Measurements play a pivotal role in the advance of science and technology. To name just two examples, the global positioning system (GPS) technology relies on atomic clocks, and the detection of gravitational waves has been achieved via extremely precise interferometric measurements. The aim of my thesis is to contribute towards the goal of doing quantum metrology with nanophotonic structures. With this motivation, some problems across the fields of nanophotonics and quantum optics are tackled. First, the role of helicity within nanophotonics is explored. In the context of symmetries and conserved quantities, helicity, the projection of the total angular momentum on the linear momentum direction, is a useful addition to the more commonly considered quantities such as angular momentum. A simple but versatile experimental treatment of helicity is introduced and demonstrated on the scattering of focused light by circular nanoholes in a gold film. The helicity transformation that takes place in this light-matter interaction is studied. Another section is devoted to the topic of quantum light sources. It is shown how to influence and measure the spectrotemporal wave function of photon pairs by exploiting properties of the spontaneous parametric down-conversion (SPDC) process. The proposed technique also allows to determine the distribution of time delays between the two photons in a pair, which is typically a challenging experimental task. Finally, a quantum metrology experiment on the interaction of light with chiral molecules is presented. In this proof-of-concept experiment entangled photon pairs are used for the measurement of natural optical activity and its wavelength dependence, the optical rotatory dispersion.
Measurements play a pivotal role in the advance of science and technology. To name just two examples, the global positioning system (GPS) technology relies on atomic clocks, and the detection of gravitational waves has been achieved via extremely precise interferometric measurements. The aim of my thesis is to contribute towards the goal of doing quantum metrology with nanophotonic structures. With this motivation, some problems across the fields of nanophotonics and quantum optics are tackled. First, the role of helicity within nanophotonics is explored. In the context of symmetries and conserved quantities, helicity, the projection of the total angular momentum on the linear momentum direction, is a useful addition to the more commonly considered quantities such as angular momentum. A simple but versatile experimental treatment of helicity is introduced and demonstrated on the scattering of focused light by circular nanoholes in a gold film. The helicity transformation that takes place in this light-matter interaction is studied. Another section is devoted to the topic of quantum light sources. It is shown how to influence and measure the spectrotemporal wave function of photon pairs by exploiting properties of the spontaneous parametric down-conversion (SPDC) process. The proposed technique also allows to determine the distribution of time delays between the two photons in a pair, which is typically a challenging experimental task. Finally, a quantum metrology experiment on the interaction of light with chiral molecules is presented. In this proof-of-concept experiment entangled photon pairs are used for the measurement of natural optical activity and its wavelength dependence, the optical rotatory dispersion.
Nano-engineering is crucial in realizing compact photonic systems for light routing and conditioning with ever more complex optical functions. It also promises to elevate the precision of experiments in high-precision optical metrology to an unprecedented level, e.g., optical atomic clocks and gravitational wave detectors - the most precise experiments ever developed by humankind. In this contribution, I give an overview of the development and possibilities of nanophotonic devices for applications in precision optical experiments. I explain relevant physical phenomena of light-matter interaction and illustrate the role of material properties in these experiments.
The quantum description of light offers a unique set of optical effects that has led to promising applications beyond those described by classical physics. Although well-defined quantum states of light do not persist in typical classical environments, phenomena such as entanglement often enhance optical approaches to communication, measurement, and sensing. With the emergence of new tasks in classical and quantum optical technology, new tools are required that must be specifically engineered including the generation of quantum states. This thesis is concerned with three principle tasks in engineering and implementing entangled photonic states. First, the use of frequency anti-correlated and polarization entangled two-photon states generated during spontaneous parametric down conversion (SPDC) to precisely evaluate optical delays with quantum interferometry is demonstrated in a realistic commercially available optical telecommunication device. Second, the study of correlated orbital angular momentum (OAM) states for efficient object identification is presented. Finally, experimental efforts towards the development of sources for entangled weak coherent states are discussed. The generation of broadband entangled states leading to well-defined second order interference patterns is a necessary step for the application of low coherence quantum interferometry as a metrological device. The flexibility of non-uniformly chirped periodically poled nonlinear crystals offers a rich set of tools for precise state engineering. The experimental evaluation of a broadband source of polarization entanglement is presented. In addition, design considerations for applications that require optimized quantum interference features are discussed along with a numerical investigation of the limits of quantum interferometry with even order dispersion cancellation. We present an experimental demonstration of correlated OAM sensing exploiting the two-dimensional and correlated nature of states produced during SPDC projected onto the OAM basis. Efficient object recognition through the identification of azimuthal symmetries of arbitrary objects is achieved by observing the full two-photon joint OAM spectrum and focusing on non-conserved OAM components not found in the natural OAM spectrum of SPDC. Finally, quantum key distribution (QKD) is currently the most successful quantum optical application; however, a limiting trade off between the achievable rates and distances confines the approach to niche applications. The generation of entangled coherent states has been proposed to transition QKD into a new regime that would set aside single photons and two-photon entangled states for higher intensity coherent pulses. The key technical limitation that has prohibited the demonstration of such states is a reliable source of single-photon cross phase modulation. The plausibility and experimental efforts towards creating such an environment in a solid state device is presented.
The aim of this thesis is to explore nonlinear nanostructures – photonic systems with one or more dimension with nanoscale feature size – as new platforms for parametric photon-pair generation. This is motivated by the need for photon-pair sources in many technological applications of quantum optics, such as quantum communication, imaging and computing. The initial hypothesis is that nonlinear nanostructures are a promising platform to complement established photon-pair source schemes based on bulk crystals or photonic integrated circuits in terms of quantum state-engineering, footprint, functional density etc. However, nonlinear pair generation, e.g. via spontaneous parametric down-conversion (SPDC), is a new subfield in nanophotonics with a very limited number of studies existing. This constitutes the knowledge-gap addressed in this thesis. Therefore, the objective is to provide first experimental demonstrations of SPDC in subwavelength-scale and nonlinear nanostructures. We investigate the ability of such systems to control the properties of two-photon quantum states such as frequency and angular spectrum or polarization entanglement. To this end we analyze nanostructures with different degrees of complexity, starting with an unstructured thin crystal with one nanoscale dimension, leading up to a 3D nano-scale resonator with subwavelength-sized features in all dimensions. Furthermore, we test different types of nonlinear materials such as lithium niobate, group III-V semiconductors and emerging, highly nonlinear materials such as molybdenum disulfide. Additionally, we also advance the theoretical understanding by developing a comprehensive model of the quantum process of nonlinear parametric pair-generation in photonic nanostructures.
The measurement of physical quantities and measurement units standard promote the development of metrology. Especially, the developments of laser interference and atomic frequency standard bring a revolutionary leap for metrology. Many precision measurement techniques have been proposed and experimentally demonstrated, such as gravitational wave measurements and laser gyroscopes based on laser interferometry, and atomic clocks and atomic gyroscopes based on the atom interferometry. Recently, a new branch of science, quantum metrology, has grown up to further explore and exploit the quantum techniques for precision measurement of physical quantities.#br#This paper will focus on recent developments in quantum metrology and interference based on coherence and correlation of light and atom. Firstly, we briefly review the development of metrology. Then, we introduce our own researches in recent years, including quantum-correlation SU(1,1) optical interferometer based on four wave mixing process in atomic vapor and the atom-light hybrid interferometer based on Raman scattering in atomic vapor.#br#Interferometer is a powerful tool to measure physical quantities sensitive to the inference wave with high precision, and has been widely used in scientific research, industry test, navigation and guidance system. For example, the laser interferometer is able to measure optical phase sensitive quantities, including length, angular velocity, gravitational wave and so on. Meanwhile, the atom interferometer is sensitive to the change of atomic phase caused by the light, gravity, electric and magnetic fields. As a new type of interferometry, the atom-light hybrid interferometer, is sensitive to both the optical phase and atomic phase. Furthermore, SU(1,1) interferometer and nonlinear atom-light hybrid interferometer have the ability to beat the standard quantum limit of phase sensitivity. Quantum interference technology, whose phase measurement accuracy can break through the limit of standard quantum limit, is the core of quantum metrology and quantum measurement technology.
The fields of quantum and nonlinear optics have given rise to a variety of nonclassical states of light that have been proven to surpass certain limitations set by classical physics. Namely, certain squeezed and entangled states have been shown to beat the shot-noise limit when making precision phase measurements in interferometry, as well as write lithographic patterns that are smaller than classically allowed by the Rayleigh diffraction limit. Additionally, single-photon sources and entangled photon pairs have given rise to provably secure quantum key distribution for cryptography. Producing these quantum states of light has proven a difficult task. Nonlinear crystals, when pumped by a laser, produce pairs of single photons via the process of spontaneous parametric down conversion (SPDC). This process is mediated by the second order nonlinear susceptibility of the material. When pumped in a high gain regime, these crystals give rise to optical parametric amplification, which is a viable source of squeezed light. The vast majority of research in this area has focused on crystals that are seeded by vacuum in their two modes. This dissertation concerns the field of quantum nonlinear optics. It is an investigation into the processes that occur when nonlinear materials interact with the electromagnetic field on the single photon level. I have focused on seeding nonlinear crystals with quantum states of light, including single photons and entangled states. This process results in various states directly applicable to interferometry, imaging, and cryptography. Another application investigated is an absolute radiance measurement via stimulated parametric down conversion resulting from non-vacuum seeding of a nonlinear crystal. Additionally, other nonlinear processes, including four-wave mixing, nonlinear magneto-optical effects and coherent population trapping in warm atomic vapor involving quantum states of light are investigated. The process of seeding third-order nonlinear interactions, such as in atomic vapors, gives rise to a variety of interesting, nonclassical phenomena such as entangled image transfer and nonlocal imaging. Strong analogies between SPDC and four-wave mixing are drawn. I also experimentally show an all optical pi-only phase shift of one light beam via another in warm Cesium vapor.
Summary form only given. Controlling the interaction of light and matter is the basis for diverse applications ranging from light technology to quantum information processing. Nowadays, many of these applications are based on nanophotonic structures. It turns out that the confinement of light in such nanostructures imposes an inherent link between its local polarization and its propagation direction, also referred to as spin-momentum locking of light [1]. Remarkably, this leads to chiral, i.e., propagation direction-dependent effects in the emission and absorption of light, and elementary processes of light-matter interaction are fundamentally altered. For example, when coupling plasmonic particles or atoms to evanescent fields, the intrinsic mirror symmetry of the particles' emission can be broken. In our group, we observed this effect in the interaction between single rubidium atoms and the evanescent part of a light field that is confined by continuous total internal reflection in a whispering-gallery-mode microresonator [2]. In the following, this allowed us to realize chiral nanophotonic interfaces in which the emission direction of light into the structure is controlled by the polarization of the excitation light [3] or by the internal quantum state of the emitter [4], respectively. Moreover, we employed this chiral interaction to demonstrate an integrated optical isolator [5] as well as an integrated optical circulator [6] which operate at the single-photon level and which exhibit low loss. The latter are the first two examples of a new class of nonreciprocal nanophotonic devices which exploit the chiral interaction between single quantum emitters and transversally confined photons.