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Theory of Microwave to Optical Photon Upconversion Using Erbium Doped Crystals

Peter S. Barnett

Published Jan 1, 2020• 1 citation
OpenAlex

Abstract

The subject of this thesis is coherent conversion from microwave photons to optical photons. This has applications for quantum computing, and would allow interfacing between superconducting qubits and optical fibres. Specifically, we will focus on photon conversion via erbium ions in a doped crystal. \n\nWe model a device which has an erbium doped crystal inside overlapping microwave and optical cavities. Input microwave photons are combined with photons from an optical pump laser via interactions with the erbium ions. This will produce optical output photons carrying the same quantum information as the input microwave photons. We develop a description of the interaction between the atoms and the light fields, accounting for both loss effects in the single atoms, and inhomogeneous broadening of the ensemble. Our theory is compared with experimental data, and shows good agreement. \n \nWe explore various phenomena which arise in this system, including the effects of temperature and microwave power. \n\nIt is shown that the description of this device from earlier work is not valid in the regime where the conversion efficiency is greatest. Hence, this work is necessary to be able to predict the maximum conversion efficiency. \n\nWe develop a linearised model which is accurate in the regime where the microwave and optical fields are small, such as the regime used for quantum information. This model is used to maximise the photon number conversion efficiency of the device. We predict conversion efficiencies above 20%, far higher than has been achieved experimentally with using rare earth ions. Modifying our device should further increase the conversion efficiency to above 80%.

Related papers

Theory of microwave-optical conversion using rare-earth-ion dopants

Peter S. Barnett, Jevon J. Longdell

We develop a theoretical description of a device for coherent conversion of microwave-to-optical photons. For the device, dopant ions in a crystal are used as three-level systems, and interact with the fields inside overlapping microwave and optical cavities. We develop a model for the cavity fields interacting with an ensemble of ions and model the ions using an open quantum systems approach, while accounting for the effect of inhomogeneous broadening. Numerical methods are developed to allow us to accurately simulate the device. We also further develop a simplified model, applicable in the case of small cavity fields, which is relevant to quantum information applications. This simplified model is used to predict the maximum conversion efficiency of the device. We investigate the effect of various parameters, and predict that conversion efficiency of above 80% should be possible with currently existing experimental setups inside a dilution refrigerator.

arXiv:2008.10834•Physical Review A•Dec 23, 2020•11 citations

Coherent Frequency Conversion from Microwave to Optical Fields in an Erbium Doped Y2SiO5 Crystal: Towards the Single Photon Regime

Xavier Fernandez-Gonzalvo

In the context of quantum information technologies superconducting qubits (SQs) are very attractive devices for the manipulation of quantum states, and present themselves as one of our best candidates to build a quantum processor. They couple naturally to microwave photons, for which suitable quantum memories or a long distance propagation channel don’t exist. A way around these limitations is to turn these microwave photons into optical ones by building a quantum frequency converter: a device by which the frequency of a photon can be changed while preserving its non-classical correlations. Then, optical fibres could be used to link distant SQ-based devices together, facilitating the creation of a network of quantum computers. Moreover, SQs could then be coupled to quantum memories compatible with photons at optical frequencies, which are the most well developed kind of quantum memories at the present time. This thesis explores the possibility to convert single microwave photons into optical photons using erbium doped in a yttrium orthosilicate crystal (Er3+:Y2SiO5). Er3+:Y2SiO5 is a good candidate because it has a naturally occurring optical transition near 1536 nm close to the point where silica optical fibres show their minimum loss. A microwave transition can be found in two different ways: one way is to use the 167 isotope of erbium, which is the only stable isotope that shows hyperfine splitting as it has non-zero nuclear spin. The hyperfine structure of the ground state of 167Er3+:Y2SiO5 spans over about 5 GHz. The other possibility is to use the other stable isotopes of erbium and Zeeman split their ground state using an external magnetic field. A microwave transition near 5 GHz can be achieved with moderate magnetic fields due to the high 𝑔-factors of Er3+:Y2SiO5. The physical process of interest is a three wave mixing process involving two fields at optical frequencies and one field at microwave frequencies. In order to boost the efficiency of the frequency conversion process the Er3+:Y2SiO5 crystal is placed inside a microwave and an optical resonator. The problem is first explored from the theoretical point of view, where a nonlinear coefficient Λ(2) is derived (analogous to the 𝜒(2) often used in nonlinear optics), and the interaction between cavity modes and the nonlinear medium is studied. It is predicted that with a sample cooled down to millikelvin temperatures total frequency conversion between microwave and optical fields can be achieved. A preliminary hole burning spectroscopy experiment is performed with the objective of reconstructing the hyperfine structure of the excited state of 167Er3+:Y2SiO5, but the complexity of the problem makes it too difficult to achieve this goal. Then a series of experiments are shown, aimed at determining whether or not frequency conversion at the single photon level is achievable using the even isotopes of erbium in a magnetic field. These experiments are based in the Raman heterodyne spectroscopy technique, which is used in combination with electron paramagnetic resonance and optical absorption spectroscopy. In all experiments the sample is cooled down to cryogenic temperatures near 4 K. A first experiment shows that the frequency conversion process exists in Er3+:Y2SiO5, in a setup where only a microwave resonator is used, but not an optical one. A second experiment is performed in a similar setup, this time presenting a quantitative study of the properties of the frequency conversion process, and its comparison with the theoretical model previously derived. A third experiment is performed, which incorporates an optical cavity to the system. The interaction between the erbium ions and the optical cavity introduces a whole new range of experimental complications, which are studied and discussed. Then, the frequency conversion signal is studied anew, showing an unexpected highly non-linear scaling behaviour with the input powers. A hypothesis explaining this unexpected behaviour is given, referring to stray optical absorption in the inhomogeneous line of Er3+:Y2SiO5 (and in particular 167Er3+:Y2SiO5), which can be bleached out under certain circumstances due to spectral hole burning effects. The overall maximum frequency conversion efficiency observed is of 3 × 10^−4 per Watt of pump laser power. While this value is still far from the target several ways of improvement are proposed, including cooling down the system to millikelvin temperatures, increasing the dopant concentration and modifying the geometry of the resonators.

•Jan 1, 2017•1 citation

Quantum nanophotonic devices based on rare-earth-doped crystals (Conference Presentation)

Andrei Faraon, Tian Zhong, Jonathan M. Kindem +4 more

Quantum light-matter interfaces that reversibly map the quantum state of photons onto the quantum states of atoms, are essential components in the quantum engineering toolbox with applications in quantum communication, computing, and quantum-enabled sensing. In this talk I present our progress towards developing on-chip quantum light-matter interfaces based on nanophotonic resonators fabricated in rare-earth-doped crystals known to exhibit the longest optical and spin coherence times in the solid state. We recently demonstrated coherent control of neodymium (Nd3+) ions coupled to yttrium orthosilicate Y2SiO5 (YSO) photonic crystal nano-beam resonator. The coupling of the Nd3+ 883 nm 4I9/2-4F3/2 transition to the nano-resonator results in a 40 fold enhancement of the transition rate (Purcell effect), and increased optical absorption (~80%) - adequate for realizing efficient optical quantum memories via cavity impedance matching. Optical coherence times T2 up to 100 μs with low spectral diffusion were measured for ions embedded in photonic crystals, which are comparable to those observed in unprocessed bulk samples. This indicates that the remarkable coherence properties of REIs are preserved during nanofabrication process. Multi-temporal mode photon storage using stimulated photon echo and atomic frequency comb (AFC) protocols were implemented in these nano-resonators. Our current technology can be readily transferred to Erbium (Er) doped YSO devices, therefore opening the possibility of efficient on-chip optical quantum memory at 1.5 μm telecom wavelength. Integration with superconducting qubits can lead to devices for reversible quantum conversion of optical photons to microwave photons.

•Apr 28, 2017•0 citations

Toward Microwave-to-Optical Conversion using Erbium Doped Crystals and Integrated Resonators

Jake Rochman, John G. Bartholomew, Ioana Craiciu +5 more

We present progress towards a bidirectional coherent microwave-to-optical photon converter using an ensemble of rare-earth ions coupled to integrated photonic and microwave resonators.

Conference on Lasers and Electro-Optics•May 5, 2019•0 citations

Toward Microwave-to-Optical Conversion using Erbium Doped Crystals and Integrated Resonators

Jake Rochman, John G. Bartholomew, Ioana Craiciu +5 more

We present progress towards a bidirectional coherent microwave-to-optical photon converter using an ensemble of rare-earth ions coupled to integrated photonic and microwave resonators.

Conference on Lasers and Electro-Optics•Jan 1, 2019•0 citations

Investigation of Fully Concentrated Rare-Earth Crytals for Microwave Upconversion

Jonathan R. Everts

Superconducting qubits are currently one of the leading qubit designs, showing great success in some of the world's most powerful quantum computers. Superconducting qubits, however, communicate at microwave frequencies, which is problematic when it comes to the task of long distance communication as unless the communication channel is cryogenically cooled the microwave photons are swamped by thermal noise. Optical photons, on the other hand, are ideal for long distance communication, particularly at frequencies that lie within the telecommunications band. One solution to the superconducting qubits communication problem is to create a device that can convert an input microwave photon into an optical photon with unit quantum efficiency. A device of such could then be used alongside existing optical fibre networks to connect distant superconducting processors. Furthermore, an upconversion device would allow superconducting qubit systems to take advantage of quantum technologies in the optical region, such as optical quantum memories.\n\nSeveral different approaches have been taken in attempts to experimentally implement such a device. Recently a theoretical proposal showed that the strong non-linearities that occur near the collective resonances in fully concentrated rare-earth crystals can be used to efficiently upconvert microwave photons. In this thesis we begin experimental investigations of two fully concentrated rare-earth crystals, GdVO4 and DyPO4, for their application to microwave upconversion.\n\nAbsorption spectra of the two crystals in the optical region are measured using a Fourier transform infrared spectrometer, in order to characterise and explore the possible optical states to be used in the upconversion process. Experiments are then carried out at microwave frequencies to explore the coupling between the collective spin resonances (magnons) that occur within the crystals and a microwave cavity. It is found that not only can the ultrastrong coupling regime be reached in these systems but that the linewidth of the magnon mode is narrow, measuring 35MHz at T = 25mK. This is the first experimental evidence of ultrastrong coupling between a microwave cavity and antiferromagnetic magnon modes in a rare-earth crystal. Furthermore, narrow transition linewidths are a crucial requirement in the proposed upconversion method, therefore the narrow linewidth experimentally measured here is an important validation of the proposals feasibility. \n\nThe results presented in this thesis show that microwave upconversion mediated by fully concentrated rare-earth crystals has an exciting future. Perhaps one day rare-earth crystals will be used to overcome the major communication problem superconducting qubits currently face.

•Jan 1, 2020•0 citations
The subject of this thesis is coherent conversion from microwave photons to optical photons. This has applications for quantum computing, and would allow interfacing between superconducting qubits and optical fibres. Specifically, we will focus on photon conversion via erbium ions in a doped crystal. \n\nWe model a device which has an erbium doped crystal inside overlapping microwave and optical cavities. Input microwave photons are combined with photons from an optical pump laser via interactions with the erbium ions. This will produce optical output photons carrying the same quantum information as the input microwave photons. We develop a description of the interaction between the atoms and the light fields, accounting for both loss effects in the single atoms, and inhomogeneous broadening of the ensemble. Our theory is compared with experimental data, and shows good agreement. \n \nWe explore various phenomena which arise in this system, including the effects of temperature and microwave power. \n\nIt is shown that the description of this device from earlier work is not valid in the regime where the conversion efficiency is greatest. Hence, this work is necessary to be able to predict the maximum conversion efficiency. \n\nWe develop a linearised model which is accurate in the regime where the microwave and optical fields are small, such as the regime used for quantum information. This model is used to maximise the photon number conversion efficiency of the device. We predict conversion efficiencies above 20%, far higher than has been achieved experimentally with using rare earth ions. Modifying our device should further increase the conversion efficiency to above 80%.
We develop a theoretical description of a device for coherent conversion of microwave-to-optical photons. For the device, dopant ions in a crystal are used as three-level systems, and interact with the fields inside overlapping microwave and optical cavities. We develop a model for the cavity fields interacting with an ensemble of ions and model the ions using an open quantum systems approach, while accounting for the effect of inhomogeneous broadening. Numerical methods are developed to allow us to accurately simulate the device. We also further develop a simplified model, applicable in the case of small cavity fields, which is relevant to quantum information applications. This simplified model is used to predict the maximum conversion efficiency of the device. We investigate the effect of various parameters, and predict that conversion efficiency of above 80% should be possible with currently existing experimental setups inside a dilution refrigerator.
In the context of quantum information technologies superconducting qubits (SQs) are very attractive devices for the manipulation of quantum states, and present themselves as one of our best candidates to build a quantum processor. They couple naturally to microwave photons, for which suitable quantum memories or a long distance propagation channel don’t exist. A way around these limitations is to turn these microwave photons into optical ones by building a quantum frequency converter: a device by which the frequency of a photon can be changed while preserving its non-classical correlations. Then, optical fibres could be used to link distant SQ-based devices together, facilitating the creation of a network of quantum computers. Moreover, SQs could then be coupled to quantum memories compatible with photons at optical frequencies, which are the most well developed kind of quantum memories at the present time. This thesis explores the possibility to convert single microwave photons into optical photons using erbium doped in a yttrium orthosilicate crystal (Er3+:Y2SiO5). Er3+:Y2SiO5 is a good candidate because it has a naturally occurring optical transition near 1536 nm close to the point where silica optical fibres show their minimum loss. A microwave transition can be found in two different ways: one way is to use the 167 isotope of erbium, which is the only stable isotope that shows hyperfine splitting as it has non-zero nuclear spin. The hyperfine structure of the ground state of 167Er3+:Y2SiO5 spans over about 5 GHz. The other possibility is to use the other stable isotopes of erbium and Zeeman split their ground state using an external magnetic field. A microwave transition near 5 GHz can be achieved with moderate magnetic fields due to the high 𝑔-factors of Er3+:Y2SiO5. The physical process of interest is a three wave mixing process involving two fields at optical frequencies and one field at microwave frequencies. In order to boost the efficiency of the frequency conversion process the Er3+:Y2SiO5 crystal is placed inside a microwave and an optical resonator. The problem is first explored from the theoretical point of view, where a nonlinear coefficient Λ(2) is derived (analogous to the 𝜒(2) often used in nonlinear optics), and the interaction between cavity modes and the nonlinear medium is studied. It is predicted that with a sample cooled down to millikelvin temperatures total frequency conversion between microwave and optical fields can be achieved. A preliminary hole burning spectroscopy experiment is performed with the objective of reconstructing the hyperfine structure of the excited state of 167Er3+:Y2SiO5, but the complexity of the problem makes it too difficult to achieve this goal. Then a series of experiments are shown, aimed at determining whether or not frequency conversion at the single photon level is achievable using the even isotopes of erbium in a magnetic field. These experiments are based in the Raman heterodyne spectroscopy technique, which is used in combination with electron paramagnetic resonance and optical absorption spectroscopy. In all experiments the sample is cooled down to cryogenic temperatures near 4 K. A first experiment shows that the frequency conversion process exists in Er3+:Y2SiO5, in a setup where only a microwave resonator is used, but not an optical one. A second experiment is performed in a similar setup, this time presenting a quantitative study of the properties of the frequency conversion process, and its comparison with the theoretical model previously derived. A third experiment is performed, which incorporates an optical cavity to the system. The interaction between the erbium ions and the optical cavity introduces a whole new range of experimental complications, which are studied and discussed. Then, the frequency conversion signal is studied anew, showing an unexpected highly non-linear scaling behaviour with the input powers. A hypothesis explaining this unexpected behaviour is given, referring to stray optical absorption in the inhomogeneous line of Er3+:Y2SiO5 (and in particular 167Er3+:Y2SiO5), which can be bleached out under certain circumstances due to spectral hole burning effects. The overall maximum frequency conversion efficiency observed is of 3 × 10^−4 per Watt of pump laser power. While this value is still far from the target several ways of improvement are proposed, including cooling down the system to millikelvin temperatures, increasing the dopant concentration and modifying the geometry of the resonators.
Quantum light-matter interfaces that reversibly map the quantum state of photons onto the quantum states of atoms, are essential components in the quantum engineering toolbox with applications in quantum communication, computing, and quantum-enabled sensing. In this talk I present our progress towards developing on-chip quantum light-matter interfaces based on nanophotonic resonators fabricated in rare-earth-doped crystals known to exhibit the longest optical and spin coherence times in the solid state. We recently demonstrated coherent control of neodymium (Nd3+) ions coupled to yttrium orthosilicate Y2SiO5 (YSO) photonic crystal nano-beam resonator. The coupling of the Nd3+ 883 nm 4I9/2-4F3/2 transition to the nano-resonator results in a 40 fold enhancement of the transition rate (Purcell effect), and increased optical absorption (~80%) - adequate for realizing efficient optical quantum memories via cavity impedance matching. Optical coherence times T2 up to 100 μs with low spectral diffusion were measured for ions embedded in photonic crystals, which are comparable to those observed in unprocessed bulk samples. This indicates that the remarkable coherence properties of REIs are preserved during nanofabrication process. Multi-temporal mode photon storage using stimulated photon echo and atomic frequency comb (AFC) protocols were implemented in these nano-resonators. Our current technology can be readily transferred to Erbium (Er) doped YSO devices, therefore opening the possibility of efficient on-chip optical quantum memory at 1.5 μm telecom wavelength. Integration with superconducting qubits can lead to devices for reversible quantum conversion of optical photons to microwave photons.
Superconducting qubits are currently one of the leading qubit designs, showing great success in some of the world's most powerful quantum computers. Superconducting qubits, however, communicate at microwave frequencies, which is problematic when it comes to the task of long distance communication as unless the communication channel is cryogenically cooled the microwave photons are swamped by thermal noise. Optical photons, on the other hand, are ideal for long distance communication, particularly at frequencies that lie within the telecommunications band. One solution to the superconducting qubits communication problem is to create a device that can convert an input microwave photon into an optical photon with unit quantum efficiency. A device of such could then be used alongside existing optical fibre networks to connect distant superconducting processors. Furthermore, an upconversion device would allow superconducting qubit systems to take advantage of quantum technologies in the optical region, such as optical quantum memories.\n\nSeveral different approaches have been taken in attempts to experimentally implement such a device. Recently a theoretical proposal showed that the strong non-linearities that occur near the collective resonances in fully concentrated rare-earth crystals can be used to efficiently upconvert microwave photons. In this thesis we begin experimental investigations of two fully concentrated rare-earth crystals, GdVO4 and DyPO4, for their application to microwave upconversion.\n\nAbsorption spectra of the two crystals in the optical region are measured using a Fourier transform infrared spectrometer, in order to characterise and explore the possible optical states to be used in the upconversion process. Experiments are then carried out at microwave frequencies to explore the coupling between the collective spin resonances (magnons) that occur within the crystals and a microwave cavity. It is found that not only can the ultrastrong coupling regime be reached in these systems but that the linewidth of the magnon mode is narrow, measuring 35MHz at T = 25mK. This is the first experimental evidence of ultrastrong coupling between a microwave cavity and antiferromagnetic magnon modes in a rare-earth crystal. Furthermore, narrow transition linewidths are a crucial requirement in the proposed upconversion method, therefore the narrow linewidth experimentally measured here is an important validation of the proposals feasibility. \n\nThe results presented in this thesis show that microwave upconversion mediated by fully concentrated rare-earth crystals has an exciting future. Perhaps one day rare-earth crystals will be used to overcome the major communication problem superconducting qubits currently face.