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Probes of nonequilibrium quantum matter and many-body delocalization

Yunxiang Liao

Published Mar 9, 2018• 0 citations
OpenAlex

Abstract

In this thesis, we consider two different topics: the probes of out-of-equilibrium topological matter and many-body-localization (MBL) in higher dimensions. The first part focuses on the two-dimensional (2D) topological Floquet p+ip superfluid induced by an instantaneous quench of the interaction strength. We investigate radio-frequency (rf) spectroscopy, metal-to-superconductor tunneling, and angle-resolved photoemission spectroscopy (ARPES) as probes of this out-of-equilibrium quantum system in both the cold-atomic and solid-state realizations. We notice a single avoided crossing in the Floquet band structure and a population inversion in the occupation of these bands. In addition, the rf spectrum is well captured by a quasiequilibrium approximation and shows a robust gap. We also compute the rf signal when only the lower Floquet band is occupied as well as the tunneling signal. In both cases, the spectra show wildly different behaviors compared with the rf signal from the post-quench state, and the gap disappears for strong quenches. We attribute this to the fact that the distribution function influences the rf but not the tunneling signal. Finally, we look into the ARPES spectrum which exhibits a clear series of Floquet copies. The second part is devoted to interacting fermions in the presence of quenched disorder. We derive a finite-temperature Keldysh response theory for such a system in the delocalized phase, in the form of the Finkel'stein nonlinear sigma model (FNLσM). Applicable to any symmetry class with at least a U(1) symmetry, our formulation automatically incorporates the correct infrared cutoffs for quantum corrections to transport, and provides a framework to study the real and virtual scattering processes. In particular, we are able to rederive from the FNLσM the Altshuler-Aronov-Khmelnitsky equations for dephasing. We then propose a strategy to approach the 2D ergodic-to-MBL transition from the ergodic side. Such a transition is explored as a dephasing catastrophe in an isolated system with short-range interactions. In this case, the self-generated heat bath responsible for dephasing exhibits diffusive (non-Markovian) density fluctuations. We recast the dephasing of quantum interference corrections as a self-interacting polymer loop, and study its critical behavior using renormalization group approach. In dimensions d=4-ε, we identify a nontrivial fixed point corresponding to a finite temperature where the dephasing time diverges. This fixed point can be associated with a toy version of 2D ergodic-to-MBL transition, provided that it survives to ε=2.

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Quantum Dynamics, Localization, and Fractal-mediated Superconductivity and Magnetism

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Isolated, many-body quantum systems, evolving under their intrinsic dynamics, exhibit a multitude of exotic phenomena and raise foundational questions about statistical mechanics. A flurry of theoretical work has been devoted to understanding how these systems reach thermal equilibrium in the absence of coupling to an external bath and, when thermalization does not occur, investigating the emergent non-equilibrium phases of matter. With the advent of synthetic quantum systems, such as ultra-cold atoms in optical lattices or trapped ions, these questions are no longer academic and can be directly studied in the laboratory. This dissertation explores the non-equilibrium phenomena that stem from the interplay between interactions, disorder, symmetry, topology, and external driving. First, we study how strong disorder, leading to many-body localization, can arrest the heating of a Floquet system and stabilize symmetry-protected topological order that does not have a static analogue. We analyze its dynamical and entanglement properties, highlight its duality to a discrete time crystal, and propose an experimental implementation in a cold-atom setting.Quenched disorder and the many-body localized state are crucial ingredients in protecting macroscopic quantum coherence. We explore the stability of many-body localization in two and higher dimensions and analyze its robustness to rare regions of weak disorder.We then study a second example of non-thermal behavior, namely integrability. We show that a class of random spin models, realizable in systems of atoms coupled to an optical cavity, gives rise to a rich dynamical phase diagram, which includes regions of integrability, classical chaos, and of a novel integrable structure whose conservation laws are reminiscent of the integrals of motion found in a many-body localized phase.The third group of disordered, non-ergodic systems we consider, spin glasses, have fascinating connections to complexity theory and the hardness of constraint satisfaction. We define a statistical ensemble that interpolates between the classical and quantum limits of such a problem and show that there exists a sharp boundary separating satisfiable and unsatisfiable phases.

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Disorder Driven Transitions in Non-Equilibrium Quantum Systems

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•Jun 7, 2016•0 citations
In this thesis, we consider two different topics: the probes of out-of-equilibrium topological matter and many-body-localization (MBL) in higher dimensions. The first part focuses on the two-dimensional (2D) topological Floquet p+ip superfluid induced by an instantaneous quench of the interaction strength. We investigate radio-frequency (rf) spectroscopy, metal-to-superconductor tunneling, and angle-resolved photoemission spectroscopy (ARPES) as probes of this out-of-equilibrium quantum system in both the cold-atomic and solid-state realizations. We notice a single avoided crossing in the Floquet band structure and a population inversion in the occupation of these bands. In addition, the rf spectrum is well captured by a quasiequilibrium approximation and shows a robust gap. We also compute the rf signal when only the lower Floquet band is occupied as well as the tunneling signal. In both cases, the spectra show wildly different behaviors compared with the rf signal from the post-quench state, and the gap disappears for strong quenches. We attribute this to the fact that the distribution function influences the rf but not the tunneling signal. Finally, we look into the ARPES spectrum which exhibits a clear series of Floquet copies. The second part is devoted to interacting fermions in the presence of quenched disorder. We derive a finite-temperature Keldysh response theory for such a system in the delocalized phase, in the form of the Finkel'stein nonlinear sigma model (FNLσM). Applicable to any symmetry class with at least a U(1) symmetry, our formulation automatically incorporates the correct infrared cutoffs for quantum corrections to transport, and provides a framework to study the real and virtual scattering processes. In particular, we are able to rederive from the FNLσM the Altshuler-Aronov-Khmelnitsky equations for dephasing. We then propose a strategy to approach the 2D ergodic-to-MBL transition from the ergodic side. Such a transition is explored as a dephasing catastrophe in an isolated system with short-range interactions. In this case, the self-generated heat bath responsible for dephasing exhibits diffusive (non-Markovian) density fluctuations. We recast the dephasing of quantum interference corrections as a self-interacting polymer loop, and study its critical behavior using renormalization group approach. In dimensions d=4-ε, we identify a nontrivial fixed point corresponding to a finite temperature where the dephasing time diverges. This fixed point can be associated with a toy version of 2D ergodic-to-MBL transition, provided that it survives to ε=2.
In this thesis, we consider two topics that involve strong spatial or temporal fluctuations in interacting quantum many-body systems. We first consider far-from equilibrium quantum hydrodynamics in light-driven helical edge states of a 2D topological insulator. We then consider the enhancement of superconducting and magnetic instabilities in fermion systems with random or structured inhomogeneity, driven by the nesting of fractal wave functions. In the first part, we study quantum quenches of helical edge liquids with spin-flip inelastic scattering. Counterpropagating charge packets in helical edges can be created by an ultrashort electric pulse applied across a 2D topological insulator. Localized “hot spots” that form due to scattering enable two types of strongly nonlinear wave dynamics. First, propagating packets develop self-focusing shock fronts. Second, colliding packets with opposite charge can exhibit near-perfect retroreflection, despite strong dissipation. This leads to an interaction-mediated frequency doubling that could be detected experimentally from emitted terahertz radiation. In the second part, we study the enhanced correlation effects in many-fermion systems induced by structured or random inhomogeneities. We consider the interplay of superconductivity and a wide spectrum of critical (multifractal) wave functions (“spectrum-wide quantum criticality,” SWQC) in the one-dimensional Aubry-Andr ́e and power-law random-banded matrix models (PRBMs) with attractive interactions, using self-consistent BCS theory. We find that SWQC survives the incorporation of attractive interactions at the Anderson localization transition, whereas the pairing amplitude is maximized near this transition in both models. Although increasing inhomogeneity always depletes the superfluid stiffness, we find that superconductivity is still controlled by the fractal-enhanced amplitude near the Anderson transition. Our results suggest that SWQC, recently discovered in two-dimensional topological surface-state and nodal superconductor models, can robustly enhance superconductivity. We also study the interplay of magnetic ordering and the spectrum-wide quantum critical wave functions in PRBMs with repulsive Hubbard interaction. We employ self-consistent Hartree-Fock numerics and analytical field theory calculations using a Keldysh Finkel’stein nonlinear sigma model. We find that weak interactions delocalize the system, while strong interaction localizes the system. Ferromagnetism sets in near the Anderson transition, where the ferromagnetic spin susceptibility is also shown to peak. This indicates that ferromagnetic ordering is enhanced by the fractal wave functions. Using the sigma model, we calculate the quantum corrections to the conductance and spin susceptibility. We find that the analytical and numerical results are mutually consistent.
Periodically driven quantum systems provide a versatile platform for engineering and exploring non-equilibrium states of matter that have no equilibrium counterparts– a field commonly re- ferred to as Floquet engineering. The research presented in this thesis addresses the microscopic interpretation of experimental spectroscopic signatures, the stability of these driven states in the presence of strong many-body interactions, and the emergence of novel forms of non-equilibrium criticality encoded in quantum entanglement. The first part of the thesis focuses on the interpretation of time- and angle-resolved photo- emission spectroscopy (tr-ARPES), the primary experimental tool for detecting Floquet–Bloch sidebands (FBs). The measured signal reflects interference between processes occurring both inside the material and in the vacuum. In particular, Floquet-dressed initial states coexist and interfere with Volkov-dressed final states arising from the laser-assisted photoelectric effect (LAPE). Their experimental identification requires careful comparison with theoretical predic- tions. Using graphene as a model Dirac material, we perform a systematic comparison between two theoretical frameworks: the first-order perturbative Born approximation (PB1) and time- dependent nonequilibrium Green’s functions (tdNEGF), and compare them with experimental results. We disentangle intrinsic Floquet states, LAPE, and their interference, and quantify how polarization, incidence angle, and near-surface screening shape the observed spectra. Our findings show that, once matrix elements are included, both methods capture qualitative trends, but tdNEGF is necessary to describe the full energy–momentum-resolved features, including hybridization gaps. While non-interacting systems exhibit well-defined FBs, interacting systems absorb energy and can evolve toward an infinite-temperature state. To study this competition between coherent driving and many-body heating, in the second part we consider a one-dimensional chain of interacting spinless fermions using exact diagonalization (ED) and matrix product state (MPS) methods. We compute time-dependent spectral functions and correlation measures, and compare the spectral width of the many-body excitation continuum with the driving frequency to define low- and high-frequency regimes. In our parameter regime, low-frequency driving leads to strong overlap between Floquet sectors, resulting in rapid heating and loss of coherence. For weakly populated continua, we find a transient timescale for the suppression of FBs. When the driving frequency exceeds the continuum width, FBs are well separated and long-lived. Thefinalpartofthethesisinvestigatesnon-equilibriumphenomenafromaninformation-theoretic perspective. Wereportanewclassofdynamicalphasetransitions,termedtemporalentanglement transitions (TET) characterized by non-analytic reorganizations of the entanglement spectrum, in a periodically driven transverse-field Ising chain. These transitions occur in the spectrum of the entanglement Hamiltonian and are signaled by dynamical spontaneous symmetry breaking, marked by the closure of the Schmidt gap and parity flips. These transitions remain invisible to conventional local observables. Finite-size scaling reveals that TET belong to a universality class with a correlation-length exponent ν = 1, mirroring equilibrium Ising universality despite their purely dynamical origin.
The interaction of time-dependent electromagnetic fields with electrons in quantum materials can give rise to many both fundamentally interesting as well as technologically relevant phenomena like transient band structure manipulations or the emergence of prethermal states of matter, which are not a result of heating. This thesis contributes theoretical insights to both these topics: We model the interference of Floquet and Volkov side bands, which are a result of the dressing of electron states by light, in a time-resolved angle-resolved photoemission spectroscopy (ARPES) experiment. Furthermore, we analyze the emergence of a band-like feature in the non-equilibrium spectral function of a one-dimensional charge-density wave insulator upon periodic driving. Secondly, we use the fermionic truncated Wigner approximation (fTWA), a phase space method for the time evolution of interacting fermions, to study the light-induced order parameter dynamics in SU(N)-symmetric fermionic lattice models. By comparison with exact analytical results for an interaction quench in the Hubbard model, we find that dephasing-induced prethermalization is correctly described by fTWA. We discuss photoinduced prethermal transitions between competing phases of matter in the large-N Hubbard-Heisenberg model and find a pronounced frequency-dependence of the transition. This work contributes to a better understanding of photoinduced order parameter dynamics from a microscopic perspective.
This thesis reports on first experiments on the observation of ergodicity breaking in a two-component, interacting fermionic gas of Potassium-40 subject to quasi-periodic optical lattices in one and two dimensions, demonstrating the breakdown of thermalization in highly excited states of isolated quantum systems. Our observations can be explained by the phenomenon of many-body localization, a non-ergodic phase of matter, whose properties can be detected with non-equilibrium probes. To probe such a phase, we first design a far-from-equilibrium initial state and then monitor how much the system remembers of this design during time evolution. This allows us to identify regimes and timescales where disorder can protect local quantum information and distinguish such cases from regimes where interactions amalgamate local information into highly nonlocal quantum correlations. We then describe how this treatment systematically breaks down in all real-world systems as the system is (necessarily) coupled to some bath-like structure. Following very recent developments, we are further able to show that order can exist even in driven quantum systems, which were earlier thought to exhibit no interesting features, corresponding to an infinite temperature state. We also extend the experimental realm to explore two dimensions and show that the dynamics emerge as a distinct interplay of interactions, disorder, and dimensions. Upon probing a putative MBL transition, we further show signatures of a new kind of slow relaxation, potentially arising due to randomness in the initial state. We close with some theoretical results on probing quantum dynamics ensuing in the absence of transport and a discussion of exciting areas for future experiments.
Isolated, many-body quantum systems, evolving under their intrinsic dynamics, exhibit a multitude of exotic phenomena and raise foundational questions about statistical mechanics. A flurry of theoretical work has been devoted to understanding how these systems reach thermal equilibrium in the absence of coupling to an external bath and, when thermalization does not occur, investigating the emergent non-equilibrium phases of matter. With the advent of synthetic quantum systems, such as ultra-cold atoms in optical lattices or trapped ions, these questions are no longer academic and can be directly studied in the laboratory. This dissertation explores the non-equilibrium phenomena that stem from the interplay between interactions, disorder, symmetry, topology, and external driving. First, we study how strong disorder, leading to many-body localization, can arrest the heating of a Floquet system and stabilize symmetry-protected topological order that does not have a static analogue. We analyze its dynamical and entanglement properties, highlight its duality to a discrete time crystal, and propose an experimental implementation in a cold-atom setting.Quenched disorder and the many-body localized state are crucial ingredients in protecting macroscopic quantum coherence. We explore the stability of many-body localization in two and higher dimensions and analyze its robustness to rare regions of weak disorder.We then study a second example of non-thermal behavior, namely integrability. We show that a class of random spin models, realizable in systems of atoms coupled to an optical cavity, gives rise to a rich dynamical phase diagram, which includes regions of integrability, classical chaos, and of a novel integrable structure whose conservation laws are reminiscent of the integrals of motion found in a many-body localized phase.The third group of disordered, non-ergodic systems we consider, spin glasses, have fascinating connections to complexity theory and the hardness of constraint satisfaction. We define a statistical ensemble that interpolates between the classical and quantum limits of such a problem and show that there exists a sharp boundary separating satisfiable and unsatisfiable phases.
This thesis presents studies of the role of disorder in non-equilibrium quantum systems. The quantum states relevant to dynamics in these systems are very different from the ground state of the Hamiltonian. Two distinct systems are studied, (i) periodically driven Hamiltonians in two dimensions, and (ii) electrons in a one-dimensional lattice with power-law decaying hopping amplitudes. In the first system, the novel phases that are induced from the interplay of periodic driving, topology and disorder are studied. In the second system, the Anderson transition in all the eigenstates of the Hamiltonian are studied, as a function of the power-law exponent of the hopping amplitude. In periodically driven systems the study focuses on the effect of disorder in the nature of the topology of the steady states. First, we investigate the robustness to disorder of Floquet topological insulators (FTIs) occurring in semiconductor quantum wells. Such FTIs are generated by resonantly driving a transition between the valence and conduction band. We show that when disorder is added, the topological nature of such FTIs persists as long as there is a gap at the resonant quasienergy. For strong enough disorder, this gap closes and all the states become localized as the system undergoes a transition to a trivial insulator. Interestingly, the effects of disorder are not necessarily adverse, disorder can also induce a transition from a trivial to a topological system, thereby establishing a Floquet Topological Anderson Insulator (FTAI). Such a state would be a dynamical realization of the topological Anderson insulator. We identify the conditions on the driving field necessary for observing such a transition. We realize such a disorder induced topological Floquet spectrum in the driven honeycomb lattice and quantum well models. Finally, we show that two-dimensional periodically driven quantum systems with spatial disorder admit a unique topological phase, which we call the anomalous Floquet-Anderson insulator (AFAI). The AFAI is characterized by a quasienergy spectrum featuring chiral edge modes coexisting with a fully localized bulk. Such a spectrum is impossible for a time-independent, local Hamiltonian. These unique characteristics of the AFAI give rise to a new topologically protected nonequilibrium transport phenomenon: quantized, yet nonadiabatic, charge pumping. We identify the topological invariants that distinguish the AFAI from a trivial, fully localized phase, and show that the two phases are separated by a phase transition. The thesis also present the study of disordered systems using Wegner's Flow equations. The Flow Equation Method was proposed as a technique for studying excited states in an interacting system in one dimension. We apply this method to a one-dimensional tight binding problem with power-law decaying hoppings. This model presents a transition as a function of the exponent of the decay. It is shown that the the entire phase diagram, i.e. the delocalized, critical and localized phases in these systems can be studied using this technique. Based on this technique, we develop a strong-bond renormalization group that procedure where we solve the Flow Equations iteratively. This renormalization group approach provides a new framework to study the transition in this system.