the two-level system under consideration, leads to the collective behavior of the atomic system in resonant electromagnetic field. The broadband probe field attenuation and the sideband amplification of the probe under the action of the coherent pump were observed. The amplification dependence on the pump intensity was obtained. The model of the parametrically enhanced collective interactions was developed and comparison the experimental data was made.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•May 30, 2002•1 citation
Spectral properties of fluorescent radiation from a two-level quantum system with broken inversion spatial symmetry, which can be described by a model of an one-electron two-level atom whose electric dipole moment operator has permanent unequal diagonal matrix elements, were studied. The case of the excitation of this system by a polychromatic laser field, comprised of N−1N-1N−1 high-frequency components with the frequencies close to or being in resonance with the atomic transition frequency, and a low-frequency component whose frequency coincides with the Rabi frequency of the high-frequency components, was considered. Special attention was given to the resonant bichromatic and nearly resonant trichromatic excitation. In the former case it was shown that by changing the intensity of the low-frequency component, one can efficiently alter spectral properties of the fluorescent radiation of the system in the high-frequency range, while in the latter case it was found that the fluorescent behavior of the system in question reveals a kind of an optoelectronic transistor effect. Options for the experimental detection and practical usage of the effects under study were discussed.
Let us consider preliminary two situations. In the first of them the monochromatic radiation is absorbing. The increase of its intensity leads to the diminution of an absorption down to zero in a limiting case, i.e. to the effect of saturated absorption. In the second case an absorption of test radiation with a small intensity is observing, while two—level atom is strongly interacting with a perturbing field. This case is characterized by asymmetric dependence of absorption on the frequency difference w- w = A, where w and w are the frequencies of two light waves. As it was shown by Rautian and Sobelman in 19611, the amplification of test radiation arises in a certain range of frequency offsets A instead of the absorption, and the energy transfers from a strong wave to a weak one. In this paper we study the problem which appears from the above situation, when the intensity of test radiation increases. Such an increase leads to new maxima in absorption spectra of test radiation at frequencies A = i n = 2, 3 4 . . . which are additional to the main maxima at n R A = where R the Rabi frequency. These new resonances were observed by Bonch-Bruevich, Vartanyan, and Chigir in 19792 and cal led the subradiat ive structure. We have the following simple approximate expression for R obtained in the case of interaction with two fields: Q =d(?+E2)1"2/h. (1) R 0 1 There are two essential effects in the described situation: the saturation of absorption and the nonlinear interference effect. The last causes the redistribution of an absorbed energy between radiation components, the negative absorption (amplification) without population inversion, and the multiphoton parametric resonances at difference frequencies. The laser generation on the base7of the negative absorption without population inversion was obtained in 1989. The following problems arise from the facts reviewed above: 1. The calculation of absorption coefficients for individual components of a strong polychromatic radiation with an equidistant spectrum. 2. Determining of a generalized Rabi frequency and verification of the simple formula A = In for maxima of resonances. n R The aim of this paper is to solve these problems.
Experimental and theoretical investigation of the coherent propagation and amplification of polychromatic broadband laser pulses in optically dense resonant media without population inversion was carried out for the cases of plasma in a Ne glow discharge and a pulse discharge in Hg-Ar mixture. High density of Ne and Hg atoms in the metastable state (about 1012 cm-3), which was chosen to be the ground state of the two-level system under consideration, leads to the collective behavior of the atomic system in resonant electromagnetic field. The broadband probe field attenuation and the sideband amplification of the probe under the action of the coherent pump were observed. The amplification dependence on the pump intensity was obtained. The model of the parametrically enhanced collective interactions was developed and comparison the experimental data was made.