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Optics Express

Spatially dependent hyper-Raman scattering in five-level cold atoms

Junqiang Chen, Zhiping Wang, Benli Yu

Published Mar 11, 2021• 20 citations
Publisher

Abstract

We demonstrate a scheme to control the spatially dependent hyper-Raman scattering based on electromagnetically induced transparency in a cold atomic system. By adjusting the different system parameters, one can effectively modulate the phase and intensity of the generated Raman field. Specifically, we show that electromagnetically induced transparency creates quantum interference, which results in greatly enhanced efficiency for the generated Raman field. Such improvement in Raman efficiency makes our scheme suitable for generation of short-wavelength coherent radiation, conversion of frequency, and nonlinear spectroscopy based on orbital angular momentum light.

DOI
10.1364/oe.420015

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We demonstrate a scheme to control the spatially dependent hyper-Raman scattering based on electromagnetically induced transparency in a cold atomic system. By adjusting the different system parameters, one can effectively modulate the phase and intensity of the generated Raman field. Specifically, we show that electromagnetically induced transparency creates quantum interference, which results in greatly enhanced efficiency for the generated Raman field. Such improvement in Raman efficiency makes our scheme suitable for generation of short-wavelength coherent radiation, conversion of frequency, and nonlinear spectroscopy based on orbital angular momentum light.
An efficient scheme for controlling the spatial Raman gain is proposed in a cold atomic ensemble with a four-level N-typed configuration. The cold atoms are driven by the Laguerre-Gaussian (LG) vortex beams. Considering the control and driving fields are vortex beams and using experimentally achievable parameters, we identify the condition under which the topological charges (TCs) allows us to manipulate the radial distribution of the Raman gain spectra. It is found that the spatial Raman gain can be effectively controlled via adjusting the relevant optical parameters. Furthermore, we show interesting optical properties of vortex-induced transparency(VIT) and vortex-induced gain (VIG) via controlling the spatial Raman-gain spectrum. Finally we show that the azimuthal modulation of the Raman gain profiles can be realized and controlled when the control field consists of a travelling-wave (TW) field and two optical vortex fields. Our scheme may provide a feasible approach for constructing novel vortex beams based on cold atomic ensemble.
Abstract In this paper, we suggest a theoretical model for the exchange of the orbital angular momentum (OAM) state of laser fields in a real cold atomic system for realization in an experimental setup. By using four-wave mixing (FWM) processes, we study the spatial dependence of the new weak generated signal light under electromagnetically induced transparency conditions when one of the laser lights becomes an optical vortex. We discuss the spatial dependence of FWM processes via experimental parameters for different conditions of the OAM of vortex light. We have found that the intensity and phase distributions of the new generated light depends strongly on the OAM number of the optical vortex light. Moreover, we investigate the absorption spectrum of the new generated signal light for different OAM of the optical vortex light. Our obtained results may have potential applications in quantum information science.
This dissertation reports experimental studies of nonlinear optical effects manifested by electromagnetically induced transparency (EIT) in cold Rb atoms. The cold Rb atoms are confined in a magneto-optic trap (MOT) obtained with the standard laser cooling and trapping technique. Because of the near zero Doppler shift and a high phase density, the cold Rb sample is well suited for studies of atomic coherence and interference and related applications, and the experiments can be compared quantitatively with theoretical calculations. It is shown that with EIT induced in the multi-level Rb system by laser fields, the linear absorption is suppressed and the nonlinear susceptibility is enhanced, which enables studies of nonlinear optics in the cold atoms with slow photons and at low light intensities. Three independent experiments are described and the experimental results are presented. First, an experimental method that can produce simultaneously co-propagating slow and fast light pulses is discussed and the experimental demonstration is reported. Second, it is shown that in a three-level Rb system coupled by multi-color laser fields, the multi-channel two-photon Raman transitions can be manipulated by the relative phase and frequency of a control laser field. Third, a scheme for all-optical switching near single photon levels is developed. The scheme is based on the phase-dependent multi-photon interference in a coherently coupled four-level system. The phase dependent multi-photon interference is observed and switching of a single light pulse by a control pulse containing ∼20 photons is demonstrated. These experimental studies reveal new phenomena manifested by quantum coherence and interference in cold atoms, contribute to the advancement of fundamental quantum optics and nonlinear optics at ultra-low light intensities, and may lead to the development of new techniques to control quantum states of atoms and photons, which will be useful for applications in quantum measurements and quantum photonic devices.
In this paper, we propose and analyze an optical multi-wave mixing scheme for the generation of coherent light in a five-level atomic system in the context of electromagnetically induced transparency. A detailed semiclassical study of the propagation of generated mixing and probe fields is demonstrated. The analytical dependence of the generated mixing field on the probe field and the respective detuning is predicted. Such a nonlinear optical process can be used for generating short-wavelength radiation at low pump intensities.
We propose an efficient scheme to manipulate spontaneous emission spectra using optical vortices carrying orbital angular momentum (OAM) in a coherently driven cold five-level atomic system assisted by a radio frequency (RF) or microwave field. Using experimentally achievable parameters, we find that the spontaneous emission is strongly influenced by quantum destructive interference. And we show that the structured light profile of the probe field can be transferred to the spontaneous emission spectrum via spontaneously generated coherence (SGC). With the aid of SGC, the intensities and detunings of the control and RF fields can be used to tailor the vortex-induced spontaneous emission spectra. When the control and RF fields are configured as vortex beams, it is demonstrated that the spontaneous emission can be coherently controlled through quantum interference by adjusting their topological charges (TCs). Furthermore, we explore intriguing optical properties of the vortex-induced spontaneous emission by varying the TCs of the probe and control fields. This coherently driven atomic system features three closely spaced levels, giving rise to multiple vortex-induced SGC pathways. Our scheme opens avenues for applications in structured light, ranging from optical storage to optical communication.