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Broadband Geodesic Pulses for Three Spin Systems: Time-Optimal Realization of Effective Trilinear Coupling Terms and Indirect SWAP Gates

Timo O. Reiss, Navin Khaneja, Steffen J. Glaser

Published Jan 1, 2003• 31 citations
OpenAlex

Abstract

Broadband implementations of time-optimal geodesic pulse elements are introduced for the efficient creation of effective trilinear coupling terms for spin systems consisting of three weakly coupled spins 1/2. Based on these pulse elements, the time-optimal implementation of indirect SWAP operations is demonstrated experimentally. The duration of indirect SWAP gates based on broadband geodesic sequence is reduced by 42.3 % compared to conventional approaches. 1 1

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Broadband implementations of time-optimal geodesic pulse elements are introduced for the efficient creation of effective trilinear coupling terms for spin systems consisting of three weakly coupled spins 1/2. Based on these pulse elements, the time-optimal implementation of indirect SWAP operations is demonstrated experimentally. The duration of indirect SWAP gates based on broadband geodesic sequence is reduced by 42.3 % compared to conventional approaches. 1 1
Radio-frequency pulses are used in nuclear-magnetic-resonance spectroscopy to produce unitary transfer of states. Pulse sequences that accomplish a desired transfer should be as short as possible in order to minimize the effects of relaxation, and to optimize the sensitivity of the experiments. Many coherence-transfer experiments in NMR, involving a network of coupled spins, use temporary spin decoupling to produce desired effective Hamiltonians. In this paper, we demonstrate that significant time can be saved in producing an effective Hamiltonian if spin decoupling is avoided. We provide time-optimal pulse sequences for producing an important class of effective Hamiltonians in three-spin networks. These effective Hamiltonians are useful for coherence-transfer experiments in three-spin systems and implementation of indirect swap and ${\ensuremath{\Lambda}}_{2}(U)$ gates in the context of NMR quantum computing. It is shown that computing these time-optimal pulses can be reduced to geometric problems that involve computing sub-Riemannian geodesics. Using these geometric ideas, explicit expressions for the minimum time required for producing these effective Hamiltonians, transfer of coherence, and implementation of indirect swap gates, in a three-spin network are derived (Theorems 1 and 2). It is demonstrated that geometric control techniques provide a systematic way of finding time-optimal pulse sequences for transferring coherence and synthesizing unitary transformations in quantum networks, with considerable time savings (e.g., 42.3% for constructing indirect swap gates).
What is the time-optimal way of realizing quantum operations? Here, we show how important instances of this problem can be related to the study of shortest paths on the surface of a sphere under a special metric. Specifically, we provide an efficient synthesis of a controlled-NOT (CNOT) gate between qubits (spins 12\frac{1}{2}21​) coupled indirectly via Ising-type couplings to a third spin. Our implementation of the CNOT gate is significantly shorter than conventional approaches. The pulse sequences for efficient manipulation of our coupled spin system are obtained by explicit computation of geodesics on a sphere under the special metric. These methods are also used for the efficient synthesis of indirect couplings and of the Toffoli gate. We provide experimental realizations of the presented methods on a linear three-spin chain with Ising couplings.
Here we study the optimum efficiency of the excitation of maximum quantum (MaxQ) coherence using analytical and numerical methods based on optimal control theory. The theoretical limit of the achievable MaxQ amplitude and the minimum time to achieve this limit are explored for a set of model systems consisting of up to five coupled spins. In addition to arbitrary pulse shapes, two simple pulse sequence families of practical interest are considered in the optimizations. Compared to conventional approaches, substantial gains were found both in terms of the achieved MaxQ amplitude and in pulse sequence durations. For a model system, theoretically predicted gains of a factor of three compared to the conventional pulse sequence were experimentally demonstrated. Motivated by the numerical results, also two novel analytical transfer schemes were found: Compared to conventional approaches based on non-selective pulses and delays, double-quantum coherence in two-spin systems can be created twice as fast using isotropic mixing and hard spin-selective pulses. Also it is proved that in a chain of three weakly coupled spins with the same coupling constants, triple-quantum coherence can be created in a time-optimal fashion using so-called geodesic pulses.
Experiments in coherent nuclear and electron magnetic resonance and quantum computing in general correspond to control of quantum-mechanical systems, guiding them from initial to final target states by unitary transformations. The control inputs (pulse sequences) that accomplish these unitary transformations should take as little time as possible so as to minimize the effects of relaxation and decoherence and to optimize the sensitivity of the experiments. Here, we derive a time-optimal sequences as fundamental building blocks to synthesize unitary transformations. Such sequences can be widely implemented on various physical systems, including the simulation of effective Hamiltonians for topological quantum computing on spin lattices. Experimental demonstrations are provided for a system consisting of three nuclear spins.
What is the time-optimal way of realizing quantum operations? Here, we show how important instances of this problem can be related to the study of shortest paths on the surface of a sphere under a special metric. Specifically, we provide an efficient synthesis of a controlled NOT (CNOT) gate between qubits coupled indirectly via Ising-type couplings to a third spin. Our implementation of the CNOT gate is more than twice as fast as conventional approaches. The pulse sequences for efficient manipulation of our coupled spin system are obtained by explicit computation of geodesics on a sphere under the special metric. These methods are also used for the efficient synthesis of indirect couplings and of the Toffoli gate. We provide experimental realizations of the presented methods on a linear three-spin chain with Ising couplings.