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Trapping and evolution dynamics of strongly magnetized cold gases.

Jaehoon Choi

Published Jan 1, 2006• 0 citations
OpenAlex

Abstract

Cold Rydberg atoms and ultracold plasmas have been studied in the strong-magnetization regime. In this new territory, novel atomic and plasma states---such as guiding-center drift Rydberg attains and strongly magnetized, quasi-neutral, ultracold plasmas---have been created and investigated. The evolution dynamics studies of these exotic diamagnetic forms of matter, made possible by implementing a superconducting magnetic atom trap, revealed rich dynamical features in the systems: The Landau-quantized energy structure has led to entirely different evolutions of the highly excited atoms in laser-excited or drift Rydberg states than in magnetic-field-free cases; and the presence of the strong magnetic field has drastically altered the collisional behavior and expansion dynamics of the plasmas. Furthermore, atom cooling and trapping methodology has been extended in multiple directions. Firstly, laser cooling and magnetic trapping of ground-state atoms has been demonstrated in magnetic; fields exceeding 3 Tesla, representing a 20-fold increase in the field-strength of cold-atom traps. Secondly, the trapping of Rydberg atoms with a lifetime of 80 ms has been achieved. This trapping technique exploits the quasi-free nature of Rydberg electrons, which can be adopted in other forms of Rydberg-atom trapping. Lastly; the trapping of two-component, ultracold plasmas has been demonstrated in a nested Penning-trap configuration. The confinement of quasi-neutral ultracold plasmas allowed us to observe novel effects such as the correlation between the ionic oscillation and the electron energy distribution.

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•Jan 1, 2009•1 citation
Cold Rydberg atoms and ultracold plasmas have been studied in the strong-magnetization regime. In this new territory, novel atomic and plasma states---such as guiding-center drift Rydberg attains and strongly magnetized, quasi-neutral, ultracold plasmas---have been created and investigated. The evolution dynamics studies of these exotic diamagnetic forms of matter, made possible by implementing a superconducting magnetic atom trap, revealed rich dynamical features in the systems: The Landau-quantized energy structure has led to entirely different evolutions of the highly excited atoms in laser-excited or drift Rydberg states than in magnetic-field-free cases; and the presence of the strong magnetic field has drastically altered the collisional behavior and expansion dynamics of the plasmas. Furthermore, atom cooling and trapping methodology has been extended in multiple directions. Firstly, laser cooling and magnetic trapping of ground-state atoms has been demonstrated in magnetic; fields exceeding 3 Tesla, representing a 20-fold increase in the field-strength of cold-atom traps. Secondly, the trapping of Rydberg atoms with a lifetime of 80 ms has been achieved. This trapping technique exploits the quasi-free nature of Rydberg electrons, which can be adopted in other forms of Rydberg-atom trapping. Lastly; the trapping of two-component, ultracold plasmas has been demonstrated in a nested Penning-trap configuration. The confinement of quasi-neutral ultracold plasmas allowed us to observe novel effects such as the correlation between the ionic oscillation and the electron energy distribution.
Cold Rydberg atoms exposed to strong magnetic fields possess unique properties which open the pathway for an intriguing many-body dynamics taking place in Rydberg gases, consisting of either matter or anti-matter systems. We review both the foundations and recent developments of the field in the cold and ultracold regime where trapping and cooling of Rydberg atoms have become possible. Exotic states of moving Rydberg atoms, such as giant dipole states, are discussed in detail, including their formation mechanisms in a strongly magnetized cold plasma. Inhomogeneous field configurations influence the electronic structure of Rydberg atoms, and we describe the utility of corresponding effects for achieving tightly trapped ultracold Rydberg atoms. We review recent work on large, extended cold Rydberg gases in magnetic fields and their formation in strongly magnetized ultracold plasmas through collisional recombination. Implications of these results for current antihydrogen production experiments are pointed out, and techniques for the trapping and cooling of such atoms are investigated.
By photoionizing samples of laser-cooled atoms with laser light tuned just above the ionization limit, plasmas can be created with electron and ion temperatures below 10 K. These ultracold neutral plasmas have extended the temperature bounds of plasma physics by two orders of magnitude. Table-top experiments, using many of the tools from atomic physics, allow for the study of plasma phenomena in this new regime with independent control over the density and temperature of the plasma through the excitation process. Characteristic of these systems is an inhomogeneous density profile, inherited from the density distribution of the laser-cooled neutral atom sample. Most work has dealt with unconfined plasmas in vacuum, which expand outward at velocities of order 100 m/s, governed by electron pressure, and with lifetimes of order 100 μs, limited by stray electric fields. Using detection of charged particles and optical detection techniques, a wide variety of properties and phenomena have been observed, including expansion dynamics, collective excitations in both the electrons and ions, and collisional properties. Through three-body recombination collisions, the plasmas rapidly form Rydberg atoms, and clouds of cold Rydberg atoms have been observed to spontaneously avalanche ionize to form plasmas. Of particular interest is the possibility of the formation of strongly coupled plasmas, where Coulomb forces dominate thermal motion and correlations become important. The strongest impediment to strong coupling is disorder-induced heating, a process in which Coulomb energy from an initially disordered sample is converted into thermal energy. This restricts electrons to a weakly coupled regime and leaves the ions barely within the strongly coupled regime. This review will give an overview of the field of ultracold neutral plasmas, from its inception in 1999 to current work, including efforts to increase strong coupling and effects on plasma properties due to strong coupling.
We have observed the evolution of cold Rydberg gases and ultracold plasmas in an environment that allows for the control of interactions of the blackbody radiation temperature from 4K to 300K. The work in this thesis describes the influence of initial densities, populations, excitation state, evolution time and thermal background temperature on the evolution of cold Rydberg gases as well as directly excited ultracold plasmas. With some initial ionization, cold-Rydberg-atom gases easily develop a positive space charge that traps electrons for times on the order of tens of mus. This acts as a catalyst for electron-Rydberg atom collisions, increasing the collision probabilities by orders of magnitude and profoundly altering the final state of the Rydberg gas. Using state-selective field ionization, we have provided direct proof that these collisions cause changes in l-states, and we have seen the first experimental evidence that they also lead to inelastic n-changing collisions, as predicted by theory. We have also found evidence for Rydberg-Rydberg collisions, enabled by the attractive electric-dipole forces between atoms in high-l states and possibly by van-der-Waal's interactions at very high-n . Thermal interactions are seen to influence the formation of a plasma from a cold Rydberg gas. Plasmas form more easily in the presence of a 300K radiation field than at 4K, due to the contribution of thermal ionization to the plasma formation. The background temperature also appears to affect the electron temperature in both the directly excited plasma and the plasma spontaneously formed from a cold Rydberg gas. In Rydberg atom gases that have undergone partial ionization, electron temperatures were estimated using the dependence of n-changing collisions on the electron temperature.
We report on the trapping of long-lived strongly magnetized Rydberg atoms. 85Rb atoms are laser cooled and collected in a superconducting magnetic trap with a strong bias field (2.9 T) and laser excited to Rydberg states. Collisions scatter a small fraction of the Rydberg atoms into long-lived high-angular momentum "guiding-center" Rydberg states, which are magnetically trapped. The Rydberg atomic cloud is examined using a time-delayed, position-sensitive probe. We observe magnetic trapping of these Rydberg atoms for times up to 200 ms. Oscillations of the Rydberg-atom cloud in the trap reveal an average magnetic moment of the trapped Rydberg atoms of approximately -8microB. These results provide guidance for other Rydberg-atom trapping schemes and illuminate a possible route for trapping antihydrogen.
Plasmas, often called the fourth state of matter and the most common one in the universe, have parameters varying by many orders of magnitude, from temperature of a few hundred kelvin in the Earth's ionosphere to 10 16 K in the magnetosphere of a pulsar. Ultracold plasmas, produced by photoionizing a sample of laser-cooled and trapped atoms near the ionization limit, have extended traditional neutral plasma parameters by many orders of magnitude, to electron temperatures below 1 K and ion temperatures in the tens of &mu K to a few Kelvin, and densities of 10 5 cm -3 to 10 10 cm -3 . These plasmas thus provide a testing ground to study basic plasma theory in a clean and simple system with or without a magnetic field. Previous studies of ultracold plasmas have primarily concentrated on temperature measurements, collective modes and expansion dynamics in the absence of magnetic fields. This thesis presents the first study of ultracold plasma dynamics in a magnetic field. The presence of a magnetic field during the expansion can initiate various phenomena, such as plasma confinement and plasma instabilities. While the electron temperatures are very low in ultracold plasmas, we need only tens of Gauss of magnetic field to observe significant effects on the expansion dynamics. To probe the ultraocold plasma dynamics in a magnetic field, we developed a new diagnostic - projection imaging, which images the ion distribution by extracting the ions with a high voltage pulse onto a position-sensitive detector. Early in the lifetime of the plasma (< 20 &mu s), the size of the image is dominated by the time-of-flight Coulomb explosion of the dense ion cloud. For later times, we measure the 2-D Gaussian width of the ion image, obtaining the transverse expansion velocity as a function of magnetic field (up to 70 G),and observe that the transverse expansion velocity scales as B &minus1/2 , explained by a nonlinear ambipolar diffusion model that involes anisotropic diffusion in two different directions. We also present the first observation of a plasma instability in an expanding ultracold plasma. We observe periodic emission of electrons from an ultracold plasma in weak, crossed magnetic and electric fields, and a strong perturbed electron density distribution in electron time-of-flight projection images. We identify this instability as a high-frequency electron drift instability due to the coupling between the electron drift wave and electron cyclotron harmonic, which has large wavenumbers corresponding to wavelengths close to the electron gyroradius.