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Advanced Photon Counting Techniques

Mid-infrared two-photon interference and polarization entanglement

Taylor Shields, Adetunmise C. Dada, Shashi Prabhakar, Mehdi Haji Ebrahim, Gregor G. Taylor, D. Morozov, Kleanthis Erotokritou, Shigehito Miki, Masahiro Yabuno, Hirotaka Terai, Corin B. E. Gawith, Robert H. Hadfield, Matteo Clerici, Lucia Caspani, Michael Kues

Published Apr 8, 2021• 0 citations
Publisher

Abstract

Quantum-enhanced optical technologies operating within the 2- to 2.5-μm spectral region have the potential to revolutionize emerging applications in communications, sensing, and metrology. Currently, sources of entangled photons are available at visible, near-infrared and telecom wavelengths but are strongly underdeveloped at longer wavelengths. Here, using custom-designed lithium niobate crystals for spontaneous parametric down-conversion and tailored superconducting nanowire single-photon detectors, we demonstrate two-photon interference and polarization-entangled photon pairs at 2090 nm. These results open the 2- to 2.5-μm mid-infrared window for the development of optical quantum technologies such as quantum key distribution in next-generation mid-infrared fiber communication systems and future Earth-to-satellite communications.

DOI
10.1117/12.2588340

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Quantum-enhanced optical technologies operating within the 2- to 2.5-μm spectral region have the potential to revolutionize emerging applications in communications, sensing, and metrology. Currently, sources of entangled photons are available at visible, near-infrared and telecom wavelengths but are strongly underdeveloped at longer wavelengths. Here, using custom-designed lithium niobate crystals for spontaneous parametric down-conversion and tailored superconducting nanowire single-photon detectors, we demonstrate two-photon interference and polarization-entangled photon pairs at 2090 nm. These results open the 2- to 2.5-μm mid-infrared window for the development of optical quantum technologies such as quantum key distribution in next-generation mid-infrared fiber communication systems and future Earth-to-satellite communications.
Quantum-enhanced optical systems operating within the 2- to 2.5-μm spectral region have the potential to revolutionize emerging applications in communications, sensing, and metrology. However, to date, sources of entangled photons have been realized mainly in the near-infrared 700- to 1550-nm spectral window. Here, using custom-designed lithium niobate crystals for spontaneous parametric down-conversion and tailored superconducting nanowire single-photon detectors, we demonstrate two-photon interference and polarization-entangled photon pairs at 2090 nm. These results open the 2- to 2.5-μm mid-infrared window for the development of optical quantum technologies such as quantum key distribution in next-generation mid-infrared fiber communication systems and future Earth-to-satellite communications.
Quantum-enhanced optical systems operating within the 2-2.5 µm spectral region have the potential to revolutionize emerging applications in communications, sensing and metrology. However, until now, sources of entangled photons have been realized mainly in the near-infrared 700-1550 nm spectral window. Above 2 µm lies an atmospheric transparency window with nearly one-third of the solar blackbody radiation as what is typical at telecom wavelengths. There is, therefore, a growing interest to deliver sources and detectors operating in this wavelength range for free-space optical communications and in emerging fields of high-sensitivity metrology, specifically, gravitational wave detection [1,2]. Here, using a 130 fs pulsed laser at wavelength 1.05 μm to pump custom-designed non-linear crystals for spontaneous parametric down-conversion (SPDC) process and tailored superconducting nanowire single-photon detectors (SNSPD), we demonstrate for the first-time two-photon quantum interference and polarization entanglement in the mid-infrared, at ≃ 2.1 μm.
Single-photon counting has become an essential tool in quantum optics experiments, as well as remote sensing and life science applications. However conventional technologies such as single-photon avalanche diodes, as well as the availability of standard telecom optical components, has limited much of this work to the near infrared/telecom wavelength range. Superconducting nanowire single photon detectors (SNSPDs) have emerged in recent years as the gold standard in photon counting applications due to their low dark count rates, fast timing resolution and high efficiency [1]. SNSPDs have also demonstrated photon counting efficiency out to much greater wavelengths which enables us to explore new experimental possibilities in the mid-infrared [2]. In this work we design and fabricate mid-infrared SNSPDs and deploy them in a variety of photon counting experiments [3,4]. The devices are based on a NbTiN superconducting film integrated into an optical cavity to enhance absorption in the mid-infrared. We characterise these devices using an optical parametric oscillator, tuneable between 1.5 m and 4.2 m. We then deploy these in a proof-of-principle tabletop light detection and ranging (LIDAR) experiment at 2.3 m. LIDAR in the mid-infrared is attractive due to spectral regions of low atmospheric absorption and reduced solar background photon flux, when compared to telecom wavelengths. We also present results from a photon-pair source operating at 2 m. This is a key resource for extending quantum optics and quantum secure communications to the mid infrared domain. Pairs are generated using a custom lithium niobate crystal and detected using SNSPDs. We demonstrate two-photon interference and polarisation entanglement of the photon pairs at 2 m. This work opens the pathway to future development of quantum optics and quantum technologies in the mid-infrared spectral region. References [1] Gol’tsman et al Applied Physics Letters 79 705 (2001) [2] Marisli et al Nano Letters 12 (9) 4799 (2012) [3] G. G. Taylor et al Optics Express 26 (27) 38147 (2018) [4] S. Prabhakar et al Science Advances 6 (13) eaay5195 (2019)
Given the important advantages of the mid-infrared optical range (2.5 to 25 μm) for biomedical sensing, optical communications, and molecular spectroscopy, extending quantum information technology to this region is highly attractive. However, the development of mid-infrared quantum information technology is still in its infancy. Here, we report on the generation of a time-energy entangled photon pair in the mid-infrared wavelength band. By using frequency upconversion detection technology, we observe the two-photon Hong-Ou-Mandel interference and demonstrate the time-energy entanglement between twin photons at 3082 nm via the Franson-type interferometer, verifying the indistinguishability and nonlocality of the photons. This work is very promising for future applications of optical quantum technology in the mid-infrared band, which will bring more opportunities in the fields of quantum communication, precision sensing, and imaging.
The mid-infrared (MIR) band entangled photon source is vital for the next generation of quantum communication, quantum imaging, and quantum sensing. However, the current entangled states are mainly prepared in the visible or near-infrared bands. It is still lacking high-quality entangled photon sources in the MIR band. In this work, we optimize the poling sequence of lithium niobate to prepare two kinds of typical entangled states, the Hermit–Gaussian state and the comb-like entangled state at 3.2 µm. We have also calculated the photon pair rates and estimated the effect of fabrication resolution in the schemes. Our approach will provide entangled photon sources with excellent performance for the study of quantum information in the MIR band.
Quantum entanglement is a fundamental resource for emerging quantum technologies, enabling secure communication and enhanced sensing. For decades, generating polarization entangled states has been mainly achieved using bulk crystals with spontaneous parametric down conversion (SPDC), preventing scalability and on-chip integration. Miniaturizing the quantum source provides access to more versatility and tunability while enabling an easier integration to other devices, notably necessary for satellite-based quantum communication, and eventually reducing fabrication costs. This challenging task can be achieved with Zinc Blende GaAs nanowires. They already have shown an efficient photon pairs generation via SPDC at 1550 nm. Here we demonstrate that a pair of orthogonal GaAs nanowires constitutes a new nanoscale platform to control the quantum state at telecommunication wavelength, enabling a transition from polarization entangled to separable states as a function of the pump polarization, with fidelities reaching 90%