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Excitation of Atoms by Twisted Light

S. A.-L. Schulz

Published Aug 25, 2020• 0 citations
Publisher

Abstract

Twisted light has received a lot of attention in recent years. And there are justified reasons for this. The properties of twisted light are unusual and differ fundamentally from the plane-wave properties. The phase fronts of these light beams have a helical structure, giving them the name twisted. This helical phase structure originates from the well-defined orbital angular momentum (OAM) that they carry along their propagation direction and in addition to the spin angular momentum (SAM). Moreover, they have a characteristic intensity profile, which consists of concentric rings with a central minimum, and a phase singularity in the beam center. This thesis is based on two main parts, each dealing with a different aspect of twisted light. These investigations are carried out using Bessel beams, one type of twisted light. Twisted light beams are cylindrically symmetrical. Therefore, they are defined on the basis of circularly polarized light. This fact leads to the first question: Is it possible to generate twisted light in other polarization states? In this work, we derive how this can be achieved by using the superposition principle and how this can be used to construct linearly, radially, or azimuthally polarized Bessel beams. The focus in the second part is on excitations of atoms by twisted Bessel beams. In particular, we analyze how the use of twisted light can modify individual atomic multipole transitions. The obtained results show that for an efficient modification a precise localization of the target atom is required. In the last chapter, both aspects are combined. We analyze transitions between magnetic hyperfine states in a single trapped atom (or ion), which is exposed to an additional external magnetic field. The presented calculations for these multipole excitations are based on a formalism that accounts for the alignment of the applied external magnetic field with respect to the light propagation direction, and additionally different polarization states of the radiation field are considered. The obtained results indicate that twisted light could be of particular interest for precision experiments. One possible application is the use in single-ion clocks. The work shows that high multipole orders of the vortex beams allow excitations in the intensity minimum in the center of these beams without causing large disturbances, and thus may enable a significant reduction of the light shift in atomic transitions.

DOI
10.24355/dbbs.084-202008251545-0

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Twisted light has received a lot of attention in recent years. And there are justified reasons for this. The properties of twisted light are unusual and differ fundamentally from the plane-wave properties. The phase fronts of these light beams have a helical structure, giving them the name twisted. This helical phase structure originates from the well-defined orbital angular momentum (OAM) that they carry along their propagation direction and in addition to the spin angular momentum (SAM). Moreover, they have a characteristic intensity profile, which consists of concentric rings with a central minimum, and a phase singularity in the beam center. This thesis is based on two main parts, each dealing with a different aspect of twisted light. These investigations are carried out using Bessel beams, one type of twisted light. Twisted light beams are cylindrically symmetrical. Therefore, they are defined on the basis of circularly polarized light. This fact leads to the first question: Is it possible to generate twisted light in other polarization states? In this work, we derive how this can be achieved by using the superposition principle and how this can be used to construct linearly, radially, or azimuthally polarized Bessel beams. The focus in the second part is on excitations of atoms by twisted Bessel beams. In particular, we analyze how the use of twisted light can modify individual atomic multipole transitions. The obtained results show that for an efficient modification a precise localization of the target atom is required. In the last chapter, both aspects are combined. We analyze transitions between magnetic hyperfine states in a single trapped atom (or ion), which is exposed to an additional external magnetic field. The presented calculations for these multipole excitations are based on a formalism that accounts for the alignment of the applied external magnetic field with respect to the light propagation direction, and additionally different polarization states of the radiation field are considered. The obtained results indicate that twisted light could be of particular interest for precision experiments. One possible application is the use in single-ion clocks. The work shows that high multipole orders of the vortex beams allow excitations in the intensity minimum in the center of these beams without causing large disturbances, and thus may enable a significant reduction of the light shift in atomic transitions.
Synopsis In this work, we present how the AC-Stark shift can be suppressed by using twisted light beams for photoexcitations. Twisted light beams carry a non-zero projection of orbital angular momentum (OAM) onto their propagation direction, have a helical phase front and an intensity minimum in the beam center. Atoms located in this minimum experience a reduced AC-Stark shift and, therefore, twisted beams may be considered as valuable tool to drive atomic clock transitions. In this contribution, particular emphasis is paid to the electric-octupole (E3) transition 2 S1/2 → 2 F7/2 in the 171 Yb+ ion.
In this paper we analyze the novel quantum properties of atomic photo-excitations generated by Orbital Angular Momentum (OAM) photons. It was previously predicted for Bessel beams (BB), that transitionsin atomic systems driven by twisted laser beams obey a modified set of position-dependent angular-momentum selection rules. It was also shown, that in the case of perfect alignment of the atom on the beam axis, total angular momentum of the photon must be fully transferred to the internal degrees of freedom of the target, which causes dramatic enhancement of higher-multipole processes. As a result, weak atomic transitions, which are hardly observable in interactions with simple states of light, become accessible with OAM photons. In the current paper, we extend the earlier developed theory to describe atomic photoexcitations by Bessel-Gauss (BG) and Laguerre-Gauss (LG) modes. It allowed us to infer the information about the phase structure of the beam, such as mode content and topological charge. The formalism exhibits a high level of sensitivity to the polarization content of the laser beam, which is on the order of 0.005% of the polarization admixture. The theoretical predictions are confirmed experimentally for photo-excitation of Ca40+ ions, trapped in a micro-structured, segmented Paul trap. The full set of quadrupole transitions from the S-state were generated by 729nm OAM laser beam shaped with a holographic phase-plate with a fork-dislocation. The experiment was conducted by Ferdinand Schmidt-Kaler's group at the University of Mainz.
A theoretical study is performed for the excitation of a single atom localized in the center of twisted light modes. Here we present the explicit dependence of excitation rates on critical parameters, such as the polarization of light, its orbital angular momentum projection, and the orientation of its propagation axis with respect to the atomic quantization axis. The effect of a spatial spread of the atom is also considered in detail. The expressions for transition rates obtained in this work can be used for any atom of arbitrary electronic configuration. For definiteness we apply them to the specific case of the $^{2}S_{1/2}(F=0)\ensuremath{\rightarrow}^{2}F_{7/2}(F=3,M=0)$ electric octupole (E3) transition in 171Yb+{^{171}\mathrm{Yb}}^{+}171Yb+ ion. Our analytical and numerical results are suitable for the analysis and planning of future experiments on the excitation of electric-dipole-forbidden transitions by twisted light modes in optical atomic clocks.
In 1992, Les Allen and coworkers within Han Woerdman's group realized that light beams with an azimuthal phase dependence described by an additional exp(iℓθ) term, where ℓ can take any integer value and θ is the angular position within the beam, carry an orbital angular momentum. This orbital angular momentum is additional to the spin angular momentum associated with circular polarization. These azimuthally phased beams comprise ℓ intertwined helical phase fronts, skewed with respect to the beam axis, meaning that at all positions within the beam cross section, the wavefront normal and associated momentum density has a well-defined azimuthal component. The insight of Allen and coworkers was that for all beams described in this way, when integrated over the beam cross section, the orbital angular momentum (OAM) is ℓℏ per photon. Laguerre-Gaussian and high-order Bessel beams are both examples of mode families having these properties. A further feature of these beams is that the phase singularity on the beam axis precludes a nonzero on-axis intensity and therefore all such beams with ℓ ≠0 have an annular intensity cross section (see Fig. 4.1). The circulation of the optical momentum and energy around the singularity leads them also to be called optical vortices. The further recognition that beams carrying defined amounts of OAM could be created within the laboratory means that over the last 15 years they have formed the basis of many investigations, ranging from the transfer of OAM to microscopic particles (in optical spanners or optical wrenches) to studies of the fundamental properties of light in both the classical and quantum regimes. However, although OAM is an immensely useful concept, one must emphasize that all its properties are simply those predicted by standard electromagnetic theory. The purpose of this chapter is to consider how sets of helical laser modes carrying OAM can be used for information transfer.
A form of quantum control is proposed by applying twisted light, also known as optical vortex beams, to drive ultranarrow atomic transitions in neutral Ca, Mg, Yb, Sr, Hg, and Cd bosonic isotopes. This innovative all-optical spectroscopic method introduces spatially tailored electric and magnetic fields to fully rewrite atomic selection rules, reducing simultaneously probe-induced frequency shifts and additional action of external ac and dc field distortions. A twisted-light focused probe beam produces strong longitudinal electric and magnetic fields along the laser propagation axis, which opens the $^{1}S_{0}\ensuremath{\rightarrow}^{3}P_{0}$ doubly forbidden clock transition with a high E1M1E1M1E1M1 two-photon excitation rate. This long-lived clock transition is thus immune to nonscalar electromagnetic perturbations. Zeeman components of the M2M2M2 magnetic quadrupole $^{1}S_{0}\ensuremath{\rightarrow}^{3}P_{2}$ transition considered for quantum computation and simulation are now selectively driven by transverse or longitudinal field gradients with vanishing electric fields. These field gradients are manipulated by the mutual action of orbital and spin angular momentum of the light beam and are used in presence of tunable vector and tensor polarizabilities. A combination of these two different twisted-light induced clock transitions within a single quantum system, at the same magic wavelength and in presence of a common thermal environment, significantly reduces systematic uncertainties. Furthermore, it generates an optical synthetic frequency which efficiently limits the blackbody radiation shift and its variations at room temperature. Engineering light-matter interaction by optical vortices merged with composite pulses will ultimately benefit experimental atomic and molecular platforms targeting an optimal coherent control of quantum states, reliant quantum simulation, novel approaches to atomic interferometry, and precision tests of fundamental theories in physics and high-accuracy optical metrology.
Theoretical work has already established the existence of a light-induced torque acting on the centre of mass of an atom, ion or molecule immersed in twisted light, where the transition frequency is suitably detuned from that of the twisted light beam. The twisted beam carries l units of orbital angular momentum per photon, and the steady-state saturation form of the torque is also determined by the width of the upper state in the atomic transition. It has been shown that, to leading order, the transfer of orbital angular momentum can only occur between the twisted light and the centre of mass motion. We argue here that, for small linewidth, the full time-dependence of the torque is needed to account correctly for the dynamics of atoms in a twisted light beam. We outline the theoretical framework needed to derive this full time-dependence, applying the theory to the motion in a twisted light beam of Eu3+ ions, which possess a particularly narrow linewidth state. For relatively large linewidth, the steady-state forces and torque are appropriate, but the processes of cooling and trapping require the application of several suitably oriented twisted beams. The description of atomic motion in multiple twisted beams demands the application of special coordinate transformations. We show how to construct the appropriate transformation matrices to represent a twisted light beam propagating in an arbitrary direction, and we proceed to investigate the cooling and trapping of Mg+ ions in sets of pairs of counter-propagating twisted beams in two-dimensional and three-dimensional molasses configurations.