In general, the process of spin squeezing is employed for atomic sensors that are essentially free from the effect of spontaneous emission. In the case of an atomic clock based on coherent population trapping, spontaneous emission plays a key role. Specifically, when the clock is realized in the Ramsey configuration employing a pair of pulses separated in time, it is the spontaneous emission process during the first pulse that creates the coherent population trapping, by optically pumping the atoms into the so-called dark state. We show in this talk that it is still possible to apply the process of spin squeezing to enhance the sensitivity of such a clock, by designing carefully the sequence of steps in the protocol. Specifically, we consider the approach of using the maximally entangled Schroedinger Cat states, produced via one axis twist squeezing, to achieve Heisenberg Limited sensitivity, representing an improvement in sensitivity by as much as four orders of magnitude.
In general, the process of spin squeezing is employed for atomic sensors that are essentially free from the effect of spontaneous emission. In the case of an atomic clock based on coherent population trapping, spontaneous emission plays a key role. Specifically, when the clock is realized in the Ramsey configuration employing a pair of pulses separated in time, it is the spontaneous emission process during the first pulse that creates the coherent population trapping, by optically pumping the atoms into the so-called dark state. We show in this talk that it is still possible to apply the process of spin squeezing to enhance the sensitivity of such a clock, by designing carefully the sequence of steps in the protocol. Specifically, we consider the approach of using the maximally entangled Schroedinger Cat states, produced via one axis twist squeezing, to achieve Heisenberg Limited sensitivity, representing an improvement in sensitivity by as much as four orders of magnitude.
The coherent population trapping (CPT) effect is used for making compact atomic clocks. There are two types of CPT clocks: the one in which the Raman beams are applied continuously and the one in which two CPT pulses separated by a dark period are applied (Ramsey scheme). It is obvious that the technique of spin squeezing can only be applied to the Ramsey CPT clock to enhance the sensitivity. However, it is not apparent how to adapt to the CPT clock the protocols for the microwave clock using one-axis-twist squeezing (OATS), since the Ramsey CPT clock is not trivially equivalent to the Ramsey microwave clock. In this paper, we show explicitly how to adapt two protocols using OATS, namely, the Schr\"odinger cat state protocol (SCSP) and the generalization thereof, and the echo squeezing protocol (ESP), to the CPT clock. The ESP magnifies the phase shift by a factor of N/e, while the SCSP magnifies the phase shift by a factor of N/2, making it able to achieve a higher sensitivity in the presence of excess noise.
In a conventional atomic interferometer employing N atoms, the phase sensitivity is at the standard quantum limit: 1/N. Using spin-squeezing, the sensitivity can be increased, either by lowering the quantum noise or via phase amplification, or a combination thereof. Here, we show how to increase the sensitivity, to the Heisenberg limit of 1/N, while increasing the quantum noise by N, thereby suppressing by the same factor the effect of excess noise. The protocol uses a Schrodinger Cat state representing a superposition of two collective states of N atoms, behaving as a single entity with an N-fold increase in Compton frequency. The resulting N-fold phase magnification is revealed by using atomic state detection instead of collective state detection. We also show how to realize an atomic clock based on such a Schrodinger Cat state, with an N-fold increase in the effective transition frequency. We discuss potential experimental constraints for implementing this scheme, using one axis twist squeezing employing the cavity feedback scheme, and show that the effects of cavity decay and spontaneous emission are highly suppressed. We find that the maximum improvement in sensitivity can be close to the ideal limit, for as many as ten million atoms.
We investigate theoretically and experimentally a nondestructive interferometric measurement of the state population of an ensemble of laser-cooled and trapped atoms. This study is a step toward generation of (pseudo)spin squeezing of cold atoms targeted at the improvement of the cesium clock performance beyond the limit set by the quantum projection noise of atoms. We calculate the phase shift and the quantum noise of a near-resonant optical probe pulse propagating through a cloud of cold 133Cs atoms. We analyze the figure of merit for a quantum nondemolition (QND) measurement of the collective pseudospin and show that it can be expressed simply as a product of the ensemble optical density and the pulse-integrated rate of the spontaneous emission caused by the off-resonant probe light. Based on this, we propose a protocol for the sequence of operations required to generate and utilize spin squeezing for the improved atomic clock performance via a QND measurement on the probe light. In the experimental part we demonstrate that the interferometric measurement of the atomic population can reach a sensitivity of the order of Nat in a cloud of Nat cold atoms, which is an important benchmark toward the experimental realization of the theoretically analyzed protocol.
In a conventional atomic interferometer employing N atoms, the phase sensitivity is at the standard quantum limit: 1/N. Using spin-squeezing, the sensitivity can be increased, either by lowering the quantum noise or via phase amplification, or a combination thereof. Here, we show how to increase the sensitivity, to the Heisenberg limit of 1/N, while increasing the quantum noise by N, thereby suppressing by the same factor the effect of excess noise. The protocol uses a Schrodinger Cat state representing a superposition of two collective states of N atoms, behaving as a single entity with an N-fold increase in Compton frequency. The resulting N-fold phase magnification is revealed by using atomic state detection instead of collective state detection. We also show how to realize an atomic clock based on such a Schrodinger Cat state, with an N-fold increase in the effective transition frequency. We discuss potential experimental constraints for implementing this scheme, using one axis twist squeezing employing the cavity feedback scheme, and show that the effects of cavity decay and spontaneous emission are highly suppressed. We find that the maximum improvement in sensitivity can be close to the ideal limit, for as many as ten million atoms.
The generation of entanglement in atomic systems plays a central topic in the fields of quantum information storage and processing. Moreover, a special category of entangled states of multi-atom ensembles, spin squeezed states, have been proven to lead to considerable improvement in the sensitivity of precision measurements compared to systems involving uncorrelated atoms. A treatment of entanglement in open systems is, however, incomplete without a precise description of the process of decoherence which necessarily accompanies it. The theory of entanglement and decoherence are the two main topics of this thesis. Methods are described for the generation of strong correlations in large atomic ensembles using either cavity quantum electrodynamics or measurement outcome conditioned quantum dynamics. Moreover, the description of loss of entanglement resulting from the coupling to a noise reservoir (electromagnetic vacuum) is explored. A spin squeezing parameter is used throughout this thesis as both a measure of entanglement strength and as an indication of the sensitivity improvement above the so-called standard quantum limit (sensitivity obtained with uncorrelated particles) in metrology. The first scheme considered consists of a single mode cavity field interacting with a collection of atoms for which spin squeezing is produced in both resonant and off-resonant regimes. In the resonant case, transfer of squeezing from a field state to the atoms is analyzed, while in the off-resonant regime squeezing is produced via an effective nonlinear interaction (one-axis twisting Hamiltonian). A second, more experimentally realistic case, is one involving the interaction of free space atoms with laser pulses; a projective measurement of a source field originating from atomic fluctuations provides a means of preparing atomic collective states such as spin squeezed and Schrodinger cat states. A new unravelling is proposed, that employs the detection of photon number in a single output channel and is capable of producing mesoscopic Schrodinger cat states in a single step. As a first step to understanding the role of cooperative decoherence, of importance in the case of dense pencil-shaped atomic ensembles, the collective spin decoherence of a two multilevel atom system is derived. This calculation is also relevant to entanglement loss for two qubits manipulated using with reading/writing pulses. Finally, a scheme is proposed in which arbitrarily strong entanglement can be produced in a four-wave mixing setup, where the preparation of the atoms in a dark state limits the decoherence to negligible values.
This thesis describes new results on the entanglement of atomic spins in Ramsey interferometry, optical atomic clocks and trapped ions. It is divided into three parts: First, we investigate improvements to conventional Ramsey interferometry with entanglement and adding only rotations of the collective spin to adjust the signal and measurement directions. The geometric degrees of freedom, connected to the rotations, are analytically optimized for a large class of generalized Ramsey protocols to allow efficient optimization of all parameters. Besides a unification of existing approaches, the main result is that there is only one new protocol, where a previously unused double inversion is applied. Studies of the local sensitivity show that this protocol reaches the fundamental quantum Fisher information limit and is yet robust against errors during preparation and measurement. In the second section we investigate the conditions under which optical atomic clocks exhibit increased long-term stability when applying weakly entangled, spin squeezed states. We discuss the common case of an atomic clock with a single ensemble, typical Brownian frequency noise and finite dead time. Theoretical modelling of the servo loop allows quantitative predictions of the optimal stability for given values of dead time and laser noise, in very good agreement with numerical simulations of the closed feedback loop. The main result is that, even with the current most stable lasers, the clock stability can only be improved for ensembles below a critical atom number of about one thousand in optical Sr lattice clocks. Even with a future improvement of the laser performance by one order of magnitude, the critical atom number still remains below 100,000. In contrast, clocks based on smaller, non-scalable ensembles, such as ion clocks, can already benefit from squeezed states with current clock lasers. Thus the last section considers the robust generation of entanglement in ion traps. An error budget including relevant experimental error sources is calculated for state-of-the-art quantum gates, driven by oscillating microwave gradients in surface traps. Amplitude modulation of the driving fields is shown to efficiently counteract the current limitations from motional mode instability. The predicted increase of the gate quality was demonstrated by the group of C. Ospelkaus at PTB Braunschweig, who measured gates with errors as low as ~ 10^(-3). In a similar approach, interactions between spin and motion can also be generated by combining oscillating rf-fields with a static magnetic field gradient. Penning traps designed for precision spectroscopy already feature large magnetic field gradients at the edge of a magnetic bottle configuration. We present parameters and conditions under which laser-free coupling of spin and quantized motion for (anti-)protons is possible at these points, in a step towards quantum logic spectroscopy for (anti-)protons.