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Characterising a tunable, pulsed atomic beam using matter-wave interferometry

James G. Morley, R. L. Flack, Hiley, BJ, P. F. Barker

Published Aug 4, 2021• 3 citations
OpenAlex

Abstract

We describe the creation and characterisation of a velocity tunable, spin-polarized beam of slow metastable argon atoms. We show that the beam velocity can be determined with a precision below 1% using matter-wave interferometry. The profile of the interference pattern was also used to determine the velocity spread of the beam, as well as the Van der Waals (VdW) co-efficient for the interaction between the metastable atoms and the multi-slit silicon nitride grating. The VdW co-efficient was determined to be C_{3} = 1.84 ± 0.17 a.u., in good agreement with values derived from spectroscopic data. Finally, the spin polarization of the beam produced during acceleration of the beam was also measured, demonstrating a spatially uniform spin polarization of 96% in the m = +2 state.

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Characterising a tunable, pulsed atomic beam using matter-wave interferometry

J Morley, R. L. Flack, Basil J. Hiley +1 more

Abstract We describe the creation and characterisation of a velocity tunable, spin-polarized beam of slow metastable argon atoms. We show that the beam velocity can be determined with a precision below 1% using matter-wave interferometry. The profile of the interference pattern was also used to determine the velocity spread of the beam, as well as the Van der Waals (VdW) co-efficient for the interaction between the metastable atoms and the multi-slit silicon nitride grating. The VdW co-efficient was determined to be C 3 = 1.84 ± 0.17 a.u., in good agreement with values derived from spectroscopic data. Finally, the spin polarization of the beam produced during acceleration of the beam was also measured, demonstrating a spatially uniform spin polarization of 96% in the m = +2 state.

arXiv:2103.04756•Journal of Physics B Atomic Molecular and Optical Physics•Jun 3, 2021•5 citations

Towards a weak measurement of transverse momentum in a matter-wave interferometer

Joel Morley

This thesis describes the construction of an atomic matter-wave interferometer, combined with a spin-state interferometer, used to weakly measure the average transverse momentum of the atoms. A velocity-tuneable cold atomic beam was constructed and characterised. By applying radiation pressure to a magneto-optical trap, the beam's velocity was selected between 1-52 ms-1. The beam was used to produce interference fringes in a matter-wave interferometer which consisted of a mutli-slit Si3Ni4 grating and a planar atom detector placed below the grating. The interference pattern was used to measure the average beam velocity and the Van der Waals coefficient between the atoms and the grating. This was the first instance of such a measurement. Below the grating a longitudinal Stern-Gerlach interferometer was constructed. The phase shift of the atom's spin, due to the Zeeman effect from the interferometer's magnetic field, was measured. The phase shift provided a measurement of the interferometer's magnetic field in the μT range. An experiment combining the two interferometers to weakly measure the atom's transverse momentum is described and modelled.

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The paper presents an experiment based on an efficient coupling between atomic Zeeman states (for atoms with internal angular momentum) allowed by the quadrupolar component of the surface- induced van der Waals (vdW) interaction. This exo-energetic "vdW - Zeeman" transition provides a tuneable (magnetic field intensity dependent) beam splitter that was theoretically illustrated by the simplest possible interferometer: an atomic counterpart of Fresnel biprism. The velocity - adjustable atomic beam is here coming across two opposite surfaces (single slit of a nano-grating). For a transverse coherent radius large enough, the atom wave packet is strongly inelastically diffracted by the two opposite surfaces at some distances from the slit to yield non localised interference fringes. The calculation has been done for Ar metastable atoms with a grating of 100 nm period and different velocities of the atoms (560 to 10 m/s). Via the interference pattern (Schlieren image), this device should give access to such novel information as the oscillating part of the complex vdW - interaction transition amplitude. This simplest configuration is not sensitive to inertial effect. As a next step, a loop - closing transmission grating was added to realize a new type of compact interferometer.

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Atom diffraction with a ‘natural’ metastable atom nozzle beam

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The resonant metastability-exchange process is used to obtain a metastable atom beam with intrinsic properties close to those of a ground-state atom nozzle beam (small angular aperture, narrow velocity distribution). The estimated effective source diameter (15 µm) is small enough to provide at a distance of 597 mm a transverse coherence radius of about 873 nm for argon, 1236 nm for neon and 1660 nm for helium. It is demonstrated both by experiment and numerical calculations with He*, Ne* and Ar* metastable atoms, that this beam gives rise to diffraction effects on the transmitted angular pattern of a silicon-nitride nano-slit grating (period 100 nm). Observed patterns are in good agreement with previous measurements with He* and Ne* metastable atoms. For argon, a calculation taking into account the angular aperture of the beam (0.35 mrad) and the effect of the van der Waals interaction—the van der Waals constant C 3 = 1.83 +0.1 −0.15 au being derived from spectroscopic data—leads to a good agreement with experiment.

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Van der Waals - Zeeman transitions of slow metastable argon atoms Ar*(3P2)

M. Hamamda, Thierry Taillandier-Loize, F. Perales +4 more

Metastable argon atoms Ar*(3P2), produced by electron bombardment of a nozzle beam of ground state Ar atoms, are slowed down from their initial thermal velocity of 560 m/s down to a few tens of m/s, using a standard Zeeman slower. In this decelerator, a repulsive force is induced by a counter-propagating σ+- polarized laser beam, locked in frequency on the3P2-3D3closed transition (λ= 811.5 nm) and then detuned by 340 MHz. A special profile of longitudinal magnetic field is adjusted in order to maintain atoms in resonance with light all over the device, by compensating the variable Doppler shift by the convenient Zeeman shift. Low velocities, e.g. 55 m/s, are accessible but due to spontaneous emission randomly distributed recoil momentums enlarge both angular and velocity distributions of the beam. Nevertheless, by placing off axis collimating slits and grating, it is in principle possible to observe transmission and/or diffraction phenomena specific of low velocities.

Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)•May 1, 2011•0 citations

Matter-wave/atom interferometry

John F. Clauser, Shifang Li

Although interferometry's earliest and most familiar use is with photons, the discovery of matter-wave (deBroglie-wave) interference for electrons demanded the development of quantum mechanics. Since then, matter-wave interferometry has been performed with neutrons, Cooper electron-pairs, and most recently, with whole atoms and diatomic molecules. This talk describes our recent high-flux atom interferometry experiments using the generalized Talbot-vonLau effect. Our interferometer consists of a sequence of three planar vacuum-slit diffraction gratings, microfabricated from silicon nitride membranes. DeBroglie-wave interference fringes are sensed by measuring the transmission of potassium atoms on a hot- wire as a function of grating relative position. Different spatial Fourier components (up to sixth) in the diffraction pattern are resonant in the interferometer at different atomic velocities (i.e., at different wavelengths). When a laser cooled slow atomic beam is incident, various different diffraction patterns are observed as a function of atomic velocity. In an alternative `Heisenberg Microscope' configuration an incident thermal beam produces a velocity average over different fringe Fourier components. AC modulated weak laser light passing through the interferometer interacts selectively with atoms at a specific velocity. The associated fringe pattern is then ac modulated and revealed by its selective destruction.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Dec 12, 1994•0 citations
We describe the creation and characterisation of a velocity tunable, spin-polarized beam of slow metastable argon atoms. We show that the beam velocity can be determined with a precision below 1% using matter-wave interferometry. The profile of the interference pattern was also used to determine the velocity spread of the beam, as well as the Van der Waals (VdW) co-efficient for the interaction between the metastable atoms and the multi-slit silicon nitride grating. The VdW co-efficient was determined to be C_{3} = 1.84 ± 0.17 a.u., in good agreement with values derived from spectroscopic data. Finally, the spin polarization of the beam produced during acceleration of the beam was also measured, demonstrating a spatially uniform spin polarization of 96% in the m = +2 state.
Abstract We describe the creation and characterisation of a velocity tunable, spin-polarized beam of slow metastable argon atoms. We show that the beam velocity can be determined with a precision below 1% using matter-wave interferometry. The profile of the interference pattern was also used to determine the velocity spread of the beam, as well as the Van der Waals (VdW) co-efficient for the interaction between the metastable atoms and the multi-slit silicon nitride grating. The VdW co-efficient was determined to be C 3 = 1.84 ± 0.17 a.u., in good agreement with values derived from spectroscopic data. Finally, the spin polarization of the beam produced during acceleration of the beam was also measured, demonstrating a spatially uniform spin polarization of 96% in the m = +2 state.
This thesis describes the construction of an atomic matter-wave interferometer, combined with a spin-state interferometer, used to weakly measure the average transverse momentum of the atoms. A velocity-tuneable cold atomic beam was constructed and characterised. By applying radiation pressure to a magneto-optical trap, the beam's velocity was selected between 1-52 ms-1. The beam was used to produce interference fringes in a matter-wave interferometer which consisted of a mutli-slit Si3Ni4 grating and a planar atom detector placed below the grating. The interference pattern was used to measure the average beam velocity and the Van der Waals coefficient between the atoms and the grating. This was the first instance of such a measurement. Below the grating a longitudinal Stern-Gerlach interferometer was constructed. The phase shift of the atom's spin, due to the Zeeman effect from the interferometer's magnetic field, was measured. The phase shift provided a measurement of the interferometer's magnetic field in the μT range. An experiment combining the two interferometers to weakly measure the atom's transverse momentum is described and modelled.
The paper presents an experiment based on an efficient coupling between atomic Zeeman states (for atoms with internal angular momentum) allowed by the quadrupolar component of the surface- induced van der Waals (vdW) interaction. This exo-energetic "vdW - Zeeman" transition provides a tuneable (magnetic field intensity dependent) beam splitter that was theoretically illustrated by the simplest possible interferometer: an atomic counterpart of Fresnel biprism. The velocity - adjustable atomic beam is here coming across two opposite surfaces (single slit of a nano-grating). For a transverse coherent radius large enough, the atom wave packet is strongly inelastically diffracted by the two opposite surfaces at some distances from the slit to yield non localised interference fringes. The calculation has been done for Ar metastable atoms with a grating of 100 nm period and different velocities of the atoms (560 to 10 m/s). Via the interference pattern (Schlieren image), this device should give access to such novel information as the oscillating part of the complex vdW - interaction transition amplitude. This simplest configuration is not sensitive to inertial effect. As a next step, a loop - closing transmission grating was added to realize a new type of compact interferometer.
The resonant metastability-exchange process is used to obtain a metastable atom beam with intrinsic properties close to those of a ground-state atom nozzle beam (small angular aperture, narrow velocity distribution). The estimated effective source diameter (15 µm) is small enough to provide at a distance of 597 mm a transverse coherence radius of about 873 nm for argon, 1236 nm for neon and 1660 nm for helium. It is demonstrated both by experiment and numerical calculations with He*, Ne* and Ar* metastable atoms, that this beam gives rise to diffraction effects on the transmitted angular pattern of a silicon-nitride nano-slit grating (period 100 nm). Observed patterns are in good agreement with previous measurements with He* and Ne* metastable atoms. For argon, a calculation taking into account the angular aperture of the beam (0.35 mrad) and the effect of the van der Waals interaction—the van der Waals constant C 3 = 1.83 +0.1 −0.15 au being derived from spectroscopic data—leads to a good agreement with experiment.
Metastable argon atoms Ar*(3P2), produced by electron bombardment of a nozzle beam of ground state Ar atoms, are slowed down from their initial thermal velocity of 560 m/s down to a few tens of m/s, using a standard Zeeman slower. In this decelerator, a repulsive force is induced by a counter-propagating σ+- polarized laser beam, locked in frequency on the3P2-3D3closed transition (λ= 811.5 nm) and then detuned by 340 MHz. A special profile of longitudinal magnetic field is adjusted in order to maintain atoms in resonance with light all over the device, by compensating the variable Doppler shift by the convenient Zeeman shift. Low velocities, e.g. 55 m/s, are accessible but due to spontaneous emission randomly distributed recoil momentums enlarge both angular and velocity distributions of the beam. Nevertheless, by placing off axis collimating slits and grating, it is in principle possible to observe transmission and/or diffraction phenomena specific of low velocities.
Although interferometry's earliest and most familiar use is with photons, the discovery of matter-wave (deBroglie-wave) interference for electrons demanded the development of quantum mechanics. Since then, matter-wave interferometry has been performed with neutrons, Cooper electron-pairs, and most recently, with whole atoms and diatomic molecules. This talk describes our recent high-flux atom interferometry experiments using the generalized Talbot-vonLau effect. Our interferometer consists of a sequence of three planar vacuum-slit diffraction gratings, microfabricated from silicon nitride membranes. DeBroglie-wave interference fringes are sensed by measuring the transmission of potassium atoms on a hot- wire as a function of grating relative position. Different spatial Fourier components (up to sixth) in the diffraction pattern are resonant in the interferometer at different atomic velocities (i.e., at different wavelengths). When a laser cooled slow atomic beam is incident, various different diffraction patterns are observed as a function of atomic velocity. In an alternative `Heisenberg Microscope' configuration an incident thermal beam produces a velocity average over different fringe Fourier components. AC modulated weak laser light passing through the interferometer interacts selectively with atoms at a specific velocity. The associated fringe pattern is then ac modulated and revealed by its selective destruction.