With the advent of ultracold atomic gases experimentally realized by laser cooling techniques nearly 40 years ago, the doors to accessing novel physical behaviour have been opened wide and far. Experimentally, research in this domain started with alkali atoms, proceeded with alkaline earth atoms, and only more recently embarked on atoms with higher complexity of their spectrum, as e.g. the highly dipolar lanthanide atomic species erbium and dysprosium. Those elements possess a non-vanishing orbital angular momentum in the ground state, leading to ample advantages for the manipulation with far-detuned laser light in phase imprinting schemes, as losses due to spontaneous scattering can be suppressed radically in comparison to the case of alkali atomic species. This beneficial behaviour will be used in the future for the generation of synthetic magnetic fields for electrically neutral erbium atoms aimed at investigating fractional quantum Hall physics. This thesis describes in the first part the generation of an atomic erbium Bose-Einstein condensate in a hybrid crossed optical dipole trap. The main purpose of this endeavor was an enhancement of absolute atom number of the degenerate ensemble and long-term stability of the experimental setup with respect to the use of a single beam dipole trap. A comparison of the here achieved results with respect to those achieved in only a single CO2 laser beam dipole trap is illustrated. In the second part of this thesis a theoretical evaluation of the generation of synthetic magnetic fields for ultracold erbium atoms in prospect for experimental investigations of fractional quantum Hall physics is presented. One of the most promising techniques for the realization of strong synthetic magnetic fields is by phase imprinting via Raman manipulation. Here for the theoretical calculation of such fields with erbium atoms a compared to earlier work on alkali atoms new modified optical Raman coupling scheme in a σ+ - σ- beam polarization configuration is chosen. It is shown that sufficiently high field strengths with good spatial homogeneity can be reached for experimentally viable parameters. Additionally, an estimation for the expected Laughlin gap in the proposed erbium atomic fractional quantum Hall system is given.
With the advent of ultracold atomic gases experimentally realized by laser cooling techniques nearly 40 years ago, the doors to accessing novel physical behaviour have been opened wide and far. Experimentally, research in this domain started with alkali atoms, proceeded with alkaline earth atoms, and only more recently embarked on atoms with higher complexity of their spectrum, as e.g. the highly dipolar lanthanide atomic species erbium and dysprosium. Those elements possess a non-vanishing orbital angular momentum in the ground state, leading to ample advantages for the manipulation with far-detuned laser light in phase imprinting schemes, as losses due to spontaneous scattering can be suppressed radically in comparison to the case of alkali atomic species. This beneficial behaviour will be used in the future for the generation of synthetic magnetic fields for electrically neutral erbium atoms aimed at investigating fractional quantum Hall physics. This thesis describes in the first part the generation of an atomic erbium Bose-Einstein condensate in a hybrid crossed optical dipole trap. The main purpose of this endeavor was an enhancement of absolute atom number of the degenerate ensemble and long-term stability of the experimental setup with respect to the use of a single beam dipole trap. A comparison of the here achieved results with respect to those achieved in only a single CO2 laser beam dipole trap is illustrated. In the second part of this thesis a theoretical evaluation of the generation of synthetic magnetic fields for ultracold erbium atoms in prospect for experimental investigations of fractional quantum Hall physics is presented. One of the most promising techniques for the realization of strong synthetic magnetic fields is by phase imprinting via Raman manipulation. Here for the theoretical calculation of such fields with erbium atoms a compared to earlier work on alkali atoms new modified optical Raman coupling scheme in a σ+ - σ- beam polarization configuration is chosen. It is shown that sufficiently high field strengths with good spatial homogeneity can be reached for experimentally viable parameters. Additionally, an estimation for the expected Laughlin gap in the proposed erbium atomic fractional quantum Hall system is given.
The implementation of the fractional quantum Hall effect in ultracold atomic quantum gases remains, despite substantial advances in the field, a major challenge. Since atoms are electrically neutral, a key ingredient is the generation of sufficiently strong artificial gauge fields. Here we theoretically investigate the synthetization of such fields for bosonic erbium atoms by phase imprinting with two counterpropagating optical Raman beams. Given the nonvanishing orbital angular momentum of the rare-earth atomic species erbium in the electronic ground state and the availability of narrow-line transitions, heating from photon scattering is expected to be lower than in atomic alkali-metal species. We give a parameter regime for which strong synthetic magnetic fields with good spatial homogeneity are predicted. We also estimate the size of the Laughlin gap expected from the s-wave contribution of the interactions for typical experimental parameters of a two-dimensional atomic erbium microcloud. Our analysis shows that cold rare-earth atomic ensembles are highly attractive candidate systems for experimental explorations of the fractional quantum Hall regime.
Physics of ultra cold atoms and molecules is one of the most rapidly developing areas of the modern atomic, molecular, optical physics and quantum optics.This area covers several sub-areas of diverse importance, but definitely two trends can be easily identifies: i) fundamental research on properties of ultra cold atoms and molecules, and in particular atomic and molecular condensates trapped and lattice gases; here the fundamental questions of nature and form of phase transitions in degenerate systems are being posed and studied; ii) more applications oriented research on ultracold atoms and molecules, involving in particular applications in precision measurements, atomic clocks, frequency standards, atom and molecule interferometry, quantum information, quantum engineering, "super" chemistry etc.This thesis concerns both of these major trends.The applications, or more specifically quantum engineering aspect are discussed in the first four chapters of the thesis, which deal with optical manipulations of ultra cold gases, in particular optical generation of vortices in Bose condensates, quasi-solitons in Fermi gases, and retarded dipole-dipole interactions in Bose, or Fermi gases.This thesis consists of four main chapters.Chapter 2, "Optical generation of vortices in Bose Einstein Condensates".In this chapter we study theoretically the generation of vortices by phase imprinting in trapped Bose-Einstein condensates.Phase imprinting is achieved by passing a short off-resonance laser pulse through an appropriately designed absorption plate, and impinging it on a condensate.We answer the fundamental question of how the circulation and the vortex are introduced into the system, and discuss the creation of vortex arrays.We discuss vortex dynamics and interactions in such configurations.Various methods of vortex detection based on interference combined with Bragg scattering are also analyzed.In Chapter 3, "Fermionic 'Solitons'" we investigate in detail the concept of low energy excitations of ultra cold Fermi gases.This excitations are generated using the same idea of phase imprinting as that employed in the generation of vortices in BEC.We address in this chapter some questions concerning the generation (via phase imprinting) of soliton-like solutions in a single-component Fermi gas of neutral atoms at zero and finite temperatures.By using both numerical and analytical calculations, we find the conditions under which it is possible to find in non-interacting Fermi gases, quasisolitons which resemble the properties of solitons in non-linear integrable equations.We present the results for both spatially homogeneous and trapped cases, and emphasize the importance of Fermi statistics and the absence of interactions for the existence of such solutions.In Chapter 4, "Generating Dipole Condensate" we keep studying the possibilities of optical manipulations of ultracold gases.In particular, we study two different ways to laser-induce dipole-dipole interactions in trapped Bose-Einstein condensates.The first one employs the fact that those atoms in high Rydberg states posses a large dipolar moment.We first analyze the idea of imposing the dipole moment as a time average over short stroboscopic pulses.These pulses are coherently transporting the atoms from the ground atomic state to some high Rydberg state and back.The second idea is based on the observation that in strong static or oscillatory electric fields, atoms polarize and acquire dipole moment.We analyze the possibilities and limitations of inducing such a high electric field using lasers of low frequency.In Chapter 5, "Dipolar BCS", we continue our study of trapped fermionic gases, with the analysis of the BCS transition in trapped dipolar fermionic gases.We find that the critical strength of the dipole-dipole interaction to achieve BCS pairing, depends on the trap geometry.We find the particular form of this dependence, and present the solutions for the order parameter.This first chapter is meant as a general introduction to the thesis.This introduction is by no means exhaustive, and should be rather treated as a collection of basic facts concerning ultra cold gases, without rigorous derivations.The last subsection of the introductory chapter, discusses very briefly the most important achievements and trends in the field and the current state of the art.
In 1925, Einstein predicted the condensation of bosons into the ground state of the system for low (but finite) temperatures. Several phenomena, including superfluidity and superconductivity have been associated with Bose-Einstein condensation, but these systems interact strongly with their environment and pure Bose-Einstein condensation could not be established. It took 70 years, in which time the laser was discovered, and laser cooling techniques to manipulate atoms in a dilute atomic gas, before Bose-Einstein condensation in dilute atomic gases could be demonstrated in 1995. In the first condensation experiments, BECs were created in a magnetic trap. Since in a magnetic trap not all mF states of the atom can be trapped simultaneously, thereby limiting the number of experiments that can be done, other ways of trapping and generating BECs were sought and found. In 2001, the first all-optical BEC was made, where the dipole force was used to trap atoms in the crossing of two far red detuned laser beams. In an optical dipole trap not only atoms in different internal states can be trapped, but also different atomic species simultaneously. In this thesis, the formation of an all-optical Bose-Einstein condensate with rubidium atoms is presented. Conventional all-optical BECs are usually created in high power CO2 laser dipole traps, or have complicated laser cooling schemes and complex dipole trap setups. In our simple and straightforward setup, we load rubidium atoms from a magneto-optical trap into a crossed optical dipole trap created by a single frequency Yb:YAG laser with a wavelength at 1030 nm. The small wavelength allows for a small diffraction limit, and permits us to use standard optical materials, thus making the experimental setup cost effective. Other attempts to achieve Bose-Einstein condensation in a multi-mode (frequency) fiber laser at 1064 nm failed, because the atom loss was quite high. It is assumed that the multi-mode character of the fiber laser induces Raman transitions in rubidium atoms, thereby heating them. We can trap about ∼ 5E7 atoms in a single beam dipole trap out of ∼ 5E9 atoms trapped in theMOT, and ∼ 350,000 atoms can be trapped in a crossed beam dipole trap due to the smaller trap volume. 70% of the atoms in the dipole trap is optically pumped into one mF state. Quantum degeneracy is reached by evaporatively cooling the atoms in the crossed dipole trap by ramping down the laser power with three linear ramps. We can independently change the power of each beam by an AOM. This allows us to use one beam as an atom waveguide for future experiments. After evaporation, we typically have about 10,000 atoms at a temperature below the critical temperature. We have proved Bose-Einstein condensation by using the anisotropic expansion of a quantum degenerate gas trapped in an anisotropic potential. The aspect ratio of our atom cloud changed during a time of flight from 0.7 to 1.2 in 10 ms, thus proving that we have reached quantum degeneracy. We have about 5,000 condensed atoms in our optical dipole trap at a temperature less than 100 nK. The remaining atoms are thermal. Bose-Einstein condensation is obtained within 8 s, and we can repeat the experiment every 30 s. It should be mentioned that the Bose-Einstein experiment was moved from the ”Leibniz Universität Hannover” to the ”Technische Universität Darmstadt”, and had to be completely rebuilt. All-optical Bose-Einstein condensation was reached within one year after the move. Our Bose-Einstein condensation setup presents an ideal starting point for using our condensates in combination with miniaturized atom optical setups based on our novel microfabricated optical elements. With our microlenses, we can create a number of possible dipole trap configurations, such as the dipole trap array or the cylindrical microlens array. Using microlenses in miniaturized atom optical setups opens a completely new field of coherent atom optics. Also because the tight confinement of the microtraps allows us to load a 3D BEC, a 1D BEC, or a Tonks-Girardeau gas in the micropotentials depending on the density.
Research on degenerate quantum gases of dilute atomic gases has become a well established field in modern physics and revealed many astonishing phenomena. The first experiments on Bose and Fermi gases at low temperatures aimed to prove the predictions of quantum mechanics on a macroscopic scale. Since then we make use of Bose and Fermi gases and mixtures of any combination to model other many body systems. A property of Bose Einstein condensates is superfluidity which we want to investigate further in toroidal potentials with a new apparatus which can produce an all-optical BEC. This means trapping thermal atoms in an optical dipole trap and cooling the sample by evaporation into the quantum degenerate regime. This new technique was first successfully demonstrated by M.D. Barrett et al. in 2001 and promises to be faster and simpler than the well established and common way of evaporation in magnetic traps. A new apparatus was built by the author and we report on the experimental details of the trapping of 87Rb atoms from a hot vapour and cooling them in a magneto-optical trap, and further evaporation to quantum degeneracy in a crossed optical dipole trap operating at a wavelength of l = 1064nm, with accurate control of the power in both beams via a feedback loop. The evaporation of neutral atoms of 87Rb in far red detuned optical dipole traps using linearly polarised laser light is spin independent, and mixed spinor condensates of the F=1 manifold can be formed. As an empirical technique we found by applying a magnetic gradient field during the final evaporation that we can selectively populate mF spin states or prepare mixtures. This intriguing mechanism was found earlier as well by M. S. Chang, but is yet not fully understood and subject of our future research. We can now routinely prepare an almost pure condensate containing up to 7000 atoms in the condensed phase purely in the mF = 0 spin state. This thesis contains the theoretical framework of Bose-Einstein condensation with in mean-field theory, the concepts of cooling of atoms in magneto-optical traps, the trapping and evaporation in optical dipole traps and the experimental realisation. In the future this experiment will be extended by a fast scanning dipole trap to apply arbitrary time averaged potentials of more complex geometries, such as toroidal traps to study the effects of superfluidity in a periodic potential. The production of toroidal traps and cold atoms in such a trap are outlined in this thesis.
Quantum gas microscopy of dipolar atoms is a promising opportunity to expand upon previous quantum simulations of neutral atoms in optical lattices. Erbium atoms interact via the long-range magnetic dipole-dipole interaction, which leads to a variety of new many-body effects and strongly correlated phases that are currently unexplored in microscopes with only short-range interactions. In this thesis I will detail progress toward the construction of an erbium quantum gas microscope as well as the techniques we implemented to produce a Bose-Einstein condensate of 8×104 atoms in under a second. These include the installation of a dual-stage magneto-optical trap, a stroboscopic optical dipole trap, as well as a tunable crossed optical dipole trap that allows for efficient evaporation of both bosonic and fermionic isotopes. I will also discuss the frequency stabilization systems we have implemented to produce laser linewidths of less than 1 kHz for near-resonant laser cooling on narrow transitions and a custom, high NA reflective objective to be used as part of a high resolution imaging system. Finally, I will discuss the noise properties of charge-coupled devices and the photon counting techniques that are needed for having high fidelities while using fast imaging schemes.
Optical trapping as a viable means of exploring the physics of ultracold dilute atomic gases has revealed a new spectrum of physical phenomena. In particular, macroscopic and sudden occupation of the ground state below a critical temperature—-a phenomenon known as Bose-Einstein condensation—-has become an even richer system for the study of quantum mechanics, ultracold collisions, and many-body physics in general. Optical trapping liberates the spin degree of the BEC, making the order parameter vectorial (‘spinor BEC’), as opposed to the scalar order of traditional magnetically trapped condensates. The work described within is divided into two main efforts. The first encompasses the all-optical creation of a Bose-Einstein condensate in rubidium vapor. An all-optical path to spinor BEC (as opposed to transfer to an optical trap from a magnetic-trap condensate) was desired both for the simplicity of the experimental setup and also for the potential gains in speed of creation; evaporative cooling, the only known path to dilute-gas condensation, works only as efficiently as the rate of elastic collisions in the gas, a rate that starts out much higher in optical traps. The first all-optical BEC was formed elsewhere in 2001; the years following saw many groups worldwide seeking to create their own version. Our own all-optical spinor BEC, made with a single-beam dipole trap formed by a focused CO₂ laser, is described here, with particular attention paid to trap loading, measurement of trap parameters, and the use of a novel 780 nm high-power laser system. The second part describes initial experiments performed with the nascent condensate. The spinor properties of the condensate are documented, and a measurement is made of the density-dependent rate of spin mixing in the condensate. In addition, we demonstrate a novel dual-beam atom laser formed by outcoupling oppositely polarized components of the condensate, whose populations have been coherently evolved through spin dynamics. We drive coherent spin-mixing evolution through adiabatic compression of the initially weak trap. Such dual beams, nominally number-correlated through the angular momentum-conserving collision m=0 + m=0 ⇌ m=+1 + m=-1 have been proposed as tools to explore entanglement and squeezing in Bose-Einstein condensates.