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Non-thermal energy fluctuations of a diamond spin qutrit with feedback-controlled dissipative dynamics

Santiago Hernández-Gómez, Stefano Gherardini, Nicolas Staudenmaier, Francesco Poggiali, Michele Campisi, Andrea Trombettoni, F. S. Cataliotti, Paola Cappellaro, Nicole Fabbri

Published May 28, 2021• 2 citations

Abstract

Engineered dynamical maps that combine not only coherent, but also unital and dissipative transformations of quantum states, have demonstrated a number of technological applications, and promise to be a beneficial tool also in quantum thermodynamic processes. Here, we exploit control of a spin qutrit to investigate energy exchange fluctuations of an open quantum system. The qutrit engineer dynamics can be understood as an autonomous feedback process, where random measurement events condition the subsequent dissipative evolution. To analyze this dynamical process, we introduce a generalization of the Sagawa-Ueda-Tasaki relation for dissipative dynamics and verify it experimentally. Not only we characterize the efficacy of the autonomous feedback protocol, but also find that the characteristic function of energy variations $G(\eta)$ becomes insensitive to the process details at a single specific value of its argument. This allows us to demonstrate that a fluctuation theorem of the Jarzynski type holds for this general dissipative feedback dynamics, while previous relations were limited to unital dynamics. Moreover, in addition to the feedback efficacy, we find a witness of unitality associated with the fixed point of the dynamics.

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Engineered dynamical maps that combine not only coherent, but also unital and dissipative transformations of quantum states, have demonstrated a number of technological applications, and promise to be a beneficial tool also in quantum thermodynamic processes. Here, we exploit control of a spin qutrit to investigate energy exchange fluctuations of an open quantum system. The qutrit engineer dynamics can be understood as an autonomous feedback process, where random measurement events condition the subsequent dissipative evolution. To analyze this dynamical process, we introduce a generalization of the Sagawa-Ueda-Tasaki relation for dissipative dynamics and verify it experimentally. Not only we characterize the efficacy of the autonomous feedback protocol, but also find that the characteristic function of energy variations

G(\eta)

becomes insensitive to the process details at a single specific value of its argument. This allows us to demonstrate that a fluctuation theorem of the Jarzynski type holds for this general dissipative feedback dynamics, while previous relations were limited to unital dynamics. Moreover, in addition to the feedback efficacy, we find a witness of unitality associated with the fixed point of the dynamics.

Discrete quantum feedback control consists of a managed dynamics according to the information acquired by a previous measurement. Energy fluctuations along such dynamics satisfy generalized fluctuation relations, which are useful tools to study the thermodynamics of systems far away from equilibrium. Due to the practical challenge to assess energy fluctuations in the quantum scenario, the experimental verification of detailed fluctuation relations in the presence of feedback control remains elusive. We present a feasible method to experimentally verify detailed fluctuation relations for discrete feedback control quantum dynamics. Two detailed fluctuation relations are developed and employed. The method is based on a quantum interferometric strategy that allows the verification of fluctuation relations in the presence of feedback control. An analytical example to illustrate the applicability of the method is discussed. The comprehensive technique introduced here can be experimentally implemented at a microscale with the current technology in a variety of experimental platforms.

Feedback uses past detection outcomes to dynamically modify a quantum system and is central to quantum control. These outcomes can be stored in a memory, defined as a stochastic function of past measurements. In this work, we investigate the main properties of a general memory function subject to arbitrary feedback dynamics. We show that the memory can be treated as a classical system coupled to the monitored quantum system, and that their joint evolution is described by a hybrid bipartite state. This framework allows us to introduce information-theoretic measures that quantify the correlations between the system and the memory. Furthermore, we develop a general framework to characterize the statistics of the memory -- such as moments, cumulants, and correlation functions -- which can be applied both to general feedback-control protocols and to monitored systems without feedback. As an application, we analyze feedback schemes based on detection events in a two-level system coupled to a thermal bath, focusing on protocols that stabilize either the excited-state population or Rabi oscillations against thermal dissipation.

Thermodynamic principles governing energy and information are important tools for a deeper understanding and better control of quantum systems. In this work, we experimentally investigate the interplay of the thermodynamic costs and information flow in a quantum system undergoing iterative quantum measurement and feedback. Our study employs a state stabilization protocol involving repeated measurement and feedback on an electronic spin qubit associated with a silicon-vacancy center in diamond, which is strongly coupled to a diamond nanocavity. This setup allows us to verify the fundamental laws of nonequilibrium quantum thermodynamics, including the second law and the fluctuation theorem, both of which incorporate measures of quantum information flow induced by iterative measurement and feedback. We further assess the reducible entropy based on the feedback’s causal structure and quantitatively demonstrate the thermodynamic advantages of non-Markovian feedback over Markovian feedback. For that purpose, we extend the theoretical framework of quantum thermodynamics to include the causal structure of the applied feedback protocol. Our work lays the foundation for investigating the entropic and energetic costs of real-time quantum control in various quantum systems.

Control of open quantum systems is an essential ingredient to the realization of contemporary quantum science and technology. We demonstrate such control by employing a thermodynamically consistent framework, taking into account the fact that the drive can modify the interaction with environment. Such an effect is incorporated within the dynamical equation, leading to control dependent dissipation, this relation serves as the key element for open system control. Thermodynamics of the control process is reflected by a unidirectional flow of energy to the environment resulting in large entropy production. The control paradigm is displayed by analyzing entropy changing state to state transformations, such as heating and cooling. In addition, the generation of quantum gates under dissipative conditions is demonstrated for both non-unitary reset maps with complete memory loss and a universal set of single and double qubit unitary gates.

We present fluctuation theorems and moment generating function equalities for generalized thermodynamic observables and quantum dynamics described by completely positive trace preserving maps, with and without feedback control. Our results include the quantum Jarzynski equality and Crooks fluctuation theorem, and clarify the special role played by the thermodynamic work and thermal equilibrium states in previous studies. We show that for a specific class of generalized measurements, which include projective measurements, unitality replaces microreversibility as the condition for the physicality of the reverse process in our fluctuation theorems. We present an experimental application of our theory to the problem of extracting the system-bath coupling magnitude, which we do for a system of pairs of coupled superconducting flux qubits undergoing quantum annealing.