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Bulletin of the American Physical Society

Quantum information processing with high-density diamond nitrogen-vacancy centers in strain and magnetic fields.

Zhujing Xu, Zhang‐qi Yin, Qinkai Han, Tongcang Li

Published Mar 16, 2021• 0 citations
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Coherent population trapping at zero magnetic field was observed for nitrogen-vacancy centers in diamond under optical excitation. This was measured as a reduction in photoluminescence when the detuning between two excitation lasers matched the 2.88 GHz crystal-field splitting of the color center ground states. This behavior is highly sensitive to strain, which modifies the excited states, and was unexpected following recent experiments demonstrating optical readout of single nitrogen-vacancy electron spins based on cycling transitions. These results demonstrate for the first time that three-level Lambda configurations suitable for proposed quantum information applications can be realized simultaneously for all four orientations of nitrogen-vacancy centers at zero magnetic field.
Laser-written optical waveguides in diamonds are a key technology to enhance coupling between defect centers and light, boosting applications in nanoscale sensing and quantum information processing. However, laser writing of photonic structures produces strain in the diamond lattice, modifying the properties of defect centers in poorly understood ways. This study demonstrates that optically detected magnetic resonance spectroscopy provides sufficient information to fully characterize the spatial distribution of strain in such a device, even without a constant magnetic field. The work yields an accessible tool that could be very useful for advancing diamond-based quantum technologies.