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Annual Meeting Optical Society of America

Instabilities of counterpropagating vector waves in a nonlinear Kerr medium

Alexander L. Gaeta, Robert W. Boyd, Jay R. Ackerhalt, Peter W. Milonni

Published Jan 1, 1986• 1 citation
Publisher

Abstract

Instabilities in the interaction of counterpropagating laser beams in a nonlinear medium can have important consequences for nonlinear optical processes such as optical bistability and phase conjugation. We have performed a theoretical study of the polarization characteristics of two counterpropagating waves in an isotropic Kerr medium in order to determine the stability of the multivalued solutions found by previous workers.1 Our method involves numerical integration of the coupled-amplitude equations describing the spatial and temporal evolution of the counterpropagating vector waves.2 Our results show that the multiply stable solutions for the output polarizations of the two vector fields show hysteresis, and that the order in which the two fields are turned on determines which solution is reached. For even higher input intensities we find that the output polarizations fluctuate in time.

DOI
10.1364/oam.1986.mf6

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The steady-state polarizations of fields counterpropagating in nonlinear Kerr media can exhibit complicated behavior.1 We examine the temporal behavior for the case of an isotropic nonlinear Kerr medium and show that the polarizations are temporally unstable above a certain threshold intensity, even when the input polarizations are linear and parallel to each other. This polarization configuration is known to be spatially stable and is often chosen for the two strong pump waves in phase conjugation by degenerate four-wave mixing. We find that the threshold intensity for the polarization instability is approximately the intensity at which the phase conjugate reflectivity is equal to unity. Depending on the ratio of the two input intensities, this instability just above threshold can manifest itself as an abrupt rotation of the output polarizations to a new steady-state value or as a periodic oscillation of the output polarizations. At higher intensities the polarization can evolve chaotically in time, and depending on the ratio of the transit time through the medium to the response time of the medium the output intensity can fluctuate chaotically as well.

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We have observed that the polarizations and intensities of counterpropagating laser beams in sodium vapor are temporally unstable. The output from a stabilized dye laser tuned near to the 3S1/2 → 3P1/2 atomic transition was split to form the two counterpropagating beams. These beams were polarized with the same linear polarization and were weakly focused to a spot size of ~750 μm in sodium vapor having a density of ~3 × 1013 cm−3. We monitored the light generated in the polarization orthogonal to that of the pump beams. For a detuning of 1.01 GHz to the high-frequency side of the 3S1/2(F = 2) → 3P1/2(F = 2) transition and a power of 160 mW in one of the beams, we found that the threshold for the instability occurred at a power of 15 mW in the other beam. Slightly above threshold, the instability was found to be periodic in nature. As the intensity in the counterpropagating beam was increased far above the threshold value, wild fluctuations in the polarizations and intensities of the transmitted beams were observed. We have found that these fluctuations are chaotic and that the system evolves on a strange attractor whose dimension increases with increasing laser power. These observations are in qualitative agreement with the theoretical predictions of Gaeta et al.,1 which predict that the polarizations of counterpropagating beams in a Kerr medium are unstable to the growth of temporal fluctuations.

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•Jan 1, 1991•0 citations
Instabilities in the interaction of counterpropagating laser beams in a nonlinear medium can have important consequences for nonlinear optical processes such as optical bistability and phase conjugation. We have performed a theoretical study of the polarization characteristics of two counterpropagating waves in an isotropic Kerr medium in order to determine the stability of the multivalued solutions found by previous workers.1 Our method involves numerical integration of the coupled-amplitude equations describing the spatial and temporal evolution of the counterpropagating vector waves.2 Our results show that the multiply stable solutions for the output polarizations of the two vector fields show hysteresis, and that the order in which the two fields are turned on determines which solution is reached. For even higher input intensities we find that the output polarizations fluctuate in time.
The steady-state polarizations of fields counterpropagating in nonlinear Kerr media can exhibit complicated behavior.1 We examine the temporal behavior for the case of an isotropic nonlinear Kerr medium and show that the polarizations are temporally unstable above a certain threshold intensity, even when the input polarizations are linear and parallel to each other. This polarization configuration is known to be spatially stable and is often chosen for the two strong pump waves in phase conjugation by degenerate four-wave mixing. We find that the threshold intensity for the polarization instability is approximately the intensity at which the phase conjugate reflectivity is equal to unity. Depending on the ratio of the two input intensities, this instability just above threshold can manifest itself as an abrupt rotation of the output polarizations to a new steady-state value or as a periodic oscillation of the output polarizations. At higher intensities the polarization can evolve chaotically in time, and depending on the ratio of the transit time through the medium to the response time of the medium the output intensity can fluctuate chaotically as well.
Optical phase conjugation by four-wave mixing in a Kerr medium is considered. Two strong counterpropagating lasers pump a nonlinear medium in which they excite the third-order polarization. Mixing with a weak incident field then generates the phase-conjugated image of that field. It is shown how the polarization of the pumps and the tensorial nature of the nonlinear interaction can be accounted for by a geometrical polarization tensor. The electric field is shown to obey two coupled wave equations, which couple a positive- and negative-frequency component of the field. These wave equations allow plane-wave solutions, and we derive the dispersion relation for the wave vectors of these modes. By matching the field of such a mode across the boundaries of the medium to an external incident field, we are able to obtain analytically the Fresnel coefficients for reflection and transmission. Our expressions reduce to earlier results in the appropriate limits.
We have observed that the polarizations and intensities of counterpropagating laser beams in sodium vapor are temporally unstable. The output from a stabilized dye laser tuned near to the 3S1/2 → 3P1/2 atomic transition was split to form the two counterpropagating beams. These beams were polarized with the same linear polarization and were weakly focused to a spot size of ~750 μm in sodium vapor having a density of ~3 × 1013 cm−3. We monitored the light generated in the polarization orthogonal to that of the pump beams. For a detuning of 1.01 GHz to the high-frequency side of the 3S1/2(F = 2) → 3P1/2(F = 2) transition and a power of 160 mW in one of the beams, we found that the threshold for the instability occurred at a power of 15 mW in the other beam. Slightly above threshold, the instability was found to be periodic in nature. As the intensity in the counterpropagating beam was increased far above the threshold value, wild fluctuations in the polarizations and intensities of the transmitted beams were observed. We have found that these fluctuations are chaotic and that the system evolves on a strange attractor whose dimension increases with increasing laser power. These observations are in qualitative agreement with the theoretical predictions of Gaeta et al.,1 which predict that the polarizations of counterpropagating beams in a Kerr medium are unstable to the growth of temporal fluctuations.
Optical bistability based on the cross-interaction of two counterpropagating plane waves in a Kerr-like medium is considered. It is shown that the "input-output" characteristics of such a system have not only multivalued hysteretic response (which was demonstrated by Winful and Marburger in 1980), but also multiple isolated branches (so called isolas) with nonhysteretic jumps from these branches to the main curve (but not vice versa). The isolas were found both in the case in which the problem can be solved analytically (particularly for electrostriction mechanism of optical nonlinearity) and in the general case of arbitrary light-induced anisotropy.
The dynamical behavior of counterpropagating light waves interacting with a nonlinear medium is studied numerically. It is found that the wave and the medium form a system that becomes unstable under certain conditions and exhibits self-oscillation. Because the interacting medium is modeled by an ensemble of two-level systems, we recognize the self-oscillation frequency as the Rabi-frequency of the constituent systems. The physical mechanisms responsible for this self-oscillation are the gain and the distributed feedback of the combined lightwave-medium system. When the environment changes, in particular when the intensity is increased, this system becomes more unstable and we find that the oscillation exhibits more complex behavior, including quasi-periodic motion and chaos. We analyze the output fields by using Fourier spectra, phase portraits, and autocorrelation functions. In the chaotic regime, the Lyapunov exponents and dimensions are also calculated. A physical interpretation of the quasiperiodic motion is given by an exact calculation of the absorption spectrum of our two-level medium. The negative absorption (gain) peaks are found at the frequencies of the quasi-periodic motions, thus implying that the gain of the combined light-medium system is responsible at least in part for the observed complex behavior. In addition, we investigate the stability of the propagating plane wave when a transverse wave is added to the system as a perturbation. Instabilities are analyzed by linearizing the nonlinear equations which model the lightwave-medium system. The results show that the instability is highly-correlated with the four-wave mixing phase conjugation.