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Advanced Quantum Technologies

Spontaneous Parametric Down‐Conversion Sources for Multiphoton Experiments

Chao Zhang, Yun‐Feng Huang, Bi‐Heng Liu, Chuan‐Feng Li, Guang‐Can Guo

Published Mar 22, 2021• 126 citations
Publisher

Abstract

Abstract Entangled photon sources are desirable and key elements for photonic quantum information processing. The spontaneous parametric down‐conversion (SPDC) process is a convenient way to produce entangled photon pairs. It has been widely used and has already made great contributions to quantum information science. SPDC sources have been thoroughly studied, and a detailed review, previously lacking, is now appropriate. In this article, different types of SPDC sources suitable for multiphoton experiments are reviewed. A comparison of their respective performances is presented, focusing on the parameters of indistinguishability, collection efficiency, and brightness, from which it is possible to see how the spatial and spectral properties of the SPDC process can be tailored, step by step, to achieve near‐perfect photon pairs. Recent progress on multiplexed heralded single‐photon sources, which effectively mitigate the nondeterministic nature of the SPDC process, is also described.

DOI
10.1002/qute.202000132

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Abstract Entangled photon sources are desirable and key elements for photonic quantum information processing. The spontaneous parametric down‐conversion (SPDC) process is a convenient way to produce entangled photon pairs. It has been widely used and has already made great contributions to quantum information science. SPDC sources have been thoroughly studied, and a detailed review, previously lacking, is now appropriate. In this article, different types of SPDC sources suitable for multiphoton experiments are reviewed. A comparison of their respective performances is presented, focusing on the parameters of indistinguishability, collection efficiency, and brightness, from which it is possible to see how the spatial and spectral properties of the SPDC process can be tailored, step by step, to achieve near‐perfect photon pairs. Recent progress on multiplexed heralded single‐photon sources, which effectively mitigate the nondeterministic nature of the SPDC process, is also described.
Entangled photon pairs play a crucial role in emerging quantum technologies, acting as tamper-proof padlocks in secure quantum communication, ultra-precise probes in quantum metrology and high-fidelity information carriers in photonic quantum computing. Amongst the many technological possibilities for generating photon pairs, sources based on spontaneous parametric down-conversion (SPDC) in second-order nonlinear crystals are still the workhorse tool in quantum optics laboratories, and more recently even in long-distance quantum communication with satellites. SPDC is a widely used method to create entangled photon pairs. The number of photon pairs that can be detected in a particular choice of collection modes, typically being optical single-mode fibers, depends critically on the spatial characteristics of the multi-mode SPDC emission as well as the particular beam waist of the collection modes. While several studies have already addressed the issue of optimal fiber coupling of SPDC photons in theory and experiment, the results of these studies arrive at different conclusions. Here, we present the results of a comprehensive experimental study on the optimal collection of photon pairs into single-mode optical fibers. Our approach is based on quasi-phase-matched type II SPDC from a periodically poled KTiOPO4 (ppKTP) crystal. We discuss the influence of pump and collection focal parameters on the spectral brightness and heralding efficiency, as well as practical issues of alignment tolerances into an optical single mode fiber. Further, Using two-photon interference (Hong-Ou-Mandel interference), we assess the spectral bandwidth of the photon pairs for variable crystal lengths. The results are in good agreement with our theoretical model, thus providing the recipe of building ultra bright and stable entangled photon sources.
The generation of high purity single photons and entangled photon pairs is a crucial first step in many quantum optics experiments, including those that require quantum teleportation [1], entanglement swapping [2], and the generation of multi-photon entanglement [3]. The most widely used and established approach for creating photon pairs is spontaneous parametric down conversion (SPDC) - where pump photons undergo a non-linear optical process to create a down-converted photon pair [4]. Traditionally, the generation of high-purity heralded single photons required severe spectral filtering, introducing additional loss. However, through careful engineering of spectral correlations of the down-converted photon pairs one can circumvent the need for filtering and avoid the accompanying reduction in heralding efficiency.
A workflow for evaluation of entanglement source quality is proposed. Based on quantum state density matrices obtained from theoretical models and experimental data, we make an estimate of a potential performance of a quantum entanglement source in quantum key distribution protocols. This workflow is showcased for continuously pumped spontaneous parametric down-conversion (SPDC) source, where it highlights the trade-off between entangled pair generation rate and entanglement quality caused by multiphoton nature of the generated quantum states. We employ this characterization technique to show that secure key rate of down-converted photon pairs is limited to 0.029 bits per detection window due to intrinsic multiphoton contributions. We also report that there exists one optimum gain for continuous-wave down-conversion sources. We find a bound for secure key rate extracted from SPDC sources and make a comparison with perfectly single-pair quantum states, such as those produced by quantum dots.
The generation of entangled photon pairs through spontaneous parametric down conversion (SPDC) is widely used and considered one of the key entanglement generation techniques in quantum optics. The quality of the entanglement produced depends significantly on the physical properties of the nonlinear crystal employed in the SPDC process. In this study, we investigate the influence of the crystal parameters such as phase matching configurations on the degree of entanglement. Our results demonstrate the importance of crystal selection for achieving highly entangled photon sources, which are essential for applications in quantum communication and quantum information.
An important step for photonic quantum technologies is the demonstration of a quantum advantage through boson sampling. In order to prevent classical simulability of boson sampling, the photons need to be almost perfectly identical and almost without losses. These two requirements are connected through spectral filtering: improving one leads to a decrease of the other. A proven method of generating single photons is spontaneous parametric down-conversion (SPDC). We explore the fundamental limits of several important SPDC sources and show that an optimal tradeoff between indistinguishability and losses can always be found. We conclude that a 50-photon scattershot boson-sampling experiment using SPDC sources is possible from a computational complexity point of view. To this end, we numerically optimize SPDC sources under the regime of weak pumping and with a single spatial mode.
ABSTRACT Spontaneous parametric down conversion (SPDC) holds a pivotal role in quantum physics, facilitating the creation of entangled photon pairs, heralded single photons and squeezed light, critical resources for many applications in quantum technologies. However, their production is susceptible to physical variations, posing limitations on their robust utility. To overcome these limitations, this work introduces a method to significantly enhance the reliability of entangled photon pair generation. This approach involves introducing a composite design scheme to the SPDC process. The design is based on the development of a theoretical composite segments framework for SU(1,1), offering increased error resilience and robustness of the process. The practical application is experimentally demonstrated by modulating the nonlinear coefficient of a KTP crystal for degenerate 532–1064 nm conversion, resulting in an effective sevenfold improvement in stability of photon‐pair generation and coincidence rate against temperature fluctuations compared to conventional quasi‐phase‐matching techniques. Furthermore, the presented concept is applicable to other physical systems that exhibit SU(1,1) dynamics. This methodology can create a leap forward in quantum technologies by significantly enhancing stability and error tolerance, thus paving the way for a new generation of entangled photon sources, holding promise for quantum information processing, communication, and precision measurement applications.