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Observation of nonlocal quantum interference between the origins of a four-photon state in a silicon chip

Lan‐Tian Feng, Ming Zhang, Di Liu, Yujie Cheng, Guo‐Ping Guo, Daoxin Dai A, Guang‐Can Guo, Mario Krenn, Xi‐Feng Ren

Published Mar 26, 2021• 4 citations
OpenAlex

Abstract

Quantum mechanically, multiple particles can jointly be in a coherent superposition of two or more different states at the same time. This property is called quantum entanglement, and gives rise to characteristic nonlocal interference and stays at the heart of quantum information process. Here, rather than interference of different intrinsic properties of particles, we experimentally demonstrated coherent superposition of two different birthplaces of a four-photon state. The quantum state is created in four probabilistic photon-pair sources, two combinations of which can create photon quadruplets. Coherent elimination and revival of distributed 4-photons can be fully controlled by tuning a phase. The stringent coherence requirements are met by using a silicon-based integrated photonic chip that contains four spiral waveguides for producing photon pairs via spontaneous four-wave mixing. The experiment gives rise to peculiar nonlocal phenomena without any obvious involvement of entanglement. Besides several potential applications that exploit the new on-chip technology, it opens up the possibility for fundamental studies on nonlocality with spatially separated locations.

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Quantum mechanically, multiple particles can jointly be in a coherent superposition of two or more different states at the same time. This property is called quantum entanglement, and gives rise to characteristic nonlocal interference and stays at the heart of quantum information process. Here, rather than interference of different intrinsic properties of particles, we experimentally demonstrated coherent superposition of two different birthplaces of a four-photon state. The quantum state is created in four probabilistic photon-pair sources, two combinations of which can create photon quadruplets. Coherent elimination and revival of distributed 4-photons can be fully controlled by tuning a phase. The stringent coherence requirements are met by using a silicon-based integrated photonic chip that contains four spiral waveguides for producing photon pairs via spontaneous four-wave mixing. The experiment gives rise to peculiar nonlocal phenomena without any obvious involvement of entanglement. Besides several potential applications that exploit the new on-chip technology, it opens up the possibility for fundamental studies on nonlocality with spatially separated locations.
There has been broad interest in path identity in recent years due to its role as a foundation for numerous novel quantum information applications. Here, we experimentally demonstrate quantum coherent superposition of two different origins of a four-photon state, where multi-photon frustrated interference emerges from the quantum indistinguishability by path identity. The quantum state is created in four probabilistic photon-pair sources on one integrated silicon photonic chip, two combinations of which can create photon quadruplets. Coherent elimination and revival of the distributed four photons are fully controlled by tuning phases. The experiment gives rise to peculiar quantum interference of two possible ways to create photon quadruplets rather than interference of different intrinsic properties of photons. Besides many known potential applications, this kind of multi-photon nonlinear interference enables the possibility for various fundamental studies such as nonlocality with multiple spatially separated locations.
Quantum interference between identical photons lies at the heart of our plan to construct a silicon photonic quantum computer. Several ground-breaking experiments have demonstrated the on-chip interference between photons generated in spiral [1] and ring resonator [2] sources. However, these two-photon experiments have relied on detecting the simultaneous arrival of a pair of photons from either source. In order that such experiments can be scaled-up, we require the multiplexing of probabilistic photon pair sources into an on-demand single photon source [3]. A first step towards this is to demonstrate heralded single photons from different sources will retain the purity and indistinguishability required to interfere with high visibility [4]. In our work we examine photon pair production by spontaneous four-wave mixing in a silicon waveguide source and determine the factors that limit the heralded two-photon interference visibility. We present a novel approach to modelling this generation process using the joint- temporal amplitude and compare our results with experimental data. [1] On-chip quantum interference between silicon photon-pair sources, Nature Photonics 8, 104, (2014). [2] Qubit entanglement between ring-resonator photon-pair sources on a silicon chip, Nature Communications 6, 7948, (2015). [3] Active temporal and spatial multiplexing of photons, Optica 3, 127, (2016) [4] Indistinguishable photon pair generation using two independent silicon wire waveguides, New Journal of Physics 13, 065005, (2011).
Photonic integrated circuits represent a promising platform for applying quantum information science to areas such as quantum computation, quantum communication, and quantum metrology. While the linear optical approach has greatly contributed to this field, it is often possible to improve the functionality and scalability by making use of nonlinear processes. One interesting phenomenon is the interference between two nonlinear optical processes, where the interference occurs by removing the information as to which of two processes have occurred. In this Letter, we demonstrate a nonlinear interferometer in the pair-photon generation regime by using spontaneous four-wave mixing in an integrated silicon photonic chip. We observe a nonlinear interference in the production rate of photon pairs generated from two different four-wave mixing waveguides. We obtain an interference visibility of 96.8%. This work shows the possibility of integrating and controlling nonlinear-optical-interference components for silicon quantum photonics.
Optical nonlinearity provides a key resource for quantum information processing and the interference of quanta lies at the heart of quantum physics as well. As an interesting combination, the nonlinear interference can extend the scalability and flexibility of quantum manipulations as well as what we believe to be novel applications. In this manuscript, we propose and experimentally demonstrate what we believe to be a new nonlinear interferometer on a silicon chip between a degenerate and a non-degenerate spontaneous four-wave mixing process in the same waveguide. We observed the interference in the pairs generation rate and obtained broadband interference visibility up to 96%. Furthermore, we also provide a feasible scheme for observing four-photon nonlinear interference in a single waveguide. This work provides a novel method for realizing and controlling optical nonlinear interference, and enriches the toolbox of quantum state preparation and quantum manipulation by nonlinear processes.
The interference of quanta lies at the heart of quantum physics. The multipartite generalization of single-quanta interference creates entanglement, the coherent superposition of states shared by several quanta. Entanglement allows non-local correlations between many quanta and hence is a key resource for quantum information technology. Entanglement is typically considered to be essential for creating non-local quantum interference. Here, we show that this is not the case and demonstrate multiphoton non-local quantum interference that does not require entanglement of any intrinsic properties of the photons. We harness the superposition of the physical origin of a four-photon product state, which leads to constructive and destructive interference with the photons' mere existence. With the intrinsic indistinguishability in the generation process of photons, we realize four-photon frustrated quantum interference. This allows us to observe the following noteworthy difference to quantum entanglement: We control the non-local multipartite quantum interference with a photon that we never detect, which does not require quantum entanglement. These non-local properties pave the way for the studies of foundations of quantum physics and potential applications in quantum technologies.
While integrated photonics is a robust platform for quantum information processing, architectures for photonic quantum computing place stringent demands on high quality information carriers. Sources of single photons that are highly indistinguishable and pure, that are either near-deterministic or heralded with high efficiency, and that are suitable for mass-manufacture, have been elusive. Here, we demonstrate on-chip photon sources that simultaneously meet each of these requirements. Our photon sources are fabricated in silicon using mature processes, and exploit a dual-mode pump-delayed excitation scheme to engineer the emission of spectrally pure photon pairs through inter-modal spontaneous four-wave mixing in low-loss spiralled multi-mode waveguides. We simultaneously measure a spectral purity of 0.9904 ± 0.0006, a mutual indistinguishability of 0.987 ± 0.002, and >90% intrinsic heralding efficiency. We measure on-chip quantum interference with a visibility of 0.96 ± 0.02 between heralded photons from different sources.