Optical photons are powerful carriers of quantum information, which can be delivered in free space by satellites or in fibers on the ground over long distances. Entanglement of quantum states over long distances can empower quantum computing, quantum communications, and quantum sensing. Quantum optical memories are devices designed to store quantum information in the form of stationary excitations, such as atomic coherence, and are capable of coherently mapping these excitations to flying qubits. Quantum memories can effectively store and manipulate quantum states, making them indispensable elements in future long-distance quantum networks. Over the past two decades, quantum optical memories with high fidelities, high efficiencies, long storage times, and promising multiplexing capabilities have been developed, especially at the single-photon level. In this review, we introduce the working principles of commonly used quantum memory protocols and summarize the recent advances in quantum memory demonstrations. We also offer a vision for future quantum optical memory devices that may enable entanglement distribution over long distances.
Quantum memories will be an essential part of many quantum information protocols, including distributed quantum computing, quantum sensing, and the synchronization of repeater nodes. Most efforts toward developing such a quantum memory have been focused on matter-based storage systems, which convert the energy and information from an optical state to an atomic state of matter to be retrieved later. These matter memories, while capable of achieving great storage times, have several limitations; namely, they are inherently narrow bandwidth, they typically do not operate at key telecommunications wavelengths, and often require costly overhead in the form of cryogenics. In this work, we have developed a quantum memory that operates in free space at room temperature, allowing us to avoid all the previously mentioned limitations, and achieve a record-high time-bandwidth product.
Interaction of quantum radiation with multi-particle ensembles has sparked off intense research efforts during the past decade. Emblematic of this field is the quantum memory scheme, where a quantum state of light is mapped onto an ensemble of atoms and then recovered in its original shape. While opening new access to the basics of light–atom interaction, quantum memory also appears as a key element for information processing applications, such as linear optics quantum computation and long-distance quantum communication via quantum repeaters. Not surprisingly, it is far from trivial to practically recover a stored quantum state of light and, although impressive progress has already been accomplished, researchers are still struggling to reach this ambitious objective. This special issue provides an account of the state-of-the-art in a fast-moving research area that makes physicists, engineers and chemists work together at the forefront of their discipline, involving quantum fields and atoms in different media, magnetic resonance techniques and material science. Various strategies have been considered to store and retrieve quantum light. The explored designs belong to three main—while still overlapping—classes. In architectures derived from photon echo, information is mapped over the spectral components of inhomogeneously broadened absorption bands, such as those encountered in rare earth ion doped crystals and atomic gases in external gradient magnetic field. Protocols based on electromagnetic induced transparency also rely on resonant excitation and are ideally suited to the homogeneous absorption lines offered by laser cooled atomic clouds or ion Coulomb crystals. Finally off-resonance approaches are illustrated by Faraday and Raman processes. Coupling with an optical cavity may enhance the storage process, even for negligibly small atom number. Multiple scattering is also proposed as a way to enlarge the quantum interaction distance of light with matter. The quest for higher efficiency, better fidelity, broader bandwidth, multimode capacity and longer storage lifetime is pursued in all those approaches, as shown in this special issue. The improvement of quantum memory operation specifically requires in-depth study and control of numerous physical processes leading to atomic decoherence. The present issue reflects the development of rare earth ion doped matrices offering long lifetime superposition states, either as bulk crystals or as optical waveguides. The need for quantum sources and high efficiency detectors at the single photon level is also illustrated. Several papers address the networking of quantum memories either in long-haul cryptography or in the prospect of quantum processing. In this context, much attention has been paid recently to interfacing quantum light with superconducting qubits and with nitrogen-vacancy centers in diamond. Finally, the quantum interfacing of light with matter raises questions on entanglement. The last two papers are devoted to the generation of entanglement by dissipative processes. It is shown that long lifetime entanglement may be built in this way. We hope this special issue will help readers to become familiar with the exciting field of ensemble-based quantum memories and will stimulate them to bring deeper insights and new ideas to this area.
Single photons are a vital resource for optical quantum information processing. Efficient and deterministic single photon sources do not yet exist, however. To date, experimental demonstrations of quantum processing primitives have been implemented using non-deterministic sources combined with heralding and/or postselection. Unfortunately, even for eight photons, the data rates are already so low as to make most experiments impracticable. It is well known that quantum memories, capable of storing photons until they are needed, are a potential solution to this `scaling catastrophe'. Here, we analyze in detail the benefits of quantum memories for producing multiphoton states, showing how the production rates can be enhanced by many orders of magnitude. We identify the quantity
etaB as the most important figure of merit in this connection, where
eta and
B are the efficiency and time-bandwidth product of the memories, respectively. We go on to review our progress in implementing the most broadband memory to date, with
B<1000, in room-temperature cesium vapour. We consider the noise properties for single photon storage and the integration of the memory using waveguides.
Quantum memory is a key component of quantum networks. A successful development in enabling the distribution of quantum information requires the storage of single-photon light. Usually quantum information is encoded using a 2D space, spanned, for example, by the orthogonal polarization states of a photon. In this case, each photon carries a quantum bit of information. If the photon could be encoded in a high-dimensional space instead, the information carried by each photon could be increased from a bit to |
log2d| bits, where d is the dimension of the Hilbert space in which the photon is described. The channel capacity of the network and the transmission efficiency would then be greatly enlarged [1]. Moreover, storing high-dimensional states in quantum memory can reduce its sensitivity to memory coherence time [2], leading to significant improvements in storage capacity [3]. It is thus no surprise that many research groups are actively working on different physical systems for storing light encoded using a high-dimensional space. The degrees of freedom for position, linear momentum, time-bin or orbital angular momentum (OAM) of a photon can all be considered as a high-dimensional space for encoding. The photon's OAM has the most potential for encoding [4]. Electromagnetic waves have both spin and OAM. Spin angular momentum produces polarization. Photons with OAM can be regarded as helices with left and right handedness twisted to varying degrees (Fig. 1). Information is encoded using this handedness and the amount of twist. Because of the inherent infinite degrees of freedom for OAM, a photon can in principle carry an arbitrarily large amount of information, and hence the eagerness to store light encoded in OAM space. Although some work on this has been reported for different physical systems, what is lacking is a way of storing and releasing at some later time a true single photon, including its shape and structure [5–7]. Constructing this basic element of quantum memory has been a major challenge. The wavefront of an OAM light is a helical structure (left and center), with an optical vortex at its center in the intensity distribution of light (right). The vortex of light can carry non-zero OAM of any order m. OAM states of a different order are orthogonal. A group at the Key Laboratory of Quantum Information, Chinese Academy of Science, at the University of Science and Technology of China finally resolved this problem [8]. They reported on the first experimental realization of a true single-photon-carrying OAM stored via electromagnetically induced transparency (EIT) in a cold atomic ensemble (Fig. 2). With such a suitable candidate, this work indicates a means of constructing high-dimensional quantum memory. After this, similar results were reported by Laurat's group at Laboratoire Kastler Brossel, at Université Pierre et Marie Curie in France [9], where an extremely weak laser at single-photon level carrying OAM was also stored via EIT in a cold atomic ensemble. Ding et al. [8] first prepared two cold 85Rb atomic clouds in two magnetic-optical traps (MOT) using laser cooling and trapping techniques. They generated non-classical correlated photon pairs using spontaneous four-wave mixing in an atomic cloud. One photon of each pair was used as a trigger; the other mapped and stored in a second atomic cloud via EIT. Each photon to be stored carried one OAM unit. After a programed storage time, the photon was retrieved. What they achieved during storage included (1) proof that the non-classical correlation between the trigger photon and the retrieved photon is retained by demonstrating a strong violation of the Cauchy–Schwarz inequality, (2) a demonstration that the single-photon property of the signal photon is maintained by performing the Hanbury–Brown and Twiss experiment on the trigger photon, (3) proof that the spatial structure of the photon is also very well preserved by showing a high similarity between input and output, and (4) evidence, gathered by Sagnac interferometry, that the coherence of a single photon is also preserved. A heralded single photon is generated through spontaneous four-wave mixing in MOT 1 (a); this single photon carrying OAM is then stored through EIT in MOT 2 (b); (c) shows an image of the photon carrying OAM. Experimental measurements in the transverse position of the image carried by the photon before and after storage are presented in (d) and (e), respectively; (f) shows the simplified experimental setup for storage of a superposition of OAM. Interference patterns taken at different angle settings of the half-wave plate are shown in (g). The left column represents the experimental angle settings of the half-wave and the quarter-wave plates, the middle column gives the experimental results, and the right column gives results from theoretical simulations; (h) and (i) present the interference patterns of the input signal photon and the retrieved signal with plate angle, respectively. This is a significant breakthrough towards the realization of a quantum internet and, potentially, quantum computing. This work addresses the ability to generate, store, retrieve on demand an arbitrary single-photon-level photonic state encoded in OAM space. It signifies an important step in the development of practical quantum-enabled technologies, opens up the possibility for realizing high-dimensional quantum memories based on this degree of freedom of light, and will have a large impact in a broad physical community, especially in the quantum information and quantum optics communities. The Technology Review website of MIT comments on their work very positively with an article entitled ‘First Quantum Memory That Records the Shape of a Single Photon Unveiled in China’. Further, Nature Photonics selected this work as a research highlight. Clearly, memory that can preserve the spatial structure of photons will make the internet far more flexible and capable. Of course, there are still many basic problems remaining that need to be solved to build the future quantum internet, one of which is the construction of quantum memory exploiting entanglement. This derives from the fact that a quantum network needs the distribution of quantum-entangled photons over channels between different nodes [10]. A high-dimensional quantum internet needs to store OAM-entangled states and perform entanglement swapping to efficiently extend the achievable communication distances. While Ding et al. [8] reported the storage of light with OAM at the single-photon level, the photon was, however, still encoded in a 2D space. Therefore, whether it is possible to construct a high-dimensional quantum memory remains an open issue that needs to be investigated further.
Light facilitates exploration of quantum phenomena that illuminate the basic properties of nature and also enables radical new technologies based on these phenomena. The critical features of quantum light that underpin the opportunities for discovery and application are exceptionally low noise and strong correlations. Rapid progress in both science and technology has been stimulated by adopting components developed for optical telecommunications and networking, such as highly efficient detectors, integrated photonic circuits, and waveguide- or nanostructure-based nonlinear optical devices. These provide the means to generate new quantum states of light and matter of unprecedented scale, containing many photons with quantum correlations across space and time. Notably, networks with only several tens of photons are already beyond what can be efficiently analyzed by current computers.