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Physical Review A

Laser-detected magnetic resonance induced by radio-frequency two-photon processes

Xu‐xing Geng, Guoqing Yang, Pan-li Qi, Wangwang Tang, Shangqing Liang, Gao‐xiang Li, Guangming Huang

Published May 17, 2021• 16 citations
Publisher

Abstract

We have theoretically and experimentally investigated the laser-detected magnetic resonance induced by radio-frequency two-photon processes in ${F}_{g}=4$ of ${D}_{1}$ line of cesium atoms. The effective Hamiltonian for the interaction between the two radio-frequency magnetic fields and sublevels at the ground state of ${F}_{g}=4$ is derived. By appropriately selecting the frequencies of the two radio-frequency fields, the Raman two-photon process and the cascade two-photon process can occur, which induce the magnetic resonance detected through laser transmission spectra. The theoretical calculation results fit well with the experimental data. Our results maybe apply for measuring the high bandwidth radio-frequency magnetic fields in space and studying the magnetic-induction tomography.

DOI
10.1103/physreva.103.053112

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We have theoretically and experimentally investigated the laser-detected magnetic resonance induced by radio-frequency two-photon processes in Fg=4{F}_{g}=4Fg​=4 of D1{D}_{1}D1​ line of cesium atoms. The effective Hamiltonian for the interaction between the two radio-frequency magnetic fields and sublevels at the ground state of Fg=4{F}_{g}=4Fg​=4 is derived. By appropriately selecting the frequencies of the two radio-frequency fields, the Raman two-photon process and the cascade two-photon process can occur, which induce the magnetic resonance detected through laser transmission spectra. The theoretical calculation results fit well with the experimental data. Our results maybe apply for measuring the high bandwidth radio-frequency magnetic fields in space and studying the magnetic-induction tomography.
We theoretically and experimentally investigate the laser-detected magnetic resonance spectra dressed by a radio-frequency magnetic field in F g = 4 of D1 line of cesium atoms. The analytical expression of the transmission spectrum for magnetic resonance dressed by a radio-frequency magnetic field is derived and has substantial agreement with the transmission spectra observed in the experiment. The theoretical prediction of the ratio of the amplitudes of the two sidebands with the detuning is basically consistent with the experimental data, which confirms the validity of the analytical expression. The separation between the two sidebands under resonance shows a highly linear proportion to the amplitude of the dressing field, which may provide a useful scheme for the measurement of radio-frequency magnetic field and magnetic imaging.
We report an experimental study on the ground-state magnetic resonances of optically pumped cesium vapors at lower temperatures of about 30°C–40°C. A longitudinal static magnetic field is applied along the single laser beam to control the splitting of the Zeeman sublevels of the ground state. When the laser frequency is set to the cesium D1 spectral line (F=3→F′=4), by modifying the transverse radio frequency field, we find that the unusual weaker-absorption and zero-dip resonance phenomena occur in the optical-magnetic resonance (OMR) effects, which is called the cesium optical-RF resonance line reversals and doubling in this paper. We explore a theoretical description for these phenomena by using density matrix equations, and our calculated results are in approximate agreement with the experimental results.
Abstract We have observed the Autler–Townes (AT) effect in single- and suspected double-photon magnetic-dipole transitions in the Cesium ground-state magnetic-sublevel manifold. Experiments were performed in a Cesium vapor cell at room temperature. The D1 line was excited by laser radiation to create ground-state optical polarization, and transitions between the ground-state magnetic sublevels were excited by radio-frequency (RF) radiation. Two different excitation geometries were studied: in one case the electric field vector of the linearly polarized laser radiation was parallel to the static magnetic field, whereas in the other case these vectors were perpendicular. The oscillating magnetic field produced by the RF coils was in the plane perpendicular to the electric field vector of the laser radiation. The AT effect was confirmed by its linear dependence on the RF magnetic field amplitude, which is proportional to the Rabi frequency, in the case of single-photon transitions. With increasing RF power we also observed peaks that by their position appeared to correspond to double and even triple photon transitions, which were more pronounced when the DC magnetic field and optical electric field vectors were perpendicular. In the peak at an energy that corresponds to two photons, splitting with a quadratic dependence on the RF magnetic field amplitude could be observed. The experimental measurements are supplemented by theoretical calculations of a model J = 1 ⟶ J = 0 system.
We present an experimental study of the spectra produced by optical--radio-frequency double resonance in which resonant linearly polarized laser light is used in the optical pumping and detection processes. We show that the experimental spectra obtained for cesium are in excellent agreement with a very general theoretical model developed in our group [Weis, Bison, and Pazgalev, Phys. Rev. A 74, 033401 (2006)] and we investigate the limitations of this model. Finally, the results are discussed in view of their use in the study of relaxation processes in aligned alkali-metal vapors.
A novel coherent Raman effect induced by a laser and a radio-frequency (rf) field is used to detect cw and pulsed nuclear magnetic resonance (NMR) in ground and excited electronic states. The effect is illustrated in the impurity-ion solid Pr3+{\mathrm{Pr}}^{3+}Pr3+: LaF3{\mathrm{F}}_{3}F3​ at 1.6 K utilizing the Pr3+{\mathrm{Pr}}^{3+}Pr3+ optical transition $^{3}H_{4}({\ensuremath{\Gamma}}_{1})\ensuremath{\rightarrow}^{1}D_{2}({\ensuremath{\Gamma}}_{1})$. The laser field of frequency ${\ensuremath{\omega}}_{E}$ and the rf field (${\ensuremath{\omega}}_{H}$) induce a light wave at the sum ${\ensuremath{\omega}}_{E}+{\ensuremath{\omega}}_{H}$ (anti-Stokes) and difference ${\ensuremath{\omega}}_{E}\ensuremath{-}{\ensuremath{\omega}}_{H}$ (Stokes) frequencies, generating an absorptive or dispersive heterodyne beat signal (${\ensuremath{\omega}}_{H}$) with the laser field at a photodetector. The theory of this effect is characterized in a new three-level perturbation calculation which requires, unlike the usual stimulated Raman effect, that all three transitions be electric- or magnetic-dipole allowed. Detailed predictions are confirmed by cw measurements of the Pr3+{\mathrm{Pr}}^{3+}Pr3+: LaF3{\mathrm{F}}_{3}F3​ hyperfine splittings where the optical heterodyne signals are shot-noise limited. The Pr3+{\mathrm{Pr}}^{3+}Pr3+ nuclear quadrupole parameters are obtained for the 3H4^{3}H_{4}3H4​ and 1D2^{1}D_{2}1D2​ states where the line centers are determined with kilohertz precision. The corresponding wave functions show significant hyperfine-state mixing, as required for all three transitions to be dipole allowed. The cw line shapes are narrow (30-160 kHz), inhomogeneously broadened by nuclear magnetic interactions, and reveal either a Gaussian or an anomalous second-derivative---like line shape. The spin-echo measurements for the 3H4^{3}H_{4}3H4​ and 1D2^{1}D_{2}1D2​ hyperfine transitions yield homogeneous line shapes which are Lorentzian, and rather surprisingly, linewidths in the narrow range 10-20 kHz, a result which tests current line-broadening theories.
Theoretical study and computer modeling results of the spectra of coherent dark resonances resulted from excitation of Zeeman sublevels of the Fg=2→Fe=1 transition of the D1 line in 87Rb atoms by a frequency-modulated laser field are presented and discussed in detail. The influence of the nonlinear Zeeman effect on the structure of the coherent dark resonances is observed. It is shown that calculated for different values of the magnetic field spectra are in a good agreement with the experimental data.