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Second-Harmonic Generation for Narrow-Line Cooling of 7Li

Henry Luo

Published Feb 14, 2017• 0 citations
OpenAlex

Abstract

Laser cooling of lithium atoms is usually performed on the 2S1/2 to 2P3/2 transition at 671 nm. The Doppler temperature of this transition, which is the limit temperature of laser cooling, is 140 µK. The 2S1/2 to 3P3/2 transition at 323 nm has a Doppler temperature 7 times smaller than that of the 671 nm transition. With the 323 nm transition, it is possible to reach a temperature low enough for an all-optical production of a Bose-Einstein condensate. The 323 nm light is produced by second-harmonic generation (SHG). We present our design of the laser system that generates light at 646 nm and the frequency-doubling cavity for SHG. The laser frequency is stabilized by a Fabry-Perot cavity and an Iodine transition.

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We have used the narrow 2 S 1/2 [arrow right] 3 P 3/2 transition in the ultraviolet (UV) to laser cool and magneto-optically trap (MOT) 6 Li atoms. Laser cooling of lithium atoms is usually performed on the 2 S 1/2 [arrow right] 2 P 3/2 (D2) transition, where temperatures of twice the Doppler limit, or ∼300 μ K for lithium, are achieved. The linewidth of the UV transition is seven times narrower than the D2 line, resulting in a lower Doppler limit. We show that a MOT operating on the UV transition reaches temperatures as low as 59 μ K. We load 6 million atoms from this UV MOT into a 1070 nm optical dipole trap (ODT). We show that the light shift of the UV transition in the ODT is small and blue-shifted, facilitating efficient loading. Evaporative cooling of a two spin-state mixture of 6 Li in the ODT produces a quantum degenerate Fermi gas with 3 million atoms in only 11 seconds.

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We have used the narrow $2{S}_{1/2}\ensuremath{\rightarrow}3{P}_{3/2}$ transition in the ultraviolet (uv) to laser cool and magneto-optically trap (MOT) ${}^{6}$Li atoms. Laser cooling of lithium is usually performed on the $2{S}_{1/2}\ensuremath{\rightarrow}2{P}_{3/2}$ (D2) transition, and temperatures of $\ensuremath{\sim}$300 $\ensuremath{\mu}$K are typically achieved. The linewidth of the uv transition is seven times narrower than the D2 line, resulting in lower laser cooling temperatures. We demonstrate that a MOT operating on the uv transition reaches temperatures as low as 59 $\ensuremath{\mu}$K. Furthermore, we find that the light shift of the uv transition in an optical dipole trap at 1070 nm is small and blueshifted, facilitating efficient loading from the uv MOT. Evaporative cooling of a two spin-state mixture of ${}^{6}$Li in the optical trap produces a quantum degenerate Fermi gas with $3\ifmmode\times\else\texttimes\fi{}{10}^{6}$ atoms in a total cycle time of only 11 s.

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Laser system for secondary cooling of87Sr atoms

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A laser system with a narrow generation line for secondary laser cooling of 87 Sr atoms has been developed and investigated. It is planned to use ultracold 87 Sr atoms loaded in an optical lattice in an optical frequency standard. To this end, a 689-nm semiconductor laser has been stabilised using an external reference ultrastable cavity with vibrational and temperature compensation near the critical point. The lasing spectral width was 80 Hz (averaging time 40 ms), and the frequency drift was at a level of 0.3 Hz s -1 . Comparison of two independent laser systems yielded a minimum Allan deviation: 2 × 10 -14 for 300-s averaging. It is shown that this system satisfies all requirements necessary for secondary cooling of 87Sr atoms using the spectrally narrow 1 S 0 — 3 P 1 transition (λ = 689 nm).

Quantum Electronics•Nov 30, 2012•14 citations
Laser cooling of lithium atoms is usually performed on the 2S1/2 to 2P3/2 transition at 671 nm. The Doppler temperature of this transition, which is the limit temperature of laser cooling, is 140 µK. The 2S1/2 to 3P3/2 transition at 323 nm has a Doppler temperature 7 times smaller than that of the 671 nm transition. With the 323 nm transition, it is possible to reach a temperature low enough for an all-optical production of a Bose-Einstein condensate. The 323 nm light is produced by second-harmonic generation (SHG). We present our design of the laser system that generates light at 646 nm and the frequency-doubling cavity for SHG. The laser frequency is stabilized by a Fabry-Perot cavity and an Iodine transition.
We have used the narrow 2 S 1/2 [arrow right] 3 P 3/2 transition in the ultraviolet (UV) to laser cool and magneto-optically trap (MOT) 6 Li atoms. Laser cooling of lithium atoms is usually performed on the 2 S 1/2 [arrow right] 2 P 3/2 (D2) transition, where temperatures of twice the Doppler limit, or ∼300 μ K for lithium, are achieved. The linewidth of the UV transition is seven times narrower than the D2 line, resulting in a lower Doppler limit. We show that a MOT operating on the UV transition reaches temperatures as low as 59 μ K. We load 6 million atoms from this UV MOT into a 1070 nm optical dipole trap (ODT). We show that the light shift of the UV transition in the ODT is small and blue-shifted, facilitating efficient loading. Evaporative cooling of a two spin-state mixture of 6 Li in the ODT produces a quantum degenerate Fermi gas with 3 million atoms in only 11 seconds.
Laser cooling to micro-Kelvin temperatures requires a laser with active frequency stabilization. The linewidth of an atomic transition sets a lower bound on the Doppler cooling temperature. The 2s-2p transition in lithium-6 has a Doppler temperature of ~140 μK In contrast, the 2s-3p transition has a narrower linewidth and thus provides a lower temperature limit of ~20 μK. We present a method for stabilizing a laser to an atomic line in a vapor cell using modulation transfer spectroscopy and a home-built lock-in amplifier. Our results demonstrate successful locking of a 323 nm laser to the 2s-3p transition. The stabilized laser provides a second stage of magneto-optical trapping that results in a factor of ∼5 increase in the phase space density before evaporating to degeneracy in an optical dipole trap.
We have used the narrow $2{S}_{1/2}\ensuremath{\rightarrow}3{P}_{3/2}$ transition in the ultraviolet (uv) to laser cool and magneto-optically trap (MOT) 6{}^{6}6Li atoms. Laser cooling of lithium is usually performed on the $2{S}_{1/2}\ensuremath{\rightarrow}2{P}_{3/2}$ (D2) transition, and temperatures of $\ensuremath{\sim}$300 $\ensuremath{\mu}$K are typically achieved. The linewidth of the uv transition is seven times narrower than the D2 line, resulting in lower laser cooling temperatures. We demonstrate that a MOT operating on the uv transition reaches temperatures as low as 59 $\ensuremath{\mu}$K. Furthermore, we find that the light shift of the uv transition in an optical dipole trap at 1070 nm is small and blueshifted, facilitating efficient loading from the uv MOT. Evaporative cooling of a two spin-state mixture of 6{}^{6}6Li in the optical trap produces a quantum degenerate Fermi gas with $3\ifmmode\times\else\texttimes\fi{}{10}^{6}$ atoms in a total cycle time of only 11 s.
We demonstrate laser cooling of trapped beryllium ions at 313 nm using a frequency-doubled extended cavity diode laser operated at 626 nm, obtained by cooling a ridge waveguide diode laser chip to -31°C. Up to 32 mW of narrowband 626 nm laser radiation is obtained. After passage through an optical isolator and beam shaping optics, 14 mW of 626 nm power remains of which 70% is coupled into an external enhancement cavity containing a nonlinear crystal for second-harmonic generation. We produce up to 35 μW of 313 nm radiation, which is subsequently used to laser cool and detect 6×10(2) beryllium ions, stored in a linear Paul trap, to a temperature of about 10 mK, as evidenced by the formation of Coulomb crystals. Our setup offers a simple and affordable alternative for Doppler cooling, optical pumping, and detection to presently used laser systems.
In this thesis we present novel techniques for the study of ultracold gases of lithium atoms. In the first part of this thesis, we present the development of a narrow-linewidth laser source emitting 840mW of output power in the vicinity of the lithium D-line resonances at 671 nm. The source is based on a diode-end-pumped unidirectional ring laser operating on the 1342-nm transition in Nd:YVO4, capable of producing 1.3W of single-mode light delivered in a diffraction-limited beam. The output beam is subsequently frequency-doubled using periodically-poled potassium titanyl phosphate (ppKTP) in an external buildup cavity. We obtain doubling efficiencies of up to 86%. Tunability of the output frequency over more than 400GHz and frequency-locking of the cavity ensemble with respect to the lithium D-line transitions are accomplished. We measure the linewidth to be 200+400-200kHz. In the second part of this thesis, we employ the source in an experimental setup to produce to cool and trap lithium atoms. We realize samples of finite-temperature unitary Bose gases around the center of a Fano-Feshbach resonance, where interactions between the atoms are maximized. We present temperature-dependent measurements of the unitarity-limited three-body loss rate. The measured losses attain the limiting value imposed by quantum mechanics without adjustable parameters. This measurement allows for the introduction of a criterion for quasi-equilibrium. In this regime, by using technique based on in-situ imaging developed in our group, we provide a first measurement of the equation of state of the unitary Bose gas at low fugacities.
A laser system with a narrow generation line for secondary laser cooling of 87 Sr atoms has been developed and investigated. It is planned to use ultracold 87 Sr atoms loaded in an optical lattice in an optical frequency standard. To this end, a 689-nm semiconductor laser has been stabilised using an external reference ultrastable cavity with vibrational and temperature compensation near the critical point. The lasing spectral width was 80 Hz (averaging time 40 ms), and the frequency drift was at a level of 0.3 Hz s -1 . Comparison of two independent laser systems yielded a minimum Allan deviation: 2 × 10 -14 for 300-s averaging. It is shown that this system satisfies all requirements necessary for secondary cooling of 87Sr atoms using the spectrally narrow 1 S 0 — 3 P 1 transition (λ = 689 nm).