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International Electronic Conference on Applied Sciences (ASEC)

Statistical Measures for the Dynamical Atom-Field Coupling Constants

Abu Mohamed Alhasan

Published Nov 9, 2020• 1 citation
Publisher

Abstract

We establish a statistical-measures approach to describe the spectral-spatial analysis of the dynamical atom-field couplings associated with two-pair of pulses propagation in multilevel atomic media. The statistical measures are functional measures that depend on the collective coupling as well as on the eigenvalues of the Nonlinear-Liouville equation. The Nonlinear-Liouville equation is a nonlinear evolution equation which is a second-order differential equation in time. It describes the multi-wave mixing process within the atomic system, as well as coherent oscillations. The proposed spectral estimators prevail spatial multi-peak structure, which depends on the reduction or the enhancement of an effective Rabi-frequency. Decomposition of collective oscillations provides an intuitive guess to special-weight of the field's area. We introduce two functional wavelets to simulate the atomic polarization response. One of these functionals exposes the dependence on the multicomponent sine-Gordon equation for the atomic polarization, which is adequate at relatively small propagation distances. The second one is composed of combined sine and cosine functionals on the area of the fields. The cosine functional reflects the significance of the atomic inversion on the polarization response to electromagnetic field excitations. The proposed functional-wavelets inducts new sources for soliton features to the transition-radiation propagation associated with Maxwell-Bloch equations.

DOI
10.3390/asec2020-07618

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We establish a statistical-measures approach to describe the spectral-spatial analysis of the dynamical atom-field couplings associated with two-pair of pulses propagation in multilevel atomic media. The statistical measures are functional measures that depend on the collective coupling as well as on the eigenvalues of the Nonlinear-Liouville equation. The Nonlinear-Liouville equation is a nonlinear evolution equation which is a second-order differential equation in time. It describes the multi-wave mixing process within the atomic system, as well as coherent oscillations. The proposed spectral estimators prevail spatial multi-peak structure, which depends on the reduction or the enhancement of an effective Rabi-frequency. Decomposition of collective oscillations provides an intuitive guess to special-weight of the field's area. We introduce two functional wavelets to simulate the atomic polarization response. One of these functionals exposes the dependence on the multicomponent sine-Gordon equation for the atomic polarization, which is adequate at relatively small propagation distances. The second one is composed of combined sine and cosine functionals on the area of the fields. The cosine functional reflects the significance of the atomic inversion on the polarization response to electromagnetic field excitations. The proposed functional-wavelets inducts new sources for soliton features to the transition-radiation propagation associated with Maxwell-Bloch equations.
Microscopic models based on multilevel atoms are central to optimizing nonlinear optical responses and the coherent control of light. These models are traditionally based on single-atom effects that are parametrically extrapolated to include collective effects, such as an enhanced response or propagation within atomic media. In this work, we present a systematic analysis of the cooperative effects arising in driven systems composed of multilevel atoms coupled via a common electromagnetic environment. The analysis is based on an interplay between dressed states induced by the driving field and photon exchanges, and collective decay channels. This theory is applied to the case of four-wave mixing induced by a pair of lasers acting on an atomic pair with internal levels in the diamond configuration. The effect of interatomic correlations and collective decay over the photons created in this nonlinear process is then explored. We identify three regions of operation: (i) laser-dominated, (ii) intermediate, and (iii) dipole-dominated. The dependence of single- and two-photon correlations is studied in detail for each region by varying atomic orientations and laser parameters consistent with current experiments involving atomic gases. Photonic correlation functions are shown to exhibit a transition from a Lorentz-like dependence on the two-photon detuning—with general features that can be obtained in an isolated atom scheme—to a two-peaked distribution when the dipole-dipole interactions become relevant. For weak Rabi frequencies whose value is smaller than the highest collective decay rate, the atoms are trapped inside their ground state as they approach each other. It is found that the anisotropy of the dipole-dipole interaction and its wave nature are essential to understand the behavior of the photon correlations. Signatures of these processes are identified for existing experimental realizations. The intuition obtained from this connection helps to uncover relevant parameters that could be exploited for quantum control protocols based on dispersive and dissipative cooperative effects in multilevel systems.
We consider the interaction between a classical time-varying electric field and the atomic electrical dipole moment operator of a finite state atom and calculate approximately the mixed state evolution of the atom with such an interaction Hamiltonian up to quadratic orders in the external classical electric field using Schrodinger’s equation for mixed state evolution. From this approximate expression for the state evolution, we evaluate the average atomic electric dipole moment as a linear-quadratic function of the electric field. Later on, we also take into account Brownian motion bath noise that couples to the atomic dynamics, so that the Schrodinger equation dynamics gets modified to the Lindblad dynamics of an open quantum system, i.e., the master equation. From the average atomic dipole moment, we obtain an expression for the average polarization field of atoms constituting the medium through which the classical electromagnetic wave propagates. This average polarization is a linear-quadratic causal functional of the electric field. The resulting Maxwell equations for wave propagation, taking into account this polarization current density, thus acquire a quadratic nonlinearity which can be used to explain higher harmonic frequencies at the output of an optical fiber when the input is excited by the electric field coming from a monochromatic laser. We are then also able to calculate the mean square fluctuations in the polarization field using the evolving atomic state, and hence the electric field propagating through the medium of atoms acquires quantum fluctuations which can be used to explain time-varying random shifts in the spectral lines. As mentioned above, we include in this article an extension of this problem to the case when there is white Gaussian noise corrupting the state evolution dynamics of the atom and also the case when there is a pairwise interaction between the spin dipoles of atoms at two different locations. In the former case, we derive an approximate formula for the polarization field as well as its temporal statistical correlations, and we show how this computation can be extended to the latter case too. When there is a pairwise interaction between the atomic spins, we use a version of the approximate quantum Boltzmann equation to calculate the first and second order marginals of the atomic states, which is then used to compute the average polarization as well as its spatio-temporal correlations. Temporal correlations using second marginals of the atomic states cannot be computed using classical probabilistic methods owing to Heisenberg uncertainty, so we propose a sequential measurement-based strategy involving computation of the joint probabilities of the atomic spin components at two different times by first measuring one component of the spin, allowing for state collapse, and then following it up with nonlinear time evolution from the collapsed two-particle state using the quantum Boltzmann equation, followed further by measurement of another component of the spin at the second time.
We consider the propagation of ultrashort optical solitons in media described by a general Hamiltonian of multilevel atoms. Assuming that all transition frequencies of the medium are well below the typical wave frequency, i.e., only the contribution of infrared transitions is taken into account, we use a short-wave approximation and a rigorous application of the reductive perturbation formalism to derive a cumbersome coupled system of nonlinear partial differential equations describing ultrashort soliton evolution in such systems. The rather complicated set of coupled equations can be simplified to a generic double-sine-Gordon equation for a special case of identical three-level atoms, whereas for a special case of identical four-level atoms the system of coupled equations can be reduced to a generalized double-sine-Gordon equation. Numerical simulations showing the formation of robust breather-type solutions of both the standard double-sine-Gordon and of the generalized double-sine-Gordon equations from sinusoidal inputs with Gaussian envelopes are also presented.
We consider the interaction of electromagnetic radiation of arbitrary polarization with multilevel atoms in a self-consistent manner, taking into account both spatial and temporal dependencies of local fields. This is done by numerically solving the corresponding system of coupled Maxwell-Liouville equations for various geometries. In particular, we scrutinize linear optical properties of nanoscale atomic clusters, demonstrating the significant role played by collective effects and dephasing. It is shown that subwavelength atomic clusters exhibit two resonant modes, one of which is localized slightly below the atomic transition frequency of an individual atom, while the other is positioned considerably above it. As an initial exploration of future applications of this approach, the optical response of core-shell nanostructures, with a core consisting of silver and a shell composed of resonant atoms, is examined.
In this theoretical paper, we investigate coherence properties of the near-resonant light scattered by two atoms exposed to a strong monochromatic field. To properly incorporate saturation effects, we use a quantum Langevin approach. In contrast to the standard optical Bloch equations, this method naturally provides the inelastic spectrum of the radiated light induced by the quantum electromagnetic vacuum fluctuations. However, to get the right spectral properties of the scattered light, it is essential to correctly describe the statistical properties of these vacuum fluctuations. Because of the presence of the two atoms, these statistical properties are not Gaussian: (i) the spatial two-points correlation function displays a specklelike behavior and (ii) the three-points correlation function does not vanish. We also explain how to incorporate in a simple way propagation with a frequency-dependent scattering mean-free path, meaning that the two atoms are embedded in an average scattering dispersive medium. Finally we show that saturation-induced nonlinearities strongly modify the atomic scattering properties and, as a consequence, provide a source of decoherence in multiple scattering. This is exemplified by considering the coherent backscattering configuration where interference effects are blurred by this decoherence mechanism. This leads to a decrease of the so-called coherent backscattering enhancement factor.