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The Japan Society of Applied Physics

Broadband generation of infrared quantum entangled-photon pairs via simultaneous parametric down-conversion

Masayuki Hojo, Kōichiro Tanaka

Published Jan 26, 2021• 0 citations
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Spontaneous parametric down-conversion is an essential tool for a quantum light source in the infrared region ranging 2-5 µm for the purpose of material identification, chemical analysis, and gas sensing. So far, photon pairs from the process in a nonlinear crystal have low tunability and a narrow spectral range because of the phase-matching condition. Here, we propose a novel type of spontaneous parametric down-conversion processes that overcomes these challenges, where two photon pairs are simultaneously produced in the visible and infrared regions in periodically poled stoichiometric lithium tantalite. It allows broadband and tunable generation of infrared photon pairs that can be employed as an alternative light source for quantum infrared spectroscopy.

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Abstract Nonlinear interferometry with entangled photons allows for characterizing a sample without detecting the photons interacting with it. This method enables highly sensitive optical sensing in the wavelength regions where efficient detectors are still under development. Recently, nonlinear interferometry has been applied to interferometric measurement techniques with broadband light sources, such as Fourier‐transform infrared spectroscopy and infrared optical coherence tomography. However, they have been demonstrated with photon pairs produced through spontaneous parametric down‐conversion (SPDC) at a low parametric gain, where the average number of photons per mode is much smaller than one. The regime of high‐gain SPDC offers several important advantages, such as the amplification of light after its interaction with the sample and a large number of photons per mode at the interferometer output. This work presents broadband spectroscopy and high‐resolution optical coherence tomography with undetected photons generated via high‐gain SPDC in an aperiodically poled lithium niobate crystal. To prove the principle, reflective Fourier‐transform near‐infrared spectroscopy with a spectral bandwidth of 17 THz and optical coherence tomography with an axial resolution of 11 µm are demonstrated.

arXiv:2309.08218•Advanced Quantum Technologies•Dec 24, 2023•16 citations
Spontaneous parametric down-conversion is an essential tool for a quantum light source in the infrared region ranging 2-5 µm for the purpose of material identification, chemical analysis, and gas sensing. So far, photon pairs from the process in a nonlinear crystal have low tunability and a narrow spectral range because of the phase-matching condition. Here, we propose a novel type of spontaneous parametric down-conversion processes that overcomes these challenges, where two photon pairs are simultaneously produced in the visible and infrared regions in periodically poled stoichiometric lithium tantalite. It allows broadband and tunable generation of infrared photon pairs that can be employed as an alternative light source for quantum infrared spectroscopy.
Broadband photon-pairs from a parametric down-conversion (PDC) source are essential for quantum optics experiments in the context of spectroscopy, quantum optical coherence tomography and entangled two-photon absorption [1]–[2]. Entangled two-photon absorption benefits from the ultra-short correlation time of a highly time-frequency entangled photon-pair which increases the absorption cross-section while in spectroscopy, broad spectral coverage in the mid-infrared allows one to enter the regime of life science applications.
Abstract Nonlinear interferometry with entangled photons allows for characterizing a sample without detecting the photons interacting with it. This method enables highly sensitive optical sensing in the wavelength regions where efficient detectors are still under development. Recently, nonlinear interferometry has been applied to interferometric measurement techniques with broadband light sources, such as Fourier‐transform infrared spectroscopy and infrared optical coherence tomography. However, they have been demonstrated with photon pairs produced through spontaneous parametric down‐conversion (SPDC) at a low parametric gain, where the average number of photons per mode is much smaller than one. The regime of high‐gain SPDC offers several important advantages, such as the amplification of light after its interaction with the sample and a large number of photons per mode at the interferometer output. This work presents broadband spectroscopy and high‐resolution optical coherence tomography with undetected photons generated via high‐gain SPDC in an aperiodically poled lithium niobate crystal. To prove the principle, reflective Fourier‐transform near‐infrared spectroscopy with a spectral bandwidth of 17 THz and optical coherence tomography with an axial resolution of 11 µm are demonstrated.