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Optics Letters

Experimental realization of wavelength multiplexed nonlinear upconversion in cesium atoms

Jinze Wu, Yuhui Xu, Ruige Dong, Junxiang Zhang

Published Jun 2, 2021• 17 citations
Publisher

Abstract

Blue-violet wavelength multiplexing offers the capability to enhance the operational capacity and efficiency in optical information processing, underwater communications, biology, and medicine. Here we present a specially designed atomic scheme of cesium for simultaneously generating two blue-violet lasers at 456 and 459 nm via four-wave-mixing (FWM)-based upconversion processes. We experimentally and theoretically show that a double-diamond-type coherent system pumped with 852 and 921 nm lasers is responsible for the efficient generation of the two blue-violet lasers. In this system, the large population inversions lead to self-amplified spontaneous emissions at 15.6 and 12.1 µ m , which, in turn, serve as the seeds for enhanced double FWM processes with dual-wavelength upconversions.

DOI
10.1364/ol.428307

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Blue-violet wavelength multiplexing offers the capability to enhance the operational capacity and efficiency in optical information processing, underwater communications, biology, and medicine. Here we present a specially designed atomic scheme of cesium for simultaneously generating two blue-violet lasers at 456 and 459 nm via four-wave-mixing (FWM)-based upconversion processes. We experimentally and theoretically show that a double-diamond-type coherent system pumped with 852 and 921 nm lasers is responsible for the efficient generation of the two blue-violet lasers. In this system, the large population inversions lead to self-amplified spontaneous emissions at 15.6 and 12.1 µ m , which, in turn, serve as the seeds for enhanced double FWM processes with dual-wavelength upconversions.
Nondegenerate four-wave mixing (FWM) in diamond-type atomic systems has important applications in a wide range of fields, including quantum entanglement generation, frequency conversion, and optical information processing. Although the efficient self-seeded nondegenerate FWM with amplified spontaneous emission (ASE) has been realized extensively, the seeded nondegenerate FWM without ASE is inefficient in reported experiments so far. Here we present the experimental realization of the seeded nondegenerate FWM in cesium atoms with a significantly improved efficiency. Specifically, with two pump lasers at 852 and 921 nm and a seed laser at 895 nm, a continuous-wave laser at 876 nm is efficiently generated via FWM in a cesium vapor cell with a power up to 1.2 mW, three orders of magnitude larger than what has been achieved in previous experiments. The improvement of the efficiency benefits from the exact satisfaction of the phase-matching condition realized by an elaborately designed setup. Our results may find applications in the generation of squeezing and entanglement of light via nondegenerate FWM.
Diode-pumped alkali lasers, possessing high efficiency and narrow linewidth, can provide feasible solutions for wavelength ranges difficult to reach by commercial lasers. In this study, we investigate a generation of coherent blue light (CBL) via four-wave mixing (FWM)-based up-conversion processes in cesium (Cs) vapor. A bichromatic pumping scheme with 852- and 917-nm lasers drives the Cs atoms to the 6 D 5/2 excited level, followed by cascaded decay of 6 D 5/2 → 7 P 3/2 → 6 S 1/2 , producing 456-nm CBL under phase matching conditions. The fluorescence in multiple bands from blue to near- and far-infrared in the FWM process is demonstrated under different experimental conditions. To optimize the experimental parameters, we investigate the dependence of 456-nm CBL on the vapor temperature, frequency, and intensity of the two pump lasers. A maximum power of 2.94 mW is achieved with pump powers of 430 mW (for 852 nm) and 470 mW (for 917 nm). The corresponding conversion efficiency is 1.5%/W, three-fold higher than those in previous studies. Our results can contribute to fundamental research on atom—photon interactions and quantum metrology.
We demonstrate the generation of coherent and collimated blue light (CBL) based on cesium (Cs) 6S1/2(F = 4)→6P3/2(F' = 5)→6D5/2(F'' = 6)→7P3/2(F' = 5)→6S1/2(F = 4) diamond-type atomic system in a heated vapor cell. Two infrared pumping lasers with wavelengths at 852 nm (6S1/2→6P3/2) and 917 nm (6P3/2→6D5/2), provide step-wise excitation to the 6D5/2 excited state, and induce strong two-photon coherence between the 6S1/2 state and 6D5/2 state. The atoms undergo a double cascade accompanied with the amplified spontaneous emission at 15.1 μm via the 7P3/2 intermediate excited state, and produce a beam of 455 nm (7P3/2→6S1/2) CBL with highly spatiotemporal coherence through a parametric four-wave mixing process. We investigate the influence of experimental parameters such as polarization combination of the two pumping lasers, and their power, and the temperature of Cs vapor cell on the CBL. Especially, we add a beam of 894 nm laser operating at the 6S1/2(F = 3) →6P1/2 transition as repumping laser, which can pump atoms back to the 6S1/2(F = 4) state from the 6S1/2(F = 3) state, thus significantly improving the power of CBL. This technique of the CBL enhancement via optical pumping is also useful for the other alkali metal atoms.
We demonstrate the generation of polychromatic and collimated lights at 456 nm, 459 nm, and 761 nm based on cesium ( 133 Cs) 6S 1/2 - 6P 3/2 - 8S 1/2 - 7P 3/2 , 7P 1/2 , 6P 1/2 - 6S 1/2 multi-diamond-type atomic system via two-photon excitation with two IR pump lasers at 852 nm and 795 nm. The 456 nm, 459 nm (7P 3/2 , 7P 1/2 → 6S 1/2 ) collimated blue lights result from the self-seeded four-wave mixing process (FWM), and the 761 nm coherent light (8S 1/2 → 6P 1/2 ) is from a seeded FWM process with the injection of a third laser at 895 nm. We measure the dependency of generated polychromatic fields on the temperature of 133 Cs vapor cell and the powers of input lasers, clearly demonstrating the competition between the self-seeded FWM and seeded FWM, as they share the same excitation path. This work is helpful to further produce entangled multi-color photons for quantum communication.
Nondegenerate four-wave mixing (NFWM) is a practical and effective technique for generating or amplifying light fields at different wavelengths, and could be used to create color correlation and entanglement. Here we experimentally investigate the NFWM process in diamond atomic system via two-photon excitation with two pumps at 852 nm and 921 nm, demonstrating that a seeded NFWM with a third laser at 895 nm and two self-seeded NFWMs due to amplified spontaneous emission (ASE) occur simultaneously. We compare the two kinds of processes and show that the single- and two-photon detunings hold the key role in distinguishing them. As a result, the enhancement of seeded NFWM is obtained by selecting large one- and two-photon detunings, in which case the ASE induced self-seeded NFWM can be largely suppressed. In contrast, the ASE and its induced NFWM are effectively achieved with one- and two-photon resonant excitations allowing for population inversion for efficient ASE.
This paper reports the simultaneous output of 358.7nm and 420.3nm laser generated by two-photon excitation (52 S1/2→62 D5/2, TPE) and four-wave mixing effect (FWM) in rubidium system for the first time. Unlike some fluorescent signals, this four-wave mixing beam has a high monochromaticity and extreme directivity and can be used as a laser source. In this study, we also measured the fluorescence lines in the range of 300-820 nm under 52 S1/2→62 D5/2 TPE, and studied other transitions that may occur. The experimental results show that the blue-violet laser produced by this alkali metal rubidium four-wave mixing can provide a new laser source for underwater laser communication, display technology, fluorescence excitation, Raman spectroscopy, marine resource detection, laser biomedicine, lithography, high density information storage and other fields.