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Quantum control with spectral constraints

Zbigniew Puchaøa

Published Jan 1, 2014• 0 citations
OpenAlex

Abstract

Various constraints concerning control fields can be imposed in the real- istic implementations of quantum control systems. One of the most important is the restriction on the frequency spectrum of acceptable control parameters. It is important to consider the limitations of experimental equipment when trying to find appropriate control parameters. Therefore, in this paper, we present a general method of obtaining a piecewise-constant controls, which are robust with respect to spectral constraints. We consider here a Heisenberg spin chain; however, the method can be applied to a system with more general interactions. To model experimental restrictions, we apply an ideal low-pass filter to numerically obtained control pulses. The usage of the pro- posed method has negligible impact on the control quality as opposed to the standard approach, which does not take into account spectral limitations.

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Various constraints concerning control fields can be imposed in the real- istic implementations of quantum control systems. One of the most important is the restriction on the frequency spectrum of acceptable control parameters. It is important to consider the limitations of experimental equipment when trying to find appropriate control parameters. Therefore, in this paper, we present a general method of obtaining a piecewise-constant controls, which are robust with respect to spectral constraints. We consider here a Heisenberg spin chain; however, the method can be applied to a system with more general interactions. To model experimental restrictions, we apply an ideal low-pass filter to numerically obtained control pulses. The usage of the pro- posed method has negligible impact on the control quality as opposed to the standard approach, which does not take into account spectral limitations.
Various constraints concerning control fields can be imposed in the realistic implementations of quantum control systems. One of the most important is the restriction on the frequency spectrum of acceptable control parameters. It is important to consider the limitations of experimental equipment when trying to find appropriate control parameters. Therefore, in this paper, we present a general method of obtaining a piecewise-constant controls, which are robust with respect to spectral constraints. We consider here a Heisenberg spin chain; however, the method can be applied to a system with more general interactions. To model experimental restrictions, we apply an ideal low-pass filter to numerically obtained control pulses. The usage of the proposed method has negligible impact on the control quality as opposed to the standard approach, which does not take into account spectral limitations.
Motivated by some recent results of quantum control theory, we discuss the feasibility of local operator control in arrays of interacting qubits modeled as isotropic Heisenberg spin chains. Acting on one of the end spins, we aim at finding piecewise-constant control pulses that lead to optimal fidelities for a chosen set of quantum gates. We analyze the robustness of the obtained results for the gate fidelities to random errors in the control fields, finding that with faster switching between piecewise-constant controls the system is less susceptible to these errors. The observed behavior falls into a generic class of physical phenomena that are related to a competition between resonance- and relaxation-type behavior, exemplified by motional narrowing in NMR experiments. Finally, we discuss how the obtained optimal gate fidelities are altered when the corresponding rapidly varying piecewise-constant control fields are smoothened through spectral filtering.
We investigate the problem of control of quantum systems. Various notions of controllability of quantum systems are discussed and Lie algebraic techniques are employed to derive necessary and sufficient conditions for the resulting degrees of controllability. The results are employed to study the degree of controllability for various model systems. The problem of optimal control is formulated as a problem of maximisation of the expectation value of an observable of the system subject to dynamical constraints and costs. A class of iterative algorithms is discussed, and shown to converge to a solution of the Euler-Lagrange equations, which is a necessary condition for optimality of a solution. A numerical realisation of the algorithm is presented and potential implementation of the resulting control fields in the laboratory is discussed. The algorithm is applied to find optimal control fields for a variety of applications including selective and simultaneous excitation of individual quantum dots in a globally addressed ensemble, creation of superposition states, and selective excitation of certain vibrational modes of a simple molecule such as Hydrogen Fluoride. In each case we systematically explore the parameter space of the algorithm to select solutions with desirable physical features from the multitude of possible choices. As there are many possible optimal control fields which give similar yields the question of whether some are more robust than others is investigated. A number of optimal fields are analysed quantitatively in terms of robustness with regard to temporal and spectral noise affecting the fields, uncertainty in the model parameters and the effect of experimental limitations such as restrictions on the bandwidth of the fields. It is shown that whilst the solutions tend to be sensitive to uncertainty in the energy levels chosen for the model, they appear to be surprisingly tolerant to even severe bandwidth limitations.
We propose a monotonically convergent algorithm which can enforce spectral constraints on the control field (and extends to arbitrary filters). The procedure differs from standard algorithms in that at each iteration, the control field is taken as a linear combination of the control field (computed by the standard algorithm) and the filtered field. The parameter of the linear combination is chosen to respect the monotonic behavior of the algorithm and to be as close to the filtered field as possible. We test the efficiency of this method on molecular alignment. Using bandpass filters, we show how to select particular rotational transitions to reach high alignment efficiency. We also consider spectral constraints corresponding to experimental conditions using pulse-shaping techniques. We determine an optimal solution that could be implemented experimentally with this technique.
Shaped pulses obtained by optimal control theory often possess unphysically broad spectra. In principle, the spectral width of a pulse can be restricted by an additional constraint in the optimization functional. However, it has so far been impossible to impose spectral constraints while strictly guaranteeing monotonic convergence. Here, we show that Krotov’s method allows for simultaneously imposing temporal and spectral constraints without perturbing monotonic convergence, provided the constraints can be expressed as positive semi-definite quadratic forms. The optimized field is given by an integral equation which can be solved efficiently using the method of degenerate kernels. We demonstrate that Gaussian filters suppress undesired frequency components in the control of non-resonant two-photon absorption.
Quantum control is concerned with the realisation of desired dynamics in quantum systems, serving as a linchpin for advancing quantum technologies and fundamental research. Analytic approaches and standard optimisation algorithms do not yield satisfactory solutions for more complex quantum systems, and especially not for real world quantum systems which are open and noisy. We devise a physics-constrained Reinforcement Learning (RL) algorithm that restricts the space of possible solutions. We incorporate priors about the desired time scales of the quantum state dynamics - as well as realistic control signal limitations - as constraints to the RL algorithm. These constraints improve solution quality and enhance computational scaleability. We evaluate our method on three broadly relevant quantum systems and incorporate real-world complications, arising from dissipation and control signal perturbations. We achieve both higher fidelities - which exceed 0.999 across all systems - and better robustness to time-dependent perturbations and experimental imperfections than previous methods. Lastly, we demonstrate that incorporating multi-step feedback can yield solutions robust even to strong perturbations. Our implementation can be found at https://github.com/jan-o-e/RL4qcWpc.