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MULTIPARTITE ENTANGLEMENT ENGINEERING FOR QUANTUM INFORMATION AND METROLOGY

Yusef Maleki

Published Aug 3, 2020• 0 citations
OpenAlex

Abstract

Quantum entanglement is central to many quantum technologies and is an indispensable ingredient of quantum information theory. These facts make the generation, characterization and quantification of entangled states unavoidable tasks, beside all their fundamental significance. As a particular example of such applications one may consider quantum metrology in which quantum entanglement is shown to have a significant role for beating the classical limits. However, generation, characterization and quantification of suitable entangled states are challenging tasks, in general.\n\nIn this dissertation, we introduce new platforms for engineering multipartite entangled states that are shown to be useful for quantum information processing and quantum metrology applications. In particular, we introduce new methods which can be used for generating N00N states, as one of the most challenging states to generate, enabling realization of such states in both photonic and spintronic architectures. We sketch a rather generic quantum circuit, for the N00N state generation, that could be realized in various quantum systems. Furthermore, we extend the platform for the generation of states beyond the N00N state. Typical examples of such sates could be entangled coherent or squeezed states, for instance, that of specific importance for quantum information and metrology applications. Furthermore, we extend the protocol for the multipartite state scenario. Also, we demonstrate that attaining the ultimate sensitivity in phase estimation is not an exclusive property of the N00N states. As a result, we find a large class of entangled states that could provide us with the ultimate sensitivity achieved by the N00N state.\n\nAs a part of our effort for the N00N state generation, we develop a new scheme where N00N states could be realized in two ensembles of nitrogen--vacancy (NV) centers in diamond. This could be interesting by noting the fact that NV centers in diamonds provide a remarkably long coherence time, even at the room temperature. This opens up new possibilities for protecting N00N states against decoherence.\n\nMoreover, having the long coherence time of the ensembles of the NV centers, we show that a hybrid quantum system consisting of three ensembles of NV centers coupled to a superconducting device enables the generation of controllable macroscopic multipartite entangled states, which could be used as a building block for quantum networks.\n\nFurthermore, we investigate entanglement of nonorthogonal states in details, and more specifically, we obtain a closed-form analytical expression for the entanglement degree of a multipartite qutrit state, that offers a quantitative measure for entanglement $n$-mode nonorthogonal qutrit states with an arbitrary $n$. Such higher dimensional entangled states could be useful in quantum communication protocols.\n\n Finally, we introduce a new configuration where any pair of quantum states can perfectly be swapped between two quantum resonators enabling a realization of a universal swap operation in photonics systems. This can serve as a building block of various quantum information processors.

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One of the biggest challenges to implement quantum protocols and quantum information processing (QIP) is achieving long coherence times, usually requiring systems at ultra-low temperatures. The nitrogen-vacancy (NV) center in diamond is a promising alternative to this problem. Due to its spin properties, easy manipulation, and the possibility of doing optical state initialization and readout, it quickly became one of the best solid-state spin systems for QIP at room temperature. Here, we present the characterization of the spin-coherence of an ensemble of NV centers in an engineered sample of ultrapure diamond as a testbed for quantum protocols for quantum metrology.

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A quantumnetwork would allow the distribution of a quantum state over many spatially separated quantum nodes which individually possess the ability to generate, process and store quantum information. Connecting these nodes through quantum communication channels would enable sending quantum information over arbitrarily long distances, secret key distribution with guaranteed secure communication and distributed quantum computing. An appealing platform for implementation of quantum networks is the nitrogen-vacancy (NV) center in diamond. An NV center is an optically active defect in diamond created by the substitution of two adjacent carbon atoms in the diamond crystal matrix by a nitrogen atom and a neighboring vacancy. The NV center fits remarkably well in the described quantum network framework. Its electronic spin can be optically initialized, read out in a single shot, coherently manipulated and coupled to the nearby carbon-13 nuclear spins. These properties represent necessary ingredients of a multi-qubit quantum node. The possibility of the entanglement between the state of the NV center spin and a photon establishes a photonic quantum link which can enable the entanglement of the quantum nodes, forming a quantum network. First building blocks of the proposed quantum networks based on NV centers were demonstrated by performing entanglement between two distant NV centers separated by more than a kilometer. However, the current success rate of the entangling protocols is greatly reduced due to the low emission probability of the NV center photons into the resonant zero phonon line (ZPL) and the inefficient photon extraction from the diamond. This is the central problem which prevents promoting our experiments beyond proof-of-principle demonstration towards practical implementation of the proposed quantumnetworks. The goal of this thesis is tackling these issues by coupling NV centers to optical cavities which would greatly increase the rate of generation and collection of the ZPL photons through themechanism of Purcell enhancement. The design and the fabrication of the components constituting a diamond-basedFabry-Perot microcavity, as used in this thesis, are described in Chapter 4. For large enhancement of the NV center resonant emission, a low cavity mode volume is necessary. This is achieved by inserting a micrometers thin diamond slab into the cavity architecture; we present the fabrication details of such samples. Chapter 5 describes the fabrication of an integrated platform for microwave signal delivery to the NV centers within a diamond membrane in the cavity architecture. Microwave striplines and arrays of unique markers are embedded in the mirror onto which the diamond is bonded. We investigate the mirror optical properties post fabrication and find that the fabrication method preserves the mirror optical performance. We describe the diamond bonding method and demonstrate addressing of the NV center spin. In Chapter 6 we probe the properties of the cavity with the embedded diamond membrane through measurements of the cavity finesse. We investigate the cavity finesse dependence on length, mode structure and temperature. We further explore the operation at cryogenic temperatures by probing the effect of cryostation vibration on the cavity linewidth. Finally, in Chapter 7 we discuss ways of improving the existing experimental capabilities, outline the first steps for demonstrating enhancement of the NV center resonant emission and suggest future experiments that can be performed with this system. We conclude that coupling of the NV centers to the cavities developed in this research could lead to an increase of remote entanglement success rates by more than three orders of magnitude.

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Filip Rozpędek

Future quantum networks will enable the realisation of a large family of quantum protocols, hence allowing for implementation of various tasks ranging from quantum cryptography through quantum computing to quantum metrology.In this thesis we analyse and develop the building blocks of quantum repeater networks.These networks consist of quantum repeater nodes, which are equipped with quantum memories enabling storage of quantum information.The repeater nodes are connected using optical fibres that enable for the transmission of photonic quantum signals between the repeater nodes.We specifically focus on the two building blocks: remote entanglement generation and entanglement distillation.We then investigate various proof of principle quantum repeater schemes used for generating shared secret key between distant parties.The repeater schemes that we consider utilise one to three memory nodes capable of generating memory-photon entanglement.Finally, we introduce a novel framework for investigating a foundational aspect in the use of quantum communication related to the uncertainty principle.Efficient remote entanglement generation is an indispensable building block of most near-term quantum repeater networks.In this thesis we consider various remote entanglement generation schemes that permit multiplexing, which aims at increasing the throughput of this procedure.We find that for the specific schemes that are suitable for platforms with a single communication qubit and multiple memory qubits, the performance of the multiplexing approach is strongly dependent on the time it takes to perform local operations within the memory nodes.Entanglement distillation enables for filtering out the noise from imperfect entangled states using only local operations and classical communication.Using a general framework for optimising such schemes, which we have developed, we have proven optimality of specific generic and experimentally relevant distillation schemes.We have developed a general framework for optimising such schemes, which we have used to prove optimality of various generic and experimentally relevant distillation schemes.In designing proof of principle quantum repeater schemes we assume an informationtheoretic approach, which enables us to assess their performance in a hardware-agnostic way.We find that all the schemes that we consider can prove useful in specific parameter regimes for the nitrogen-vacancy centre platform.Moreover, we find that one scheme which has already been realised experimentally in the context of remote entanglement generation, is expected to significantly outperform every possible system based on direct communication without repeaters.However, our analysis shows that encapsulating the nitrogen-vacancy centres in optical cavities for the enhancement of the emission rates is a necessary requirement for such a successful demonstration of the first proofof-principle quantum repeater.xi xii SUMMARY Finally, we investigate the quantum uncertainty principle which is a fundamental feature of quantum mechanics, allowing for security in many quantum cryptographic protocols.We find that in a particular scenario, relevant from the perspective of quantum key distribution, a significant part of the observed uncertainty is in fact due to lack of information rather than intrinsic.If the eavesdropper could access that information, she would be able to much better, or in some cases even with certainty, guess the value of the raw bit of the generated key.

•Jun 11, 2019•6 citations
Quantum entanglement is central to many quantum technologies and is an indispensable ingredient of quantum information theory. These facts make the generation, characterization and quantification of entangled states unavoidable tasks, beside all their fundamental significance. As a particular example of such applications one may consider quantum metrology in which quantum entanglement is shown to have a significant role for beating the classical limits. However, generation, characterization and quantification of suitable entangled states are challenging tasks, in general.\n\nIn this dissertation, we introduce new platforms for engineering multipartite entangled states that are shown to be useful for quantum information processing and quantum metrology applications. In particular, we introduce new methods which can be used for generating N00N states, as one of the most challenging states to generate, enabling realization of such states in both photonic and spintronic architectures. We sketch a rather generic quantum circuit, for the N00N state generation, that could be realized in various quantum systems. Furthermore, we extend the platform for the generation of states beyond the N00N state. Typical examples of such sates could be entangled coherent or squeezed states, for instance, that of specific importance for quantum information and metrology applications. Furthermore, we extend the protocol for the multipartite state scenario. Also, we demonstrate that attaining the ultimate sensitivity in phase estimation is not an exclusive property of the N00N states. As a result, we find a large class of entangled states that could provide us with the ultimate sensitivity achieved by the N00N state.\n\nAs a part of our effort for the N00N state generation, we develop a new scheme where N00N states could be realized in two ensembles of nitrogen--vacancy (NV) centers in diamond. This could be interesting by noting the fact that NV centers in diamonds provide a remarkably long coherence time, even at the room temperature. This opens up new possibilities for protecting N00N states against decoherence.\n\nMoreover, having the long coherence time of the ensembles of the NV centers, we show that a hybrid quantum system consisting of three ensembles of NV centers coupled to a superconducting device enables the generation of controllable macroscopic multipartite entangled states, which could be used as a building block for quantum networks.\n\nFurthermore, we investigate entanglement of nonorthogonal states in details, and more specifically, we obtain a closed-form analytical expression for the entanglement degree of a multipartite qutrit state, that offers a quantitative measure for entanglement nnn-mode nonorthogonal qutrit states with an arbitrary nnn. Such higher dimensional entangled states could be useful in quantum communication protocols.\n\n Finally, we introduce a new configuration where any pair of quantum states can perfectly be swapped between two quantum resonators enabling a realization of a universal swap operation in photonics systems. This can serve as a building block of various quantum information processors.
The study of quantum mechanics, together with the ability to coherently control and manipulate quantum systems in the lab has led to a myriad of discoveries and real world applications. In this thesis we present experiments demonstrating precise control of an individual long-lived spin qubit as well as sensing applications for biology and investigation of quantum many-body dynamics.\n\nStable quantum bits, capable both of storing quantum information for macroscopic time scales and of integration inside small portable devices, are an essential building block for an array of potential applications. In the second chapter of this thesis we demonstrate high-fidelity control of a solid-state qubit, which preserves its polarization for several minutes and features coherence lifetimes exceeding 1 second at room temperature.\n\nSensitive probing of temperature variations on nanometer scales is an outstanding challenge in many areas of modern science and technology. In chapter three we show how nitrogen vacancy centers in diamond can be used as a robust, high sensitivity temperature probe. We furthermore demonstrate biological compatibility by introducing nano-sized diamonds into living cells and measuring externally induced sub-cellular temperature gradients.\n\nUnderstanding the dynamics of interacting many-body quantum systems with on-site potential disorder has proven one of the biggest challenges in quantum physics to investigate both in theory and experiment. In chapter four we demonstrate how coherent control techniques can be utilized to probe the many-body dynamics of a strongly interacting NV spin ensemble. Specifically, we show how a long-range interacting dipolar spin system exhibits characteristically slow thermalization in the presence of tunable disorder.\n\nThe presented works offer up many new areas to investigate, including complex quantum many-body effects of large, disordered spin systems, as well as applications of NV centers as bio-compatible nano-scale temperature probes.
Quantum entanglement is a kernel of quantum computation and quantum communication. We introduce a theoretical scheme to achieve the entanglement between two separated quantum nodes in a hybrid system. The proposed hybrid system based on diamond nitrogen-vacancy (NV) center spin ensemble is coherently coupled to a superconducting quantum circuit consisting of two quantum nodes and a quantum channel. Each node in our setup is composed of an NV center spin ensemble magnetically coupled to a superconducting coplanar resonator. The NV center spin ensemble composed of N identical and non-interacting NV spins, is placed in the magnetic field antinode of the superconducting coplanar resonator where the coupling is maximized. An array of superconducting quantum interference devices (SQUIDs) is inserted in the central conductor of resonator to make its frequency tunable with the magnetic flux threading through the SQUID loops. This flux is generated by passing current through an on-chip wire, so that the resonator can be brought in resonance with the NV center spins without changing their Zeeman splitting. Quantum qubits encoded into two separate nodes are connected by a vacuum superconducting coplanar resonator that is used as a quantum channel. This setup can potentially take the best elements of each individual system:NV center spin ensemble with longer coherence time capable of preparing, storing and releasing photonic quantum information, and the superconducting quantum circuits are easy to manipulate externally and can perform quantum logic gates to control quantum information rapidly. In order to realize the entanglement between two separated quantum nodes, firstly, we make a canonical transformation and obtain the Hamiltonian of the system that is reduced to two NV center spin ensembles resonantly coupled to a single mode of the superconducting coplanar resonator. Then we put forward the hybrid NV center spin-photon qubit encoding. In this hybrid encoding, the NV center spin and photon degrees of freedom enter on an equal footing into the definition of the qubit, in which case, quantum channel will switch on when three superconducting coplanar resonators are in resonance with each other, and all the manipulations can perform simply by tuning the frequencies of the superconducting coplanar resonators. Under the precise control of the evolution time, high fidelity entanglement between two separated quantum nodes is achieved. We show that this proposal can provide high fidelity quantum entanglement under realistic conditions, both in the resonant and the dispersive interaction cases. This hybrid quantum system will exhibit long coherence time and possess features like easy fabrication, integratability, and potential scalability. Furthermore, the quantum node composed of an NV center spin ensemble magnetically coupled to a superconducting coplanar resonator can be respectively integrated, which has practical applications in the realization of quantum information transmission and quantum entanglement among multiple quantum nodes.
One of the biggest challenges to implement quantum protocols and quantum information processing (QIP) is achieving long coherence times, usually requiring systems at ultra-low temperatures. The nitrogen-vacancy (NV) center in diamond is a promising alternative to this problem. Due to its spin properties, easy manipulation, and the possibility of doing optical state initialization and readout, it quickly became one of the best solid-state spin systems for QIP at room temperature. Here, we present the characterization of the spin-coherence of an ensemble of NV centers in an engineered sample of ultrapure diamond as a testbed for quantum protocols for quantum metrology.
Quantum computing and quantum communication have become the most popular research topic. Nitrogen-vacancy (NV) centers in diamond have been shown the great advantage of implementing quantum information processing. The generation of entanglement between NV centers represents a fundamental prerequisite for all quantum information technologies. In this paper, we propose a scheme to realize the high-fidelity storage and extraction of quantum entanglement information based on the NV centers at room temperature. We store the entangled information of a pair of entangled photons in the Bell state into the nuclear spins of two NV centers, which can make these two NV centers entangled. And then we illuminate how to extract the entangled information from NV centers to prepare on-demand entangled states for optical quantum information processing. The strategy of engineering entanglement demonstrated here maybe pave the way towards a NV center-based quantum network.
A quantumnetwork would allow the distribution of a quantum state over many spatially separated quantum nodes which individually possess the ability to generate, process and store quantum information. Connecting these nodes through quantum communication channels would enable sending quantum information over arbitrarily long distances, secret key distribution with guaranteed secure communication and distributed quantum computing. An appealing platform for implementation of quantum networks is the nitrogen-vacancy (NV) center in diamond. An NV center is an optically active defect in diamond created by the substitution of two adjacent carbon atoms in the diamond crystal matrix by a nitrogen atom and a neighboring vacancy. The NV center fits remarkably well in the described quantum network framework. Its electronic spin can be optically initialized, read out in a single shot, coherently manipulated and coupled to the nearby carbon-13 nuclear spins. These properties represent necessary ingredients of a multi-qubit quantum node. The possibility of the entanglement between the state of the NV center spin and a photon establishes a photonic quantum link which can enable the entanglement of the quantum nodes, forming a quantum network. First building blocks of the proposed quantum networks based on NV centers were demonstrated by performing entanglement between two distant NV centers separated by more than a kilometer. However, the current success rate of the entangling protocols is greatly reduced due to the low emission probability of the NV center photons into the resonant zero phonon line (ZPL) and the inefficient photon extraction from the diamond. This is the central problem which prevents promoting our experiments beyond proof-of-principle demonstration towards practical implementation of the proposed quantumnetworks. The goal of this thesis is tackling these issues by coupling NV centers to optical cavities which would greatly increase the rate of generation and collection of the ZPL photons through themechanism of Purcell enhancement. The design and the fabrication of the components constituting a diamond-basedFabry-Perot microcavity, as used in this thesis, are described in Chapter 4. For large enhancement of the NV center resonant emission, a low cavity mode volume is necessary. This is achieved by inserting a micrometers thin diamond slab into the cavity architecture; we present the fabrication details of such samples. Chapter 5 describes the fabrication of an integrated platform for microwave signal delivery to the NV centers within a diamond membrane in the cavity architecture. Microwave striplines and arrays of unique markers are embedded in the mirror onto which the diamond is bonded. We investigate the mirror optical properties post fabrication and find that the fabrication method preserves the mirror optical performance. We describe the diamond bonding method and demonstrate addressing of the NV center spin. In Chapter 6 we probe the properties of the cavity with the embedded diamond membrane through measurements of the cavity finesse. We investigate the cavity finesse dependence on length, mode structure and temperature. We further explore the operation at cryogenic temperatures by probing the effect of cryostation vibration on the cavity linewidth. Finally, in Chapter 7 we discuss ways of improving the existing experimental capabilities, outline the first steps for demonstrating enhancement of the NV center resonant emission and suggest future experiments that can be performed with this system. We conclude that coupling of the NV centers to the cavities developed in this research could lead to an increase of remote entanglement success rates by more than three orders of magnitude.
Future quantum networks will enable the realisation of a large family of quantum protocols, hence allowing for implementation of various tasks ranging from quantum cryptography through quantum computing to quantum metrology.In this thesis we analyse and develop the building blocks of quantum repeater networks.These networks consist of quantum repeater nodes, which are equipped with quantum memories enabling storage of quantum information.The repeater nodes are connected using optical fibres that enable for the transmission of photonic quantum signals between the repeater nodes.We specifically focus on the two building blocks: remote entanglement generation and entanglement distillation.We then investigate various proof of principle quantum repeater schemes used for generating shared secret key between distant parties.The repeater schemes that we consider utilise one to three memory nodes capable of generating memory-photon entanglement.Finally, we introduce a novel framework for investigating a foundational aspect in the use of quantum communication related to the uncertainty principle.Efficient remote entanglement generation is an indispensable building block of most near-term quantum repeater networks.In this thesis we consider various remote entanglement generation schemes that permit multiplexing, which aims at increasing the throughput of this procedure.We find that for the specific schemes that are suitable for platforms with a single communication qubit and multiple memory qubits, the performance of the multiplexing approach is strongly dependent on the time it takes to perform local operations within the memory nodes.Entanglement distillation enables for filtering out the noise from imperfect entangled states using only local operations and classical communication.Using a general framework for optimising such schemes, which we have developed, we have proven optimality of specific generic and experimentally relevant distillation schemes.We have developed a general framework for optimising such schemes, which we have used to prove optimality of various generic and experimentally relevant distillation schemes.In designing proof of principle quantum repeater schemes we assume an informationtheoretic approach, which enables us to assess their performance in a hardware-agnostic way.We find that all the schemes that we consider can prove useful in specific parameter regimes for the nitrogen-vacancy centre platform.Moreover, we find that one scheme which has already been realised experimentally in the context of remote entanglement generation, is expected to significantly outperform every possible system based on direct communication without repeaters.However, our analysis shows that encapsulating the nitrogen-vacancy centres in optical cavities for the enhancement of the emission rates is a necessary requirement for such a successful demonstration of the first proofof-principle quantum repeater.xi xii SUMMARY Finally, we investigate the quantum uncertainty principle which is a fundamental feature of quantum mechanics, allowing for security in many quantum cryptographic protocols.We find that in a particular scenario, relevant from the perspective of quantum key distribution, a significant part of the observed uncertainty is in fact due to lack of information rather than intrinsic.If the eavesdropper could access that information, she would be able to much better, or in some cases even with certainty, guess the value of the raw bit of the generated key.