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Ukrainian Journal of Physics

Raman scattering of light in crystals with the participation of the Bose-Einstein condensate of excitons

Yu. D. Zavorotnev, L. I. Stefanovich

Published Mar 1, 1983• 0 citations
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Experimental results are presented on excitonic effects related to the Bose-Einstein condensation (BEC) of excitons in Cu2O. Such effects include resonant light polarization dependent absorption, exciton creation and diffusion by absorption of scattered light, and resonant high density exciton packet induced absorption. These results are then utilized, in conjunction with similar results on excitonic BEC, to develop a plausible model for condensate amplification. Condensates are initially created at T = 1.8K with high intensity ND:YAG pulses (lambda = 532 nm) and then stimulated by a secondary source tuned around the 1S orthoexciton resonance (lambda = 609.51 nm); the latter induces the observed condensate amplification. By careful analysis of the various interactions between the secondary light source, the crystal, and the condensate itself, an improved understanding of how the secondary pulse excitations interact with the passage of a high density exciton packet is obtained.
Abstract Two‐photon resonant Raman scattering processes are studied in different scattering configurations in CuCl. Observation of Raman lines from the front face of the crystal (backward scattering) yields new information on the energy of the transverse T5 exciton and on the biexciton damping. In transmission (forward scattering), two new emission lines can be identified as due to the Raman effect. They show a strong angular dependence because of the polariton nature of the particles involved. Their characteristic features contradict an interpretation in terms of Bose‐Einstein condensed biexcitons.