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Spontaneous atomic crystallization via diffractive dephasing in optical cavities

T. Ackemann, Costa Boquete, Adrian, Baio, Giuseppe, Robb, Gordon, Oppo, Gian-Luca, Griffin, Paul

Published Jun 4, 2021• 2 citations
OpenAlex

Abstract

The design of an experiment on the spontaneous crystallization of a laser-cooled, but thermal atomic cloud into a hexagonally structured phase is discussed. Atomic interaction is mediated by the dipole potential of an optical lattice formed spontaneously in a multi-mode degenerate cavity from single-mode longitudinal pumping. The length scale of the structure is given by the diffractive dephasing between the spontaneous sidebands and the on-axis pump. A linear stability indicates that the transition can be observed in a cavity of moderate finesse compatible with having the cavity mirrors outside the vacuum cell. A new anti-reflection coated cell has been assembled for this purpose.

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Spontaneous atomic crystallization via diffractive dephasing in optical cavities

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Abstract The design of an experiment on the spontaneous crystallization of a laser-cooled, but thermal atomic cloud into a hexagonally structured phase is discussed. Atomic interaction is mediated by the dipole potential of an optical lattice formed spontaneously in a multi-mode degenerate cavity from single-mode longitudinal pumping. The length scale of the structure is given by the diffractive dephasing between the spontaneous sidebands and the on-axis pump. A linear stability indicates that the transition can be observed in a cavity of moderate finesse compatible with having the cavity mirrors outside the vacuum cell. A new anti-reflection coated cell has been assembled for this purpose.

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Self-structuring via symmetry breaking is a prominent collective phenomenon occurring in cold and ultracold atoms coupled to optical fields [1] . Experimental realizations by means of trapped dipolar gases and optical cavities have shed light onto supersolidity and crystallization in out-of-equilibrium atomic systems [2] , [3] . Recent work demonstrated the occurrence of structural phase transitions between hexagonally coordinated supersolid phases in dipolar condensates [4] . In this work, we address 2D structural transitions occurring in an ensemble of cold thermal atoms with effective optomechanical interactions mediated by a coherent beam retro-reflected by means of a feedback mirror. The feedback loop scheme is represented in Fig. 1(a) , where the dipole potential induces atomic density structures which, in turn, scatter photons into side-band modes enhancing the potential itself and leading to transverse light-atom self-structuring, sharing similarities with an effective-Kerr nonlinear medium [5] .

Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)•Jun 21, 2021•0 citations
The design of an experiment on the spontaneous crystallization of a laser-cooled, but thermal atomic cloud into a hexagonally structured phase is discussed. Atomic interaction is mediated by the dipole potential of an optical lattice formed spontaneously in a multi-mode degenerate cavity from single-mode longitudinal pumping. The length scale of the structure is given by the diffractive dephasing between the spontaneous sidebands and the on-axis pump. A linear stability indicates that the transition can be observed in a cavity of moderate finesse compatible with having the cavity mirrors outside the vacuum cell. A new anti-reflection coated cell has been assembled for this purpose.
Abstract The design of an experiment on the spontaneous crystallization of a laser-cooled, but thermal atomic cloud into a hexagonally structured phase is discussed. Atomic interaction is mediated by the dipole potential of an optical lattice formed spontaneously in a multi-mode degenerate cavity from single-mode longitudinal pumping. The length scale of the structure is given by the diffractive dephasing between the spontaneous sidebands and the on-axis pump. A linear stability indicates that the transition can be observed in a cavity of moderate finesse compatible with having the cavity mirrors outside the vacuum cell. A new anti-reflection coated cell has been assembled for this purpose.
This article discusses self-organization in cold atoms via light-mediated interactions induced by feedback from a single retro-reflecting mirror. Diffractive dephasing between the pump beam and the spontaneous sidebands selects the lattice period. Spontaneous breaking of the rotational and translational symmetry occur in the 2D plane transverse to the pump. We elucidate how diffractive ripples couple sites on the self-induced atomic lattice. The nonlinear phase shift of the atomic cloud imprinted onto the optical beam is the parameter determining coupling strength. The interaction can be tailored to operate either on external degrees of freedom leading to atomic crystallization for thermal atoms and supersolids for a quantum degenerate gas, or on internal degrees of freedom like populations of the excited state or Zeeman sublevels. Using the light polarization degrees of freedom on the Poincaré sphere (helicity and polarization direction), specific irreducible tensor components of the atomic Zeeman states can be coupled leading to spontaneous magnetic ordering of states of dipolar and quadrupolar nature. The requirements for critical interaction strength are compared for the different situations. Connections and extensions to longitudinally pumped cavities, counterpropagating beam schemes and the CARL instability are discussed.
The rapidly developing field of optomechanics aims at the combined control of optical and mechanical (solid-state or atomic) modes. In particular, laser cooled atoms have been used to exploit optomechanical coupling for self-organization in a variety of schemes where the accessible length scales are constrained by a combination of pump modes and those associated to a second imposed axis, typically a cavity axis. Here, we consider a system with many spatial degrees of freedom around a single distinguished axis, in which two symmetries - rotations and translations in the plane orthogonal to the pump axis - are spontaneously broken. We observe the simultaneous spatial structuring of the density of a cold atomic cloud and an optical pump beam. The resulting patterns have hexagonal symmetry. The experiment demonstrates the manipulation of matter by opto-mechanical self-assembly with adjustable length scales and can be potentially extended to quantum degenerate gases.
Abstract Cold atom setups are now commonly employed in simulations of condensed matter phenomena. We present an approach to induce strong magnetic interactions between atoms on a self-organized lattice using diffraction of light. Diffractive propagation of structured light fields leads to an exchange between phase and amplitude modulated planes which can be used to couple atomic degrees of freedom via optical pumping nonlinearities. In the experiment a cold cloud of Rb atoms placed near a retro-reflecting mirror is driven by a detuned pump laser. We demonstrate spontaneous magnetic ordering in the Zeeman sublevels of the atomic ground state: anti-ferromagnetic structures on a square lattice and ferrimagnetic structures on a hexagonal lattice in zero and a weak longitudinal magnetic field, respectively. The ordered state is destroyed by a transverse magnetic field via coherent dynamics. A connection to the transverse (quantum) Ising model is drawn.
Photon-mediated interaction can be used for simulating complex many-body phenomena with ultracold atoms coupled to electromagnetic modes of an optical resonator. We study theoretically a method of producing controllable interatomic interaction mediated by forward-diffracted photons circulating inside a ring cavity. One example of such a system is the three-mode cavity, where an on-axis mode can coexist with two diffracted sidebands. We demonstrate how the self-organized stripe states of a Bose-Einstein condensate (BEC) occurring in this cavity geometry can exhibit supersolid properties, due to spontaneous breaking of the Hamiltonian's continuous translational symmetry. A numerical study of the collective excitation spectrum of these states demonstrates the existence of massless and finite-gap excitations, which are identified as phase (Goldstone) and amplitude (Higgs) atomic density modes. We further demonstrate how judicious Fourier filtering of intracavity light can be used to engineer the effective atom-atom interaction profile for many cavity modes. The numerical results in this configuration show the existence of droplet-array and single-droplet BEC states for commensurate and incommensurate cavity modes, respectively. Diffractive coupling in a cavity is thereby introduced as an alternative route towards tailoring the photon-mediated interaction of ultracold atoms. Spatial features of the self-organized optical potentials can here be tuned to scales several times larger than the pump laser wavelength such that the corresponding atomic density distributions could be imaged and manipulated using low-numerical-aperture optics. These calculations and insights pave the way towards quantum simulation of exotic nonequilibrium many-body physics with condensates in a cavity.
Self-structuring via symmetry breaking is a prominent collective phenomenon occurring in cold and ultracold atoms coupled to optical fields [1] . Experimental realizations by means of trapped dipolar gases and optical cavities have shed light onto supersolidity and crystallization in out-of-equilibrium atomic systems [2] , [3] . Recent work demonstrated the occurrence of structural phase transitions between hexagonally coordinated supersolid phases in dipolar condensates [4] . In this work, we address 2D structural transitions occurring in an ensemble of cold thermal atoms with effective optomechanical interactions mediated by a coherent beam retro-reflected by means of a feedback mirror. The feedback loop scheme is represented in Fig. 1(a) , where the dipole potential induces atomic density structures which, in turn, scatter photons into side-band modes enhancing the potential itself and leading to transverse light-atom self-structuring, sharing similarities with an effective-Kerr nonlinear medium [5] .